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arXiv:0707.0792 · Physical Review Letters

Theory of rf-Spectroscopy of Strongly Interacting Fermions

Matthias Punk, W. Zwerger

Published Oct 25, 2007• 126 citations
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Abstract

We show that strong pairing correlations in Fermi gases lead to the appearance of a gaplike structure in the rf spectrum, both in the balanced superfluid and in the normal phase above the Clogston-Chandrasekhar limit. The average rf shift of a unitary gas is proportional to the ratio of the Fermi velocity and the scattering length with the final state. In the strongly imbalanced case, the rf spectrum measures the binding energy of a minority atom to the Fermi sea of majority atoms. Our results provide a qualitative understanding of recent experiments by Schunck et al.

DOI
10.1103/physrevlett.99.170404

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We show that strong pairing correlations in Fermi gases lead to the appearance of a gaplike structure in the rf spectrum, both in the balanced superfluid and in the normal phase above the Clogston-Chandrasekhar limit. The average rf shift of a unitary gas is proportional to the ratio of the Fermi velocity and the scattering length with the final state. In the strongly imbalanced case, the rf spectrum measures the binding energy of a minority atom to the Fermi sea of majority atoms. Our results provide a qualitative understanding of recent experiments by Schunck et al.
We calculate the radio-frequency spectrum of balanced and imbalanced ultracold Fermi gases in the normal phase at unitarity. For the homogeneous case the spectrum of both the majority and minority components always has a single peak even in the pseudogap regime. We furthermore show how the double-peak structures observed in recent experiments arise due to the inhomogeneity of the trapped gas. The main experimental features observed above the critical temperature in the recent experiment of Schunck et al. [Science 316, 867 (2007)] are recovered with no fitting parameters.
After an introduction into 100 years of research on superfluidity and the concept of the BCS-BEC crossover, we describe recent experimental studies of a spin-polarized Fermi gas with strong interactions. Tomographically resolving the spatial structure of an inhomogeneous trapped sample, we have mapped out the superfluid phases in the parameter space of temperature, spin polarization, and interaction strength. Phase separation between the superfluid and the normal component occurs at low temperatures, showing spatial discontinuities in the spin polarization. The critical polarization of the normal gas increases with stronger coupling. Beyond a critical interaction strength all minority atoms pair with majority atoms, and the system can be effectively described as a boson-fermion mixture. Pairing correlations have been studied by rf spectroscopy, determining the fermion pair size and the pairing gap energy in a resonantly interacting superfluid.
This thesis studies radio-frequency spectroscopy of superfluid alkali Fermi gases. Radio-frequency and laser fields provide a coherent and well understood tool for manipulating atomic gases. However, new phenomena are expected and have already been seen experimentally when the alkali atoms become strongly interacting. Here we use a simple perturbative treatment of the atom-rf-field coupling for studying the spectroscopy of a strongly interacting gas. At ultracold temperatures fermionic atoms become paired in analogy to electrons in superconductors. The resulting binding energy, or the pairing gap, can be observed as a shift in the radio-frequency spectrum. With strong interactions, the fermions begin pairing already above the critical superfluid transition temperature. The radio-frequency spectroscopy grants a way to study these fluctuation effects quantitatively. The inhomogeneous trapping potential of the atom cloud also adds its own flavour, resulting in distinct mesoscopic effects in the radio-frequency spectra. Our theoretical models are in very good agreement with the experimental results. First order perturbation theory provides qualitatively correct lineshapes, and our generalised perturbative approach gives quantitatively correct magnitudes for the transfer rates. The inhomogeneity plays an important part also in more exotic systems in which the simple BCS-type pairing of atoms is prevented by polarising the gas. Superfluidity and phase separation in such spin-imbalanced gases has been experimentally observed. We have suggested the use of radio-frequency spectroscopy for observing exotic polarised superfluid states, present at the edges of the atom cloud.
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We examine pairing and molecule formation in strongly interacting Fermi gases, and we discuss how radio-frequency (rf) spectroscopy can reveal these features. For the balanced case, the emergence of stable molecules in the Bose-Einstein condensation regime results in a two-peak structure in the rf spectrum with clearly visible medium effects on the low-energy part of the molecular wave function. For the highly imbalanced case, we show the existence of a well-defined quasiparticle (a spin polaron) on both sides of the Feshbach resonance, we evaluate its lifetime, and we illustrate how its energy may be measured by rf spectroscopy.
We used radio-frequency spectroscopy to study pairing in the normal and superfluid phases of a strongly interacting Fermi gas with imbalanced spin populations. At high spin imbalances, the system does not become superfluid even at zero temperature. In this normal phase, full pairing of the minority atoms was observed. Hence, mismatched Fermi surfaces do not prevent pairing but can quench the superfluid state, thus realizing a system of fermion pairs that do not condense even at the lowest temperature.