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arXiv:quant-ph/9901078 · Physical Review A

Two-level atom-field interaction: Exact master equations for non-Markovian dynamics, decoherence, and relaxation

Charis Anastopoulos, B. L. Hu

Published Aug 18, 2000• 93 citations
arXivHTMLPDF

Abstract

We perform a first-principles derivation of the general master equation to study the non-Markovian dynamics of a two-level atom (2LA) interacting with an electromagnetic field (EMF). We use the influence functional method, which can incorporate the full back reaction of the field on the atom, while adopting Grassmannian variables for the 2LA and the coherent-state representation for the EMF. We find exact master equations for the cases of a free quantum field and a cavity field in the vacuum. In response to the search for mechanisms to preserve maximal coherence in quantum computations in ion trap prototypes, we apply these equations to analyze the decoherence of a 2LA in an EMF, and find that decoherence time is close to relaxation time. This is at variance with the claims by authors who studied the same system but used a different coupling model. We explain the source of difference and argue that, contrary to common belief, the EMF, when resonantly coupled to an atom, does not decohere it as efficiently as a bath does on a quantum Brownian particle. The master equations for non-Markovian dynamics derived here are expected to be useful for exploring new regimes of 2LAEMF interaction, which is becoming physically important experimentally.

DOI
10.1103/physreva.62.033821

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We perform a first-principles derivation of the general master equation to study the non-Markovian dynamics of a two-level atom (2LA) interacting with an electromagnetic field (EMF). We use the influence functional method, which can incorporate the full back reaction of the field on the atom, while adopting Grassmannian variables for the 2LA and the coherent-state representation for the EMF. We find exact master equations for the cases of a free quantum field and a cavity field in the vacuum. In response to the search for mechanisms to preserve maximal coherence in quantum computations in ion trap prototypes, we apply these equations to analyze the decoherence of a 2LA in an EMF, and find that decoherence time is close to relaxation time. This is at variance with the claims by authors who studied the same system but used a different coupling model. We explain the source of difference and argue that, contrary to common belief, the EMF, when resonantly coupled to an atom, does not decohere it as efficiently as a bath does on a quantum Brownian particle. The master equations for non-Markovian dynamics derived here are expected to be useful for exploring new regimes of 2LAEMF interaction, which is becoming physically important experimentally.
In quantum computation, it is of paramount importance to locate the parameter space where maximal coherence can be preserved in the qubit system. In recent years environment-induced decoherence based the quantum Brownian motion (QBM) models have been applied to two level systems (2LS) interacting with an electromagnetic field, leading to the general belief that 2LS are easily decohered. In a recent paper C. Anastopoulos and B. L. Hu [Phys. Rev. A62, (2000) 033821] derived a new exact non-Markovian master equation at zero temperature, from which they showed that this belief is actually misplaced. For a two-level atom (2LA)- electromagnetic field (EMF) system the decoherence time is rather long, comparable to the relaxation time. Theoretically this is because the dominant interaction is the hatsigmapm\\hat \\sigma_{\\pm}hatsigmapm​ type of coupling between the two levels (what constitutes the qubit) and the field, not the hatsigmaz\\hat \\sigma_zhatsigmaz​ type, which shows the QBM behavior. Depending on the coupling the field can act as a resonator (in an atom cavity) or as a bath (in QBM) and produce very different decoherent behavior in the system. This is not new to Cavity QED experimentalists: the 2LA-EMF system maintaining its coherence in sufficiently long duration is the reason why they can manipulate them so well to show interesting quantum coherence effects.
We study the non-Markovian dynamics of a qubit made up of a two-level atom interacting with an electromagnetic field (EMF) initially at finite temperature. Unlike most earlier studies where the bath is assumed to be fixed, we study the complete evolution of the combined qubit-EMF system, thus allowing for the coherent backaction from the bath on the qubit and the qubit on the bath in a self-consistent manner. In this way we can see the development of quantum correlations and entanglement between the system and its environment, and how that affects the decoherence and relaxation of the system. We find nonexponential decay for both the diagonal and nondiagonal matrix elements of the qubit's reduced density matrix in the pointer basis. The former shows the qubit relaxing to thermal equilibrium with the bath, while the latter shows the decoherence rate beginning at the usually predicted thermal rate, but changing to the zero-temperature value as the qubit and bath become entangled. The decoherence and relaxation rates are comparable, as in the zero-temperature case. On the entanglement of a qubit with the EMF we calculated the fidelity and the von Neumann entropy, which is a measure of the purity of the density matrix. The present more accurate non-Markovian calculations predict lower loss of fidelity and purity as compared with the Markovian results. Generally speaking, with the inclusion of quantum correlations between the qubit and its environment, the non-Markovian processes tend to slow down the drive of the system to equilibrium, prolonging the decoherence and better preserving the fidelity and purity of the system.
Decoherence of the dispersive Jaynes–Cummings model which is placed in a lossy cavity is studied by means of the time-convolutionless non-Markovian quantum master equation. The effect of the interaction between a two-level atom and photon field on the damping operator of the quantum master equation is made clear by calculating the decay of coherence and entanglement of the relevant system. It is shown that although the interaction effect on the damping operator is small when the cavity loss has the Markovian property, it becomes significantly large when the cavity loss is subject to the non-Markovian process. Furthermore, the quantum channel of the two-level atom derived by the dispersive Jaynes–Cummings model is investigated. The decay of entanglement of the two two-level atoms is examined to show the importance of the interaction effect on the damping operator.
The reduced dynamics of an atomic qubit coupled both to its own quantized center of mass motion through the spatial mode functions of the electromagnetic field, as well as the vacuum modes, is calculated in the influence functional formalism. The formalism chosen can describe the entangled non-Markovian evolution of the system with a full account of the coherent back-action of the environment on the qubit. We find a slight increase in the decoherence due to the quantized center of mass motion and give a condition on the mass and qubit resonant frequency for which the effect is important. In optically resonant alkali-metal atom systems, we find the effect to be negligibly small. The framework presented here can nevertheless be used for general considerations of the coherent evolution of qubits in moving atoms in an electromagnetic field.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
This dissertation treats quantum open system dynamics, focusing on the coherent evolution of a two-level atom (as the system) interacting with an electromagnetic field (as the bath), for purposes relevant to quantum computing. In order to maintain the quantum correlations that develop between the system and bath throughout the evolution path integral formalisms such as the influence functional and closed time path formalisms are used. Predictions of effects due to the quantum correlations in the composite interacting system are computed. Conventional treatments using Schr\"odinger-master equation and Heisenberg-Langevin approaches usually ignore system+bath quantum correlations as a technical simplification. It is argued that although neglect of system+bath correlations is generally a good approximation when the bath has a large continuous set of degrees of freedom, a residual coherence effect remains due to the non-zero bath correlation time. Though small, these effects are becoming more relevant as, with the advent of ultra cold atom sources, atom optics experiments are reaching levels at which such residual effects are becoming measurable. Three specific problems are investigated in this thesis: First is a self-dressing rederivation of the Casimir-Polder retardation force. The well known stationary atom result is reproduced and a result for a slowly moving atom is obtained which is up to twice the stationary atom correction. Second is the entangled evolution of a qubit with an initially thermal low temperature bath. The diagonal matrix elements are found to thermalize and the off-diagonal elements to decohere as expected, however they do so non-exponentially due to the quantum correlations that develop between the qubit and bath. Third is a calculation of qubit dynamics in the presence of quantized atomic motion as well as zero point fluctuations of the electromagnetic field. The decoherence rate of the qubit is found to increase slightly in that case due to the additional degree of freedom.