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arXiv:0707.0725 · Journal of Physics Condensed Matter

Quantum dynamics of a qubit coupled with a structured bath

Peihao Huang, H Zheng

Published Sep 4, 2008• 10 citations
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Abstract

The dynamics of an unbiased spin-boson model with Lorentzian spectral density is investigated theoretically in terms of the perturbation theory based on a unitary transformation. The population difference P ( t ) and susceptibility χ '' (ω) are calculated for both the off-resonance case and the on-resonance case Δ∼Ω. The approach is checked by Shiba's relation and the sum rule. As well, the coherent–incoherent transition point α c can be determined.

DOI
10.1088/0953-8984/20/39/395233

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The dynamics of an unbiased spin-boson model with Lorentzian spectral density is investigated theoretically in terms of the perturbation theory based on a unitary transformation. The population difference P ( t ) and susceptibility χ '' (ω) are calculated for both the off-resonance case and the on-resonance case Δ∼Ω. The approach is checked by Shiba's relation and the sum rule. As well, the coherent–incoherent transition point α c can be determined.
A new analytical approach, beyond the rotating wave approximation, based on unitary transformations and the non-markovian master equation for the density operator, is applied to treat the biased spin-boson model with a Lorentzian structured bath for arbitrary detunings at zero temperature. Compared to zero bias, we find that the non-equilibrium dynamics demonstrates two more damping oscillation frequencies and one additional relaxation frequency for non-zero bias. Analytical expressions for the non-markovian dynamics and the corresponding spectrum, the localized-delocalized transition point, the coherent-incoherent transition point, the analytical ground energy, the renormalized tunneling factor and the susceptibility are determined. The sum rule and the Shiba relation are checked in the coherent regime.
The decoherence of a two-state system coupled with a sub-Ohmic bath is investigated theoretically by means of the perturbation approach based on a unitary transformation. It is shown that the decoherence depends strongly and sensitively on the structure of environment. Nonadiabatic effect is treated through the introduction of a function ${\ensuremath{\xi}}_{k}$ which depends on the boson frequency and renormalized tunneling. The results are as follows: (i) the nonequilibrium correlation function P(t)P(t)P(t), the dynamical susceptibility ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$, and the equilibrium correlation function C(t)C(t)C(t) are analytically obtained for $s\ensuremath{\leqslant}1$; (ii) the phase diagram of thermodynamic transition shows the delocalized-localized transition point ${\ensuremath{\alpha}}_{l}$ which agrees with exact results and numerical data from the numerical renormalization group; (iii) the dynamical transition point ${\ensuremath{\alpha}}_{c}$ between coherent and incoherent phase is explicitly given. A crossover from the coherent oscillation to incoherent relaxation appears with increasing coupling (for $\ensuremath{\alpha}>{\ensuremath{\alpha}}_{c}$, the coherent dynamics disappear); (iv) the Shiba's relation and sum rule are exactly satisfied when $\ensuremath{\alpha}\ensuremath{\leqslant}{\ensuremath{\alpha}}_{c}$; (v) an underdamping-overdamping transition point ${\ensuremath{\alpha}}_{c}^{*}$ exists in the function $S(\ensuremath{\omega})$. Consequently, the dynamical phase diagrams in both ohmic and sub-Ohmic case are mapped out. For $\ensuremath{\Delta}⪡{\ensuremath{\omega}}_{c}$, the critical couplings (${\ensuremath{\alpha}}_{l},{\ensuremath{\alpha}}_{c}$, and ${\ensuremath{\alpha}}_{c}^{*}$) are proportional to ${\ensuremath{\Delta}}^{1\ensuremath{-}s}$.
The dynamics of the (sub-)Ohmic spin-boson model under various bath initial conditions is investigated by employing the Dirac–Frenkel time-dependent variational approach with the multiple Davydov D1 Ansatz in the interaction picture. The validity of our approach is carefully checked by comparing the results with those of the hierarchy equations of motion method. By analyzing the features of nonequilibrium dynamics, we identify the phase diagrams for different bath initial conditions. We find that for the spectral exponent s < sc, there exists a transition from coherent to quasicoherent dynamics with increasing coupling strengths. For sc < s ≤ 1, the coherent to incoherent crossover occurs at a certain coupling strength and the quasicoherent dynamics emerges at much larger couplings. The initial preparation of the bath has a considerable influence on the dynamics.
We report the results of a study of the dynamics of a two-state system coupled to an environment with peaked spectral density. An exact analytical expression for the bath correlation function is obtained. Validity range of various approximations to the correlation function for calculating the population difference of the system are discussed as function of tunneling splitting, oscillator frequency, coupling constant, damping rate and the temperature of the bath. An exact expression for the population difference for a limited range of parameters, is derived.
The non-Markovian dynamics of the driven spin-boson model at zero and finite temperature is investigated theoretically. Based on a unitary transformation and convolution theorem, the analytical expression of population difference in Laplace space is obtained. This method provides a tool to help us to understand the interference between driving and dissipation within the non-Markovian frame. We study the transient and the steady-state non-Markovian dynamics of population difference P ( t ) in the case of different temperature, driving and spin–bath coupling (SBC) strength. It has been shown that it is necessary to use non-Markovian methods when SBC is strong. At zero temperature, the curve of steady-state amplitude P lt versus Rabi driving amplitude Ω is N-like shaped. While at finite temperature, the curve becomes Λ-like shaped. These curves come from the interference between driving and dissipation. Also, from the interference pattern above, we know that large coherent oscillations can be obtained by optimizing the parameters: Rabi driving amplitude, temperature and SBC strength.
We consider a qubit coupled to a nonlinear quantum oscillator, the latter coupled to an Ohmic bath, and investigate the qubit dynamics. This composed system can be mapped onto that of a qubit coupled to an effective bath. An approximate mapping procedure to determine the spectral density of the effective bath is given. Specifically, within a linear response approximation the effective spectral density is given by knowledge of the linear susceptibility of the nonlinear quantum oscillator. To determine the actual form of the susceptibility, we consider its periodically driven counterpart, which is the problem of the quantum Duffing oscillator within linear response theory in the driving amplitude. Knowing the effective spectral density, the qubit dynamics is investigated. In particular, an analytic formula for the qubit's population difference is derived. Within the regime of validity of our theory, a very good agreement is found with predictions obtained from a Bloch-Redfield master equation approach applied to the composite qubit-nonlinear oscillator system.