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arXiv:0706.0528 · Physical Review Letters

Heralded Entanglement between Atomic Ensembles: Preparation, Decoherence, and Scaling

Julien Laurat, Kyung Soo Choi, Hui Deng, C. W. Chou, Harry J. Kimble

Published Nov 2, 2007• 356 citations
arXivHTMLPDF

Abstract

Heralded entanglement between collective excitations in two atomic ensembles is probabilistically generated, stored, and converted to single-photon fields. By way of the concurrence, quantitative characterizations are reported for the scaling behavior of entanglement with excitation probability and for the temporal dynamics of various correlations resulting in the decay of entanglement. A lower bound of the concurrence for the collective atomic state of 0.9+/-0.3 is inferred. The decay of entanglement as a function of storage time is also observed, and related to the local dynamics.

DOI
10.1103/physrevlett.99.180504

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Heralded entanglement between collective excitations in two atomic ensembles is probabilistically generated, stored, and converted to single-photon fields. By way of the concurrence, quantitative characterizations are reported for the scaling behavior of entanglement with excitation probability and for the temporal dynamics of various correlations resulting in the decay of entanglement. A lower bound of the concurrence for the collective atomic state of 0.9+/-0.3 is inferred. The decay of entanglement as a function of storage time is also observed, and related to the local dynamics.
Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.
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We report significant improvements in the retrieval efficiency of a single excitation stored in an atomic ensemble and in the subsequent generation of strongly correlated pairs of photons. A 50% probability of transforming the stored excitation into one photon in a well-defined spatio-temporal mode at the output of the ensemble is demonstrated. These improvements are illustrated by the generation of high-quality heralded single photons with a suppression of the two-photon component below 1% of the value for a coherent state. A broad characterization of our system is performed for different parameters in order to provide input for the future design of realistic quantum networks.
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