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Decoherence of Two-Level Systems Can Be Very Different From Brownian Particles

B. L. Hu

Published Jan 1, 2002• 2 citations
OpenAlex

Abstract

In quantum computation, it is of paramount importance to locate the parameter space where maximal coherence can be preserved in the qubit system. In recent years environment-induced decoherence based the quantum Brownian motion (QBM) models have been applied to two level systems (2LS) interacting with an electromagnetic field, leading to the general belief that 2LS are easily decohered. In a recent paper C. Anastopoulos and B. L. Hu [Phys. Rev. A62, (2000) 033821] derived a new exact non-Markovian master equation at zero temperature, from which they showed that this belief is actually misplaced. For a two-level atom (2LA)- electromagnetic field (EMF) system the decoherence time is rather long, comparable to the relaxation time. Theoretically this is because the dominant interaction is the $\\hat \\sigma_{\\pm}$ type of coupling between the two levels (what constitutes the qubit) and the field, not the $\\hat \\sigma_z$ type, which shows the QBM behavior. Depending on the coupling the field can act as a resonator (in an atom cavity) or as a bath (in QBM) and produce very different decoherent behavior in the system. This is not new to Cavity QED experimentalists: the 2LA-EMF system maintaining its coherence in sufficiently long duration is the reason why they can manipulate them so well to show interesting quantum coherence effects.

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We perform a first-principles derivation of the general master equation to study the non-Markovian dynamics of a two-level atom (2LA) interacting with an electromagnetic field (EMF). We use the influence functional method, which can incorporate the full back reaction of the field on the atom, while adopting Grassmannian variables for the 2LA and the coherent-state representation for the EMF. We find exact master equations for the cases of a free quantum field and a cavity field in the vacuum. In response to the search for mechanisms to preserve maximal coherence in quantum computations in ion trap prototypes, we apply these equations to analyze the decoherence of a 2LA in an EMF, and find that decoherence time is close to relaxation time. This is at variance with the claims by authors who studied the same system but used a different coupling model. We explain the source of difference and argue that, contrary to common belief, the EMF, when resonantly coupled to an atom, does not decohere it as efficiently as a bath does on a quantum Brownian particle. The master equations for non-Markovian dynamics derived here are expected to be useful for exploring new regimes of 2LAEMF interaction, which is becoming physically important experimentally.

arXiv:quant-ph/9901078•Physical Review A•Aug 18, 2000•93 citations

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We study the non-Markovian dynamics of a qubit made up of a two-level atom interacting with an electromagnetic field (EMF) initially at finite temperature. Unlike most earlier studies where the bath is assumed to be fixed, we study the complete evolution of the combined qubit-EMF system, thus allowing for the coherent backaction from the bath on the qubit and the qubit on the bath in a self-consistent manner. In this way we can see the development of quantum correlations and entanglement between the system and its environment, and how that affects the decoherence and relaxation of the system. We find nonexponential decay for both the diagonal and nondiagonal matrix elements of the qubit's reduced density matrix in the pointer basis. The former shows the qubit relaxing to thermal equilibrium with the bath, while the latter shows the decoherence rate beginning at the usually predicted thermal rate, but changing to the zero-temperature value as the qubit and bath become entangled. The decoherence and relaxation rates are comparable, as in the zero-temperature case. On the entanglement of a qubit with the EMF we calculated the fidelity and the von Neumann entropy, which is a measure of the purity of the density matrix. The present more accurate non-Markovian calculations predict lower loss of fidelity and purity as compared with the Markovian results. Generally speaking, with the inclusion of quantum correlations between the qubit and its environment, the non-Markovian processes tend to slow down the drive of the system to equilibrium, prolonging the decoherence and better preserving the fidelity and purity of the system.

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Christen H. Fleming

An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..

•Jan 1, 2011•6 citations

A CRITIQUE OF TWO-LEVEL APPROXIMATION

Kerim Savran, Tugrul Hakioglu

We examine the effect of multilevels on decoherence and dephasing properties of a quantum system consisting of a non-ideal two level subspace, identified as the qubit and a finite set of higher energy levels above this qubit subspace. The whole system is under interaction with an environmental bath through a Caldeira-Leggett type coupling. The model that we use is an rf-SQUID under macroscopic quantum coherence and coupled inductively to a flux noise characterized by an environmental spectrum. The model interaction can generate dipole couplings which can be appreciable for a number of high levels. The decoherence properties of the qubit subspace is examined numerically using the master equation formalism of the system’s reduced density matrix. We numerically examine the relaxation and dephasing times as the environmental frequency spectrum, and the multilevel system parameters are varied at zero temperature. We observe that, these time scales receive contribution from all available energies in the noise spectrum (even well above the system’s energy scales) stressing the dominant role played by the non-resonant (virtual) transitions. The relaxation and dephasing times calculated, strongly depend on the number of levels within the range of levels for which appreciable couplings are produced. Under the influence of these effects, we remark that the validity of the two level approximation is restricted not by the temperature but by these dipole couplings as well as the availability of the environmental modes at low temperatures. © 2005 by World Scientific Publishing Co. Pte. Ltd.

International Symposium on Mesoscopic Superconductivity and Spintronics (MS+S)•Aug 1, 2005•0 citations

Precision of electromagnetic control of a quantum system

Ching-Kit Chan, Lu Jeu Sham

Coherent control of a quantum system is limited both by the decoherence due to environment and the quantum nature of the control agent. The high fidelity of control demanded by fault-tolerant quantum computation and the intrinsic interest in nonclassical effects from the interplay between control and dissipation are motivations for a detailed study of the interaction dynamics between the quantum system and the macroscopic environment and control agent. We present a detailed time-evolution study of a two-level system interacting with a laser pulse and the electromagnetic vacuum in the multimode Jaynes-Cummings model. A diagrammatic formalism allows easy identification of coherent dynamics and relaxation of the two-level system. We demonstrate a computational method of dynamics with precise error bounds for fast operations versus slow decoherence, spanning the Markovian and non-Markovian regimes. Comparison against an exact model solution of our results with existing approximations of the master equation shows the lack of accuracy in the latter.

arXiv:1012.1051•Physical Review A•Sep 22, 2011•10 citations
In quantum computation, it is of paramount importance to locate the parameter space where maximal coherence can be preserved in the qubit system. In recent years environment-induced decoherence based the quantum Brownian motion (QBM) models have been applied to two level systems (2LS) interacting with an electromagnetic field, leading to the general belief that 2LS are easily decohered. In a recent paper C. Anastopoulos and B. L. Hu [Phys. Rev. A62, (2000) 033821] derived a new exact non-Markovian master equation at zero temperature, from which they showed that this belief is actually misplaced. For a two-level atom (2LA)- electromagnetic field (EMF) system the decoherence time is rather long, comparable to the relaxation time. Theoretically this is because the dominant interaction is the hatsigmapm\\hat \\sigma_{\\pm}hatsigmapm​ type of coupling between the two levels (what constitutes the qubit) and the field, not the hatsigmaz\\hat \\sigma_zhatsigmaz​ type, which shows the QBM behavior. Depending on the coupling the field can act as a resonator (in an atom cavity) or as a bath (in QBM) and produce very different decoherent behavior in the system. This is not new to Cavity QED experimentalists: the 2LA-EMF system maintaining its coherence in sufficiently long duration is the reason why they can manipulate them so well to show interesting quantum coherence effects.
We perform a first-principles derivation of the general master equation to study the non-Markovian dynamics of a two-level atom (2LA) interacting with an electromagnetic field (EMF). We use the influence functional method, which can incorporate the full back reaction of the field on the atom, while adopting Grassmannian variables for the 2LA and the coherent-state representation for the EMF. We find exact master equations for the cases of a free quantum field and a cavity field in the vacuum. In response to the search for mechanisms to preserve maximal coherence in quantum computations in ion trap prototypes, we apply these equations to analyze the decoherence of a 2LA in an EMF, and find that decoherence time is close to relaxation time. This is at variance with the claims by authors who studied the same system but used a different coupling model. We explain the source of difference and argue that, contrary to common belief, the EMF, when resonantly coupled to an atom, does not decohere it as efficiently as a bath does on a quantum Brownian particle. The master equations for non-Markovian dynamics derived here are expected to be useful for exploring new regimes of 2LAEMF interaction, which is becoming physically important experimentally.
We study the non-Markovian dynamics of a qubit made up of a two-level atom interacting with an electromagnetic field (EMF) initially at finite temperature. Unlike most earlier studies where the bath is assumed to be fixed, we study the complete evolution of the combined qubit-EMF system, thus allowing for the coherent backaction from the bath on the qubit and the qubit on the bath in a self-consistent manner. In this way we can see the development of quantum correlations and entanglement between the system and its environment, and how that affects the decoherence and relaxation of the system. We find nonexponential decay for both the diagonal and nondiagonal matrix elements of the qubit's reduced density matrix in the pointer basis. The former shows the qubit relaxing to thermal equilibrium with the bath, while the latter shows the decoherence rate beginning at the usually predicted thermal rate, but changing to the zero-temperature value as the qubit and bath become entangled. The decoherence and relaxation rates are comparable, as in the zero-temperature case. On the entanglement of a qubit with the EMF we calculated the fidelity and the von Neumann entropy, which is a measure of the purity of the density matrix. The present more accurate non-Markovian calculations predict lower loss of fidelity and purity as compared with the Markovian results. Generally speaking, with the inclusion of quantum correlations between the qubit and its environment, the non-Markovian processes tend to slow down the drive of the system to equilibrium, prolonging the decoherence and better preserving the fidelity and purity of the system.
Quantum Brownian oscillator model (QBM), in the Fock-space representation, can be viewed as a multilevel spin-boson model. At sufficiently low temperature, the oscillator degrees of freedom are dynamically reduced to the lowest two levels and the system behaves effectively as a two-level (E2L) spin-boson model (SBM) in this limit. We discuss the physical mechanism of level reduction and analyze the behavior of E2L-SBM from the QBM solutions. The availability of close solutions for the QBM enables us to study the non-Markovian features of decoherence and leakage in a SBM in the nonperturbative regime (e.g., without invoking the Born approximation) in better details than before. Our result captures very well the characteristic non-Markovian short time low temperature behavior common in many models.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
We examine the effect of multilevels on decoherence and dephasing properties of a quantum system consisting of a non-ideal two level subspace, identified as the qubit and a finite set of higher energy levels above this qubit subspace. The whole system is under interaction with an environmental bath through a Caldeira-Leggett type coupling. The model that we use is an rf-SQUID under macroscopic quantum coherence and coupled inductively to a flux noise characterized by an environmental spectrum. The model interaction can generate dipole couplings which can be appreciable for a number of high levels. The decoherence properties of the qubit subspace is examined numerically using the master equation formalism of the system’s reduced density matrix. We numerically examine the relaxation and dephasing times as the environmental frequency spectrum, and the multilevel system parameters are varied at zero temperature. We observe that, these time scales receive contribution from all available energies in the noise spectrum (even well above the system’s energy scales) stressing the dominant role played by the non-resonant (virtual) transitions. The relaxation and dephasing times calculated, strongly depend on the number of levels within the range of levels for which appreciable couplings are produced. Under the influence of these effects, we remark that the validity of the two level approximation is restricted not by the temperature but by these dipole couplings as well as the availability of the environmental modes at low temperatures. © 2005 by World Scientific Publishing Co. Pte. Ltd.
Coherent control of a quantum system is limited both by the decoherence due to environment and the quantum nature of the control agent. The high fidelity of control demanded by fault-tolerant quantum computation and the intrinsic interest in nonclassical effects from the interplay between control and dissipation are motivations for a detailed study of the interaction dynamics between the quantum system and the macroscopic environment and control agent. We present a detailed time-evolution study of a two-level system interacting with a laser pulse and the electromagnetic vacuum in the multimode Jaynes-Cummings model. A diagrammatic formalism allows easy identification of coherent dynamics and relaxation of the two-level system. We demonstrate a computational method of dynamics with precise error bounds for fast operations versus slow decoherence, spanning the Markovian and non-Markovian regimes. Comparison against an exact model solution of our results with existing approximations of the master equation shows the lack of accuracy in the latter.