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arXiv:quant-ph/0608065 · Physical Review B

Spin qubits in double quantum dots: Entanglement versus the Kondo effect

A. Ramšak, Jernej Mravlje, Rok Žitko, J. Bonča

Published Dec 21, 2006• 33 citations
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Abstract

We investigate the competition between pair entanglement of two spin qubits in double quantum dots attached to leads with various topologies and the separate entanglement of each spin with nearby electrodes. Universal behavior of entanglement is demonstrated in dependence on the mutual interactions between the spin qubits, the coupling to their environment, temperature, and magnetic field. As a consequence of quantum phase transition an abrupt switch between fully entangled and unentangled states takes place when the dots are coupled in parallel.

DOI
10.1103/physrevb.74.241305

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We investigate the competition between pair entanglement of two spin qubits in double quantum dots attached to leads with various topologies and the separate entanglement of each spin with nearby electrodes. Universal behavior of entanglement is demonstrated in dependence on the mutual interactions between the spin qubits, the coupling to their environment, temperature, and magnetic field. As a consequence of quantum phase transition an abrupt switch between fully entangled and unentangled states takes place when the dots are coupled in parallel.
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Semiconductor double‐quantum dots represent an ideal system for studying the novel spin physics of localized spins. On each quantum dot when the number of electrons is odd and the net spin is 1/2, a strong coupling of this localized spin to conducting electrons in the leads gives rise to Kondo correlation. On the other hand, in the coupled double‐quantum‐dot if the inter‐dot antiferromagnetic interaction is strong, the two spins can form a correlated spin‐singlet state, quenching the Kondo effect. This competition between Kondo and antiferromagnetic correlation is studied in a controlled manner by tuning the inter‐dot tunnel coupling. Increasing the inter‐dot tunneling, we observe a continuous transition from a single‐peaked to a double‐peaked Kondo resonance in the differential conductance. On the double‐peaked side, the differential conductance becomes suppressed at zero source‐drain bias. The observed strong suppression of the differential conductance at zero bias provides direct evidence signaling the formation of an entangled spin‐singlet state. This evidence for entanglement and the tunability of our devices bode well for quantum computation applications.
We study the interplay between Kondo correlations and the singlet-triplet exchange splitting K between the two spins in a double quantum dot. We calculate the cotunneling current with elastic and inelastic contributions and its renormalization due to Kondo correlations, away and at the degeneracy point K = 0. We show that these Kondo correlations induce pronounced peaks in the conductance G as a function of magnetic field B , inter-dot coupling t H , and temperature. The long-range part of the Coulomb interaction becomes visible due to Kondo correlations resulting in an additional peak in G vs. t H with a strong B -field dependence. These conductance peaks thus provide direct experimental access to K , and thus to a crucial control parameter for spin-based qubits and entanglement.
Strong electron and spin correlations in a double quantum dot (DQD) can give rise to different quantum states. We observe a continuous transition from a Kondo state exhibiting a single-peak Kondo resonance to another exhibiting a double peak by increasing the interdot coupling (t) in a parallel-coupled DQD. The transition into the double-peak state provides evidence for spin entanglement between the excess electrons on each dot. Toward the transition, the peak splitting merges and becomes substantially smaller than t because of strong Coulomb effects. Our device tunability bodes well for future quantum computation applications.
By means of the numerical renormalization group method, I study the Kondo effect and quantum phase transitions in a double quantum dot system with on-site repulsion UUU, interdot repulsion V,V,V, and magnetic field BBB. At zero temperature and B=0B=0B=0, there is a local spin triplet-singlet transition of the Kosterlitz-Thouless type when VVV increases to a critical value ${V}_{c}\ensuremath{\approx}U$. With increasing BBB, a singlet-triplet transition of the second order occurs at a critical magnetic field ${B}_{c}\ensuremath{\approx}V\ensuremath{-}U$. The magnetic susceptibility and the first derivatives of the spin correlation and double occupation are expected to diverge at Bc{B}_{c}Bc​ and to have different critical exponents, which are universal for different parameters. An appropriate magnetic field can restore the Kondo effect.
We consider a triple quantum dot system in a triangular geometry with one of the dots connected to metallic leads. Using Wilson’s numerical renormalization group method, we investigate quantum entanglement and its relation to the thermodynamic and transport properties in the regime where each of the dots is singly occupied on average, but with non-negligible charge fluctuations. It is shown that even in the regime of significant charge fluctuations the formation of the Kondo singlets induces switching between separable and perfectly entangled states. The quantum phase transition between unentangled and entangled states is analyzed quantitatively and the corresponding phase diagram is explained by exactly solvable spin model. In the framework of an effective model we also explain smearing of the entanglement transition for cases when the symmetry of the triple quantum dot system is relaxed.