This thesis studies radio-frequency spectroscopy of superfluid alkali Fermi gases. Radio-frequency and laser fields provide a coherent and well understood tool for manipulating atomic gases. However, new phenomena are expected and have already been seen experimentally when the alkali atoms become strongly interacting. Here we use a simple perturbative treatment of the atom-rf-field coupling for studying the spectroscopy of a strongly interacting gas. At ultracold temperatures fermionic atoms become paired in analogy to electrons in superconductors. The resulting binding energy, or the pairing gap, can be observed as a shift in the radio-frequency spectrum. With strong interactions, the fermions begin pairing already above the critical superfluid transition temperature. The radio-frequency spectroscopy grants a way to study these fluctuation effects quantitatively. The inhomogeneous trapping potential of the atom cloud also adds its own flavour, resulting in distinct mesoscopic effects in the radio-frequency spectra. Our theoretical models are in very good agreement with the experimental results. First order perturbation theory provides qualitatively correct lineshapes, and our generalised perturbative approach gives quantitatively correct magnitudes for the transfer rates. The inhomogeneity plays an important part also in more exotic systems in which the simple BCS-type pairing of atoms is prevented by polarising the gas. Superfluidity and phase separation in such spin-imbalanced gases has been experimentally observed. We have suggested the use of radio-frequency spectroscopy for observing exotic polarised superfluid states, present at the edges of the atom cloud.
This thesis studies radio-frequency spectroscopy of superfluid alkali Fermi gases. Radio-frequency and laser fields provide a coherent and well understood tool for manipulating atomic gases. However, new phenomena are expected and have already been seen experimentally when the alkali atoms become strongly interacting. Here we use a simple perturbative treatment of the atom-rf-field coupling for studying the spectroscopy of a strongly interacting gas. At ultracold temperatures fermionic atoms become paired in analogy to electrons in superconductors. The resulting binding energy, or the pairing gap, can be observed as a shift in the radio-frequency spectrum. With strong interactions, the fermions begin pairing already above the critical superfluid transition temperature. The radio-frequency spectroscopy grants a way to study these fluctuation effects quantitatively. The inhomogeneous trapping potential of the atom cloud also adds its own flavour, resulting in distinct mesoscopic effects in the radio-frequency spectra. Our theoretical models are in very good agreement with the experimental results. First order perturbation theory provides qualitatively correct lineshapes, and our generalised perturbative approach gives quantitatively correct magnitudes for the transfer rates. The inhomogeneity plays an important part also in more exotic systems in which the simple BCS-type pairing of atoms is prevented by polarising the gas. Superfluidity and phase separation in such spin-imbalanced gases has been experimentally observed. We have suggested the use of radio-frequency spectroscopy for observing exotic polarised superfluid states, present at the edges of the atom cloud.
This thesis presents experiments investigating the
phase diagram of ultracold atomic Fermi gases using radio-frequency
spectroscopy. The tunability of many experimental parameters
including the temperature, the interparticle interaction strength
and the relative population of different Fermions allows to access
very different physical regimes. Radio-frequency spectroscopy has
been developed into an ideal tool to probe correlations between
particles in these different phases. In particular, radio-frequency
spectroscopy of highly population imbalanced atomic Fermi systems
gives access to the impurity problem: A single Fermion, or Boson,
immersed in a sea of Fermions constitutes a polaron, which can be
described by Landau's Fermi liquid theory. A critical interaction
strength can be identified separating the regime of a fermionic
polaron and a bosonic polaron. Radio-frequency spectroscopy of the
polarized superfluid phase allows an accurate measure of the
superfluid gap [Delta] and allows to identify the importance of
Hartree Mean-field energies. Furthermore, it is shown how these
different physical regimes are connected.
In this paper we present an overview of radio frequency (RF) spectroscopy in the atomic Fermi superfluids. An ultimate goal is to suggest new directions in the cold gas research agenda from the condensed matter perspective.Our focus is on the experimental and theoretical literature of cold gases and photoemission spectroscopy of the cuprates particularly as it pertains to areas of overlap. This paper contains a systematic overview of the theory of RF spectroscopy, both momentum integrated and momentum resolved. We discuss the effects of traps, population imbalance, final state interactions over the entire range of temperatures and compare theory and experiment. We show that this broad range of phenomena can be accomodated within the BCS-Leggett description of BCS-BEC crossover and that this scheme also captures some of the central observations in photoemission experiments in the cuprates. In this last context, we note that the key themes which have emerged in cuprate photoemission studies involve characterization of the fermionic self energy, of the pseudogap and of the effects of superconducting coherence (in passing from above to below the superfluid transition temperature, Tc).These issues have a counterpart in the cold Fermi gases and it would be most useful in future to use these atomic systems to address these and the more sweeping question of how to describe that anomalous superfluid phase which forms in the presence of a normal state excitation gap.
Ultracold atomic gases provide an ideal system with which to study fundamental many-body physics.Exhibiting universal interactions in clean and controllable environments, long-used simple models as well as more exotic models can now be realized.The interplay between theory and experiment is therefore very active, and, in this thesis, I will detail several works, both exact analytic results and numerical calculations, which have impacts on current experiments.I begin with an introduction to the field including a brief discussion of experiments, the microscopic model of two species of interacting fermions, the BCS-BEC crossover and an overview of the various phases of atomic Fermi gases.I then describe the various results of my theoretical investigations, which are divided into five chapters.First, I describe radio frequency (RF) spectroscopy experiments and how they probe the single-particle spectral function.This leads to my results on an exact feature of the spectral lineshape, a universal large-momentum structure which exists for all states of interacting Fermi systems and has been verified in recent angle-resolved RF experiments.Second, I focus on gases which have a normal Fermi liquid ground state and show that their lineshape exhibits a characteristic jump discontinuity.I illustrate this Fermi surface singularity and the previously mentioned universal large momentum tail with explicit calculations.Third, I turn to the low energy structure of the single-particle spectral function in the superfluid state.I argue that sharp low energy quasiparticle excitations exist across the BCS-BEC crossover using a general argument that includes the interaction of fermions with the low-energy collective mode.This is illustrated with an explicit calculation within an approximation scheme.Fourth, I address the trap-induced inhomogeneity and use a Bogoliubov-deGennes analysis to test if a simple local density approximation (LDA) can provide an adequate description of a spin imbalanced Fermi system.Finally, I discuss dynamics of atomic gases motivated by a recent experiment in which two spin-polarized clouds are allowed to collide with each other.Despite the underlying attractive interactions, the clouds are seen to bounce off of each other.Using a hydrodynamic description, I argue that the short and intermediate time dynamics reflects a metastable state in which the effective interaction is repulsive.It is my hope that the work presented in this thesis can be used to gain key insights which inspire future endeavors.6.2 Time dependence of the center-of-mass positions zσ of the two spin clouds at unitarity for an initial separation z↑ (t = 0) = R z , z↓ (t = 0) = -R z using the upper branch energy functional and damping γ = 1.Red (upper) and blue (lower) curves denote the different spin species. . . . . . . . . . . . . . . .71 6.3 The upper branch energy functional obtained from lowest order constraint variational method.(a), energy as a function of the polarization P for various values of k F a s as indicated in the figure.(b), energy as a function of the interaction parameter k F a s for various values of polarization P as indicated in the figure.(c), phase diagram of the interacting two-component Fermi gases.The two vertical red dashed lines indicates the separation between three phases.For 1/(k F a s ) > 1.124, the system is in the Fermi liquid (FL) phase.For 1.124 > 1/(k F a s ) > 0.91, the system is in the partially polarized phase (PP) and for 1/(k F a s ) < 0.91, the system is fully polarized. . . . . .74 6.4 (Color online) Time dependence of the center-of-mass positions zσ of the two spin clouds for k F (0)a s = 2. . . . . . . . . . . . . . . . . . . . . . . . . . .75 6.5 (Color online) Time dependence of the center-of-mass positions zσ of the two spin clouds for k F (0)a s = 0.5. . . . . . . . . . . . . . . . . . . . . . . . . .
The ability to study ultracold atomic Fermi gases holds the promise of significant advances in testing fundamental theories of many-body quantum physics. Of particular interest are strongly interacting Fermi gases in the BCS to BEC crossover that exhibit a transition to a superfluid state at temperatures near 0.2TF , where TF is the Fermi temperature. This transition, as a fraction of TF, is extremely high compared to any known superfluid or superconductor. These gases are also in a universal regime where the physics is independent of the details of the atomic interactions and is therefore relevant to fields as diverse as condensed matter, nuclear physics and astrophysics. In this thesis, I present an experimental probe of atomic gases that uses momentum-resolved RF spectroscopy to realize an analog of angle-resolved photoemission spectroscopy (ARPES) in materials. This measurement reveals the energy and momentum of single-particle states in the strongly interacting Fermi gas. In condensed matter, ARPES has proved to be one of the most powerful experimental techniques for studying the electronic structure of strongly correlated electron materials. The ability to perform analogous measurements in ultracold Fermi gases constitutes a significant advance in our ability to directly connect ultracold atomic gases to strongly correlated electron systems. Taking advantage of this new measurement technique, I investigate a long-standing problem in the field of strongly interacting fermions, namely whether a pseudogap state consisting of incoherent fermion pairs exists at temperatures above the critical temperature for superfluidity. The photoemission data I present provide strong evidence for this state and have implications for fundamental theories of strongly interacting Fermi gases and strongly correlated electron materials. I also discuss the experimental confirmation of recently predicted universal relations for strongly interacting Fermi gases, as well as some of the first experiments involving atomic Fermi gases with p-wave pairing.
The last chapter focuses on radio-frequency spectroscopy of multi component fermion gases. Rf experiments of 6Li and 40K are first reviewed. We show that rf experiments essentially measure spin correlation functions, and internal symmetries of the interparticle interactions constrain the rf spectrum through sum rules. We self-consistently generate the spin correlation functions for 6Li within Hartree-Fock-BCS approximation. Our calculation reproduces the mean field shift observed in experiments for normal gases, and confirms that a second peak detected at higher frequencies in the rf spectrum at sufficiently low temperatures arises from paired fermions. We define a mean frequency shift by the sum rules, and show that it is proportional to the square of BCS pairing gap. The discrepancy between the mean shift and the peak frequency shift observed in experiment for the condensed phase lies in the broad width of the rf spectrum function.
This dissertation presents the first experiments on radio frequency (rf) spectroscopy of a quasi-two dimensional strongly interacting ultracold atomic Fermi gas. A 50-50 mixture of spin-up and spin-down atoms is confined in a series of pancake-shaped traps produced using an optical standing-wave. To make the system quasi-two dimensional, I adjust the Fermi energy in the weakly confined direction to be comparable to the harmonic oscillator energy level spacing in the tightly confined direction. For a perfectly two dimensional system, at low enough temperature, spin-up and spin-down atoms should form dimers in the ground state of the tightly confined direction. However, in our quasi-two dimensional system I find that the simple dimer theory does not agree with the measured radio-frequency spectra. Instead, the data can be explained by polaron to polaron transitions, which is a many-body effect. Here, a polaron is a spin-down impurity surrounded by a cloud of particle-hole pairs in a spin-up Fermi sea. With this unique strongly interacting quasi-two dimensional system, I am able to study the interplay between confinement induced two-body pairing and many-body physics in confined mesoscopic systems of several hundred atoms, which has not been previously explored and offers new challenges for predictions.