Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.
Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.
It is crucial for the physical realization of quantum information networks to first establish entanglement among multiple space-separated quantum memories and then, at a user-controlled moment, to transfer the stored entanglement to quantum channels for distribution and conveyance of information. Here we present an experimental demonstration on generation, storage, and transfer of deterministic quantum entanglement among three spatially separated atomic ensembles. The off-line prepared multipartite entanglement of optical modes is mapped into three distant atomic ensembles to establish entanglement of atomic spin waves via electromagnetically induced transparency light-matter interaction. Then the stored atomic entanglement is transferred into a tripartite quadrature entangled state of light, which is space-separated and can be dynamically allocated to three quantum channels for conveying quantum information. The existence of entanglement among three released optical modes verifies that the system has the capacity to preserve multipartite entanglement. The presented protocol can be directly extended to larger quantum networks with more nodes.Continuous-variable encoding is a promising approach for quantum information and communication networks. Here, the authors show how to map entanglement from three spatial optical modes to three separated atomic samples via electromagnetically induced transparency, releasing it later on demand.
The ultimate goal of this research is to develop the essential physical ingredients required for the shared quantum gate processing unit (S-QGPU) architecture for distributed quantum computing. In this architecture, local quantum processors are connected through flying photonic qubits and a shared central gate processor, providing a route toward scalable quantum computation beyond the limitations of isolated local devices. Realizing such an architecture requires two key components: a reliable quantum link between distant nodes and a hybrid controlled gate capable of implementing nonlocal quantum operations.This thesis investigates these two ingredients in cold 87Rb atomic ensembles. The first part focuses on narrowband biphoton generation through spontaneous four-wave mixing in laser-cooled atoms. These biphotons serve as heralded single-photon sources and quantum links between distant nodes, while remaining naturally compatible with atomic quantum memories. A central result of this work is the discovery and analysis of symmetry-protected biphoton coherence time, in which the biphoton coherence becomes immune to loss associated with electromagnetically induced transparency. This effect provides a new mechanism for generating ultranarrow-band quantum light with improved robustness, and enhances both synchronization and light–matter interfacing in the S-QGPU architecture. The role of atomic-state preparation in biphoton generation is also investigated through opticalpumping-based configurations. The second part of this thesis explores atom–photon hybrid controlled gates based on the combination of quantum memory and Rydberg blockade. In these schemes, photonic qubits are mapped onto collective atomic excitations, conditional operations are implemented through strong Rydberg interactions, and the quantum states are subsequently converted back into photonic qubits. These hybrid gate schemes provide the physical mechanism for remotely controlled operations between distant quantum nodes. Together, the narrowband biphoton source and the atom–photon hybrid gate constitute the two essential building blocks of the S-QGPU architecture. This work establishes a physical foundation for distributed quantum computing with cold atomic systems and advances the development of scalable quantum networks based on efficient photon–atom interfaces.
The distribution of entanglement between different parties enables quantum communication protocols, such as quantum key distribution or teleportation. Furthermore, control of entanglement between material systems is an essential capability for scalable architectures. This talk will focus on the experimental gen-eration of such entanglement in different setups, in the regime of single photons or in the regime of continuous variables. The first part will review experiments done recently in the single excitation regime. First, by following the seminal paper of Duan, Lukin, Cirac and Zoller (DLCZ) [1], entanglement between single collective excitations stored in two re-mote atomic ensembles can be generated. In the DLCZ protocol, entanglement is created in a probabilistic but heralded way from quantum interference in the measurement process. The detection of a photon from one or the other atomic ensemble in an indistinguishable fashion results in an entangled state with one collective spin excitation shared coherently [2]. This entanglement has been used for the initial implementation of functional quantum nodes for polarization en-
Quantum entanglement is a significant quantum resource, which plays a central role in quantum communication. For realizing quantum information network, it is important to establish deterministic quantum entanglement among multiple spatial-separated quantum memories, and then the stored entanglement is transferred into the quantum channels for distributing and transmitting the quantum information at the user-control time. Firstly, we introduce the scheme of deterministic generation polarization squeezed state at 795 nm. A pair of quadrature amplitude squeezed optical fields are prepared by two degenerate optical parameter amplifiers pumped by a laser at 398 nm, and then the polarization squeezed state of light appears by combining the generated two quadrature amplitude squeezed optical beams on a polarizing beam splitter. Secondly, we present the experimental demonstration of tripartite polarization entanglement described by Stokes operators of optical field. The quadrature tripartite entangled states of light corresponding to the resonance with D1 line of rubidium atoms are transformed into the continuous-variable polarization entanglement via polarization beam splitter with three bright local optical beams. Finally, we propose the generation, storage and transfer of deterministic quantum entanglement among three spatially separated atomic ensembles. By the method of electromagnetically induced transparency light-matter interaction, the optical multiple entangled state is mapped into three distant atomic ensembles to build the entanglement among three atomic spin waves. Then, the quantum noise of entanglement stored in the atomic ensembles is transferred to the three space-seperated quadrature entangled light fields through three quantum channels. The existence of entanglement among the three released beams verifies that the system has the ability to maintain the multipartite entanglement. This protocol realizes the entanglement among three distant quantum nodes, and it can be extended to quantum network with more quantum nodes. All of these lay the foundation for realizing the large-scale quantum network communication in the future.
We present a convenient and efficient way to exchange and distribute multipartite entangled state via atomic coherence induced by electromagnetically induced transparency (EIT) in an atomic ensemble. By using the EIT-based nondegenerate four-wave mixing processes, the generation, exchange, and distribution of light-light, atom-light, and atom-atom multipartite entanglement can be achieved in a deterministic way with only coherent light fields. This EIT-induced atomic coherence acts as a quantum information processor and has the function of quantum beam splitter, quantum frequency converter, quantum entangler, and quantum repeater, which greatly facilitates the operations in quantum information processing, and holds promising applications in realistic scalable quantum communication and quantum networks
Establishing quantum entanglement between individual nodes is crucial for building large-scale quantum networks, enabling secure quantum communication, distributed quantum computing, enhanced quantum metrology and fundamental tests of quantum mechanics. However, the shared entanglements have been merely observed in either extremely low-temperature or well-isolated systems, which limits the quantum networks for the real-life applications. Here, we report the realization of heralding quantum entanglement between two atomic ensembles at room temperature, where each of them contains billions of motional atoms. By measuring the mapped-out entangled state with quantum interference, concurrence and correlation, we strongly verify the existence of a single excitation delocalized in two atomic ensembles. Remarkably, the heralded quantum entanglement of atomic ensembles can be operated with the feature of delay-choice, which illustrates the essentiality of the built-in quantum memory. The demonstrated building block paves the way for constructing quantum networks and distributing entanglement across multiple remote nodes at ambient conditions.