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arXiv:quant-ph/0702232 · Physical Review A

Stimulated-Raman-adiabatic-passage–like transitions in a harmonically modulated optical lattice

Benjamin P. Holder, L. E. Reichl

Published Jul 26, 2007• 14 citations
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Abstract

We introduce a method for the coherent acceleration of atoms trapped in an optical lattice, using the well-known model for stimulated Raman adiabatic passage (STIRAP). Specifically, we show that small harmonic modulations of the optical lattice amplitude, with frequencies tuned to the eigenvalue spacings of three ``unperturbed'' eigenstates, reveals a three-state STIRAP subsystem. We use this model to realize an experimentally achievable method for transferring trapped atoms from stationary to motional eigenstates.

DOI
10.1103/physreva.76.013420

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We introduce a method for the coherent acceleration of atoms trapped in an optical lattice, using the well-known model for stimulated Raman adiabatic passage (STIRAP). Specifically, we show that small harmonic modulations of the optical lattice amplitude, with frequencies tuned to the eigenvalue spacings of three ``unperturbed'' eigenstates, reveals a three-state STIRAP subsystem. We use this model to realize an experimentally achievable method for transferring trapped atoms from stationary to motional eigenstates.
We describe a technique for transferring a two-level atom between two adjacent potential wells of an optical lattice, using pairs of pump and Stokes pulses, each resonantly coupling the same pair of internal atomic states to form a Raman transition. Starting from a vibrational eigenstate of one well the atom slowly moves under the action of the pulse pair, to the vibrational eigenstate with the same quantum number in the neighboring well. The transfer takes place in two stages: A conventional stimulated Raman adiabatic passage (STIRAP) technique, in which Stokes precedes pump pulse, is followed by a pulse sequence where pump precedes Stokes and with an inverted sign of the Stokes envelope. In the first step the atom is accelerated toward the adjacent well and in the second step decelerated to the initial vibrational energy. The STIRAP technique avoids the introduction of stochastic motion caused by spontaneous emission from the excited internal atomic state.
Ongoing work aimed at developing highly efficient methods of populating a chosen sublevel of an energy level highlights the need to understand off-resonant effects in coherent excitation. This motivated us to re-examine some aspects of the theory of coherent excitation in a three-state system with a view to obtaining algebraic expressions for off-resonant eigenvalues and eigenvectors. Earlier work gives simple closed-form expressions for the eigenvalues this system, expressions applying even when the system is not on two-photon resonance. We present here expressions of similar simplicity for the components of the normalised eigenvectors. The analytic properties of these components explain the observed sensitivity of the stimulated-Raman-adiabatic-passage process (STIRAP) to the condition of two-photon resonance. None of the eigenstates is ‘trapped’ or ‘dark’ unless the system is on two-photon resonance; off resonance, all states have nonzero projections on the unperturbed intermediate state. A simple argument shows that no dressed state can be adiabatically connected to both the unperturbed initial and final states when the system is off two-photon resonance. That is, adiabatic transfer from initial to final state requires that these be degenerate before and after the STIRAP pulse sequence, and this implies zero two-photon detuning. However, substantial transfer probabilities are observed experimentally for very small two-photon detunings. We show that such systems are characterised by very sharp avoided crossings of two eigenvalues, and that the observed population transfer can be understood as an effect of non adiabatic transitions occurring at the avoided crossings.
Coherent manipulation of quantum states is of crucial importance in accurate control of a quantum system. A fundamental goal is coherently transferring the population of a desired state with near-unit fidelity. For this purpose, we theoretically demonstrate a novel coherent double-stimulated Raman adiabatic passage (STIRAP) in a three-level Λ-type system for realizing the switch of unequal initial preparations on two ground states. This operation uses a single optical pulse sequence accomplishing both bright-STIRAP and dark-STIRAP processes, in which the intermediate-level detuning and the pulse delay must be given an optimal adjustment. Besides, owing to the imperfection of double-STIRAP transition, the sensitivity of the switch fidelity with respect to the spontaneous loss from the intermediate state, to the pulse amplitude and to the population difference, is also discussed. This work suggests a simple and experimentally feasible all-optical approach to switch a superposition quantum state, serving as one-step closer to the goal of coherent manipulation of quantum systems.
A theoretical analysis is presented of the effect of correlation between fluctuations of laser pulse amplitudes on population transfer between the states of a three-level atom coupled by the laser field. The carrier frequencies of the pulses are tuned to resonance with the transitions between the ground and excited states, |〈 and | 2〈, and the excited and metastable states, |2〈 and |3〈, in a lambda-type configuration. The laser pulses are timed so that population transfer between states |1〈 and | 3〈 is made possible by stimulated Raman adiabatic passage (STIRAP) in the absence of fluctuations. STIRAP does not occur when the laser fields are not correlated. When the fluctuations of one pulse amplitude duplicate those of the other, STIRAP can be observed for pulse amplitudes larger than those required in the absence of fluctuations.