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arXiv:quant-ph/0703173 · Physical Review Letters

Ultraslow Propagation of Matched Pulses by Four-Wave Mixing in an Atomic Vapor

Vincent Boyer, Colin F. McCormick, E. Arimondo, Paul D. Lett

Published Oct 4, 2007• 138 citations
arXivHTMLPDF

Abstract

We have observed the ultraslow propagation of matched pulses in nondegenerate four-wave mixing in a hot atomic vapor. Probe pulses as short as 70 ns can be delayed by a tunable time of up to 40 ns with little broadening or distortion. During the propagation, a probe pulse is amplified and generates a conjugate pulse which is faster and separates from the probe pulse before getting locked to it at a fixed delay. The precise timing of this process allows us to determine the key coefficients of the susceptibility tensor. The fact that the same configuration has been shown to generate quantum correlations makes this system very promising in the context of quantum information processing.

DOI
10.1103/physrevlett.99.143601

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We have observed the ultraslow propagation of matched pulses in nondegenerate four-wave mixing in a hot atomic vapor. Probe pulses as short as 70 ns can be delayed by a tunable time of up to 40 ns with little broadening or distortion. During the propagation, a probe pulse is amplified and generates a conjugate pulse which is faster and separates from the probe pulse before getting locked to it at a fixed delay. The precise timing of this process allows us to determine the key coefficients of the susceptibility tensor. The fact that the same configuration has been shown to generate quantum correlations makes this system very promising in the context of quantum information processing.
We present an experimental study on ultraslow propagation of matched optical pulses in nondegenerate four wave mixing (FWM) in hot potassium vapor. The main figures of merit, i.e. fractional delay and fractional broadening, are determined to be 1.1 and 1.2, respectively. The latter two are approximately constant for the broad range of the two photon detuning. Input probe pulses between 20 ns and 120 ns can be delayed within broad range of the gain. The results are compared with the preceding works for Rb and Na.
We have investigated experimentally and theoretically four-wave mixing (FWM) in hot potassium vapor as a medium for producing slow and store light. Two pump and a single probe photon were mixed in double-Λ system, characterized by parametric amplification of coupled co-propagating probe and conjugate beams. We have observed very high gains of probe and conjugate, up to 60 and 80 respectively, at two photon Raman resonance, under large one photon detuning, and high K-cell temperature. Using an amplifying medium to alleviate the absorption and distortion of propagating pulses are important for slow-light propagation. We observed ultraslow propagation of probe and conjugate pulses under conditions when parametric amplification of twin beams is well below their maximum values. A fractional delays of close to 5 at a gain ∼1.5, for the probe pulse of 20 ns, have been achieved simultaneously for both probe and accompanying conjugate pulse. FWM mixing process under conditions of the experiment results in broadening of twin beams, close to observed delays.
We experimentally and theoretically study propagation of 80-ns Gaussian-like probe pulses in hot potassium vapor under conditions of four-wave mixing (FWM). The atomic scheme for FWM is off-resonant, double-$\mathrm{\ensuremath{\Lambda}}$ atomic scheme, with pump and probe photons, mediated in the K vapor, generating new probe and conjugate photons. We define the subset of FWM parameters, one-photon pump detuning, two-photon pump-probe Raman detuning, vapor density, the pump Rabi frequencies, when slowed pulses exit the vapor are also Gaussian-like. When Gaussian-like pulses exit the cell we are able to compare theoretical and experimental results for fractional delays and broadening for the probe and conjugate. We have obtained fractional delays above 1. Results of the model are compared with the experiment, with and without the model of Doppler averaging, when the atom velocity distribution is divided into different number of groups. We analyze possible causes for pulse broadening and distortion of slowed probe pulses and show that they are the result of quite different behavior of the probe pulse in the FWM vapor. Besides presenting the first results of slowing 80-ns probe pulses, this work is a useful test of the numerical model and values of parameters taken in the model that are not known in experiments.