We report significant improvements in the retrieval efficiency of a single excitation stored in an atomic ensemble and in the subsequent generation of strongly correlated pairs of photons. A 50% probability of transforming the stored excitation into one photon in a well-defined spatio-temporal mode at the output of the ensemble is demonstrated. These improvements are illustrated by the generation of high-quality heralded single photons with a suppression of the two-photon component below 1% of the value for a coherent state. A broad characterization of our system is performed for different parameters in order to provide input for the future design of realistic quantum networks.
We report significant improvements in the retrieval efficiency of a single excitation stored in an atomic ensemble and in the subsequent generation of strongly correlated pairs of photons. A 50% probability of transforming the stored excitation into one photon in a well-defined spatio-temporal mode at the output of the ensemble is demonstrated. These improvements are illustrated by the generation of high-quality heralded single photons with a suppression of the two-photon component below 1% of the value for a coherent state. A broad characterization of our system is performed for different parameters in order to provide input for the future design of realistic quantum networks.
Summary form only given. Strong interaction between two single photons [1], is a long standing and important goal in quantum photonics. This would enable a new regime of nonlinear optics and unlock several applications in quantum information science, including photon-photon gates and deterministic Bell-state measurements for quantum networking. In the context of quantum networks [2], a particularly important case is to achieve strong interaction between single photons from independent photon pairs that can be stored in quantum memories. So far, most of the efforts towards nonlinear effects at the single-photon level have been realized using weak classical input light.In this contribution, we demonstrate the storage and retrieval of a paired single photon emitted by an ensemble quantum memory in a strongly nonlinear medium based on highly excited Rydberg atomic excitations [3,4]. We demonstrate that non-classical correlations between the two photons persist after the retrieval from the Rydberg ensemble. We show that our Rydberg cold atomic ensemble displays optical nonlinearity with input pulses containing few tens of photons. Our results [5], mark an important step towards deterministic photonphoton interactions, and may enable deterministic Bell-state measurement with multimode quantum memories.
Single photons are the best carriers of quantum information for long-distance transmission. Nevertheless, maximal achievable distance is limited by the exponential decay of photons as a function of link length. The protocol of quantum repeater provides a promising solution by replacing direction transmission with segmented entanglement distribution and entanglement connection via swapping. The quantum repeater necessitates a key element of quantum memory for making efficient interconnections. An atomic ensemble is very suitable for this purpose due to the collective enhanced interaction. Single photons are stored as collective excitations in an atomic ensemble. Thus a comprehensive study of the physics relating to collective excitations is crucially important for improving the quantum memory performance and its reachable applications in quantum repeater and quantum network. In this article, we review our experimental work on cold atomic ensembles in recent years, focusing on the coherent manipulation of collective excitations. We first briefly introduce the general concept of collective excitations and the preparation process through spontaneous Raman scattering, and we review our experimental work on extending the coherence time, such as suppressing motional dephasing by increasing the spin-wave wavelength, by confining atoms with a three-dimensional optical lattice. Afterwards, we discuss about the retrieval process of collective excitations and review our experiments on using a ring-cavity enhanced setup to improve the retrieval efficiency. The coherent qubit operation in a quantum memory is very useful for enabling new functionalities for a quantum network, in a subsequent section, we thus review our work on developing Raman-based coherent operations for single excitations. Afterwards, we mention our experiments on creating a pair of atom-photon entanglement by interfering two modes of a collective excitation. Improving the entanglement preparation efficiency is crucially important, and Rydberg-based interaction provides a promising solution. Our experimental work in this direction is also reviewed. Additionally, as an application in coherent manipulation with collective excitations, we show several experiments on using excitations in remote atomic memories and demonstrating basic functionality of quantum repeater and quantum network. In short, significant progress has been made in the coherent manipulation of single collective excitations in cold atomic ensembles, and further improvement will be accelerated by the Rydberg-enabled interactions; practical applications in quantum repeater and quantum network is foreseeable in the near future.
Strong interaction between two single photons is a long standing and important goal in quantum photonics. This would enable a new regime of nonlinear optics and unlock several applications in quantum information science, including photonic quantum gates and deterministic Bell-state measurements. In the context of quantum networks, it would be important to achieve interactions between single photons from independent photon pairs storable in quantum memories. So far, most experiments showing nonlinearities at the single-photon level have used weak classical input light. Here we demonstrate the storage and retrieval of a paired single photon emitted by an ensemble quantum memory in a strongly nonlinear medium based on highly excited Rydberg atoms. We show that nonclassical correlations between the two photons persist after retrieval from the Rydberg ensemble. Our result is an important step towards deterministic photon-photon interactions, and may enable deterministic Bell-state measurements with multimode quantum memories.
Atomic ensembles in the form of rare-earth-doped crystals offer significant potential for implementing a quantum memory due to their long coherence lifetimes, enhanced light-matter interaction, and the potential for integration. We use a double Lambda configuration based on hyperfine levels in praseodymium doped yttrium orthosilicate. In this scheme, a probabilistically generated collective excitation of the internal atomic states in the form of a spin-wave is signaled by emission of a Stokes-shifted herald photon via spontaneous Raman scattering. After a storage delay, a read field addresses the appropriate transition, mapping the spin wave back to a photon, resulting in the emission of an anti-Stokes shifted retrieved photon. Momentum conservation, as dictated by phase-matching conditions, ensure that the herald and retrieved photons are emitted in a well-defined spatial modes relative to the co-propagating write and read optical fields. Inhomogeneous broadening of the absorption profile precludes straightforward implementation of the above scheme, and we resort to spectral hole-burning techniques to prepare a sub-ensemble of atoms with a narrow range of optical transition energy in the ground state. Using a second identical crystal, we also implement an optical spectral filter that suppresses the powerful write and read beams, and spontaneous-emission noise, while transmitting the herald and retrieved photons. We report on the second-order optical correlations between the herald and retrieved photons that are the signature of generation and retrieval of a stored spin-wave excitation. Demonstration of such a quantum memory is an enabling step towards distributing entanglement for a quantum repeater scheme.
Heralded entanglement between collective excitations in two atomic ensembles is probabilistically generated, stored, and converted to single-photon fields. By way of the concurrence, quantitative characterizations are reported for the scaling behavior of entanglement with excitation probability and for the temporal dynamics of various correlations resulting in the decay of entanglement. A lower bound of the concurrence for the collective atomic state of 0.9+/-0.3 is inferred. The decay of entanglement as a function of storage time is also observed, and related to the local dynamics.
In order to build long-distance quantum communications, quantum memories are required as a synchronization tool which allows entanglement to be stored and retrieved on-demand, when the system is ready to perform entanglement swapping [1]. The storage-and-retrieval efficiency is a key parameter: an increase from 60% to 90% drastically decreases, typically by 2 orders of magnitude, the average time for entanglement distribution over a distance of 600 kilometers. Within this context, we reported quantum transfer between light and cold-atom-based quantum memory featuring a single mode storage-and-retrieval efficiency as high as 87%(±5%), in the single excitation regime [2]. Moreover, we demonstrated the storage of single-photon entanglement into two memories, with a ratio of the input and output concurrences reaching 88%, a more than three-fold increase compared to prior works (Fig. 1). The demonstrated capability required operating at a very large optical depth (OD) of the atomic ensembles on theD1line of cesium, and with a strong and preserved suppression of the two-photon component.