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arXiv:quant-ph/0507245 · Physical Review A

Quantum correlations of an atomic ensemble via an incoherent bath

Mihai Macovei, Jörg Evers, Christoph H. Keitel

Published Dec 19, 2005• 26 citations
arXivHTMLPDF

Abstract

A rich variety of quantum features can be found in a collection of atoms driven only by an incoherent bath. To demonstrate this, we discuss a sample of three-level atoms in ladder configuration interacting via the surrounding bath, and show that the fluorescence light emitted by this system exhibits nonclassical properties. Realizations could be thermal baths for microwave transitions, or incoherent broadband fields for optical transitions. In a small sample of atoms, the emitted light can be switched from sub- to super-Poissonian and from antibunching to superbunching controlled by the mean number of atoms in the sample. Larger samples allow us to generate superbunched light over a wide range of bath parameters and thus fluorescence light intensities. We also identify parameter ranges where the fields emitted on the two transitions are strongly correlated or anticorrelated, such that the Cauchy-Schwarz inequality is violated. As in a moderately strong bath this violation occurs also for larger numbers of atoms, such samples exhibit macroscopic quantum effects.

DOI
10.1103/physreva.72.063809

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A rich variety of quantum features can be found in a collection of atoms driven only by an incoherent bath. To demonstrate this, we discuss a sample of three-level atoms in ladder configuration interacting via the surrounding bath, and show that the fluorescence light emitted by this system exhibits nonclassical properties. Realizations could be thermal baths for microwave transitions, or incoherent broadband fields for optical transitions. In a small sample of atoms, the emitted light can be switched from sub- to super-Poissonian and from antibunching to superbunching controlled by the mean number of atoms in the sample. Larger samples allow us to generate superbunched light over a wide range of bath parameters and thus fluorescence light intensities. We also identify parameter ranges where the fields emitted on the two transitions are strongly correlated or anticorrelated, such that the Cauchy-Schwarz inequality is violated. As in a moderately strong bath this violation occurs also for larger numbers of atoms, such samples exhibit macroscopic quantum effects.
Correlations between the emission of photons from an excited three-level atom with one transition more strongly driven than the other are studied. Antibunching, anticorrelation, and superbunching are exhibited in the four possible configurations: ``vee'' (V), ``lambda'' (\ensuremath{\Lambda}), and two cascades with the upper or lower transition strongly driven. We pay particular attention to the projection of the atom into particular states by the measurement of fluorescence, and its significance for detecting quantum jumps in the weak transition by observing the fluorescence from the strong transition. For incoherent excitation we find that cross antibunching (the anticorrelation between emissions of different types of photons) manifests itself as prolonged periods of darkness. For the V and the cascade configuration with a strongly driven lower transition, these periods herald the emission of a weak-transition photon; for the other cascade and the \ensuremath{\Lambda} configuration the periods are heralded by the emission of a weak-transition photon. For on-resonance coherent excitation, dark periods are extremely infrequent for the former two configurations, and are extremely long or infinite for the latter two.
The collective interaction of a multiparticle three-level near-equispaced ladder system with an external applied coherent field, damped via the surrounding electromagnetic field modes, is investigated. The absorption-emission properties of such a medium are shown to be adjustable via external parameters. It is demonstrated that under special conditions the collective resonance fluorescence spectral lines are narrower than the natural bandwidths. Ultranarrow spectral lines are obtained if the laser-atom interaction is mediated by an electromagnetic bath that possesses nonclassical features. Moreover, in these processes an intense flux (intensity proportional to N2{N}^{2}N2) of superbunched photons with subnatural spectral widths can be generated. Artificial atoms (i.e., quantum wells or quantum dots) are suggested as an appropriate system.
The second-order correlation function for light emitted from a strongly and near-resonantly driven dilute cloud of atoms is discussed. Because of the strong driving, the fluorescence spectrum separates into distinct peaks, for which the spectral properties can be defined individually. It is shown that the second-order correlations for various combinations of photons from different spectral lines exhibit bunching together with super-Poissonian or sub-Poissonian photon statistics, tunable by the choice of the detector positions. Additionally, a Cauchy-Schwarz inequality is violated for photons emitted from particular spectral bands. The emitted light intensity is proportional to the square of the number of particles, and thus can potentially be intense. Three different averaging procedures to model ensemble disorder are compared.
The statistical properties of fluorescent light from a single two-level atom driven by nonclassical light beams that exhibit antibunching and squeezing are discussed in the weak-field limit. The fields produced in intracavity second-harmonic generation and those produced by superposing the light from a degenerate parametric oscillator with a coherent field are considered to be the models of nonclassical light beams. These fields can be described in terms of real Gaussian random processes with nonzero mean coherent components. Analytical expressions for the fluorescent light intensity, the second-order intensity correlation function, and the variance of the photon number in the steady state are obtained. The effects of driving-field correlations, detuning, and other parameters characterizing the atom-field interaction on the statistics of scattered light are investigated. It is found that for a certain range of parameters the second-order intensity correlation function may vanish at nonzero times. Under certain other circumstances the antibunching of the fluorescent photons is enhanced. These and other interesting features that appear in the scattered light are discussed.
We investigate the photon statistics of an ensemble of coherently driven non-interacting two-level atoms in the weak driving regime. As it turns out, the system displays unique emission characteristics that are strongly in contrast to the emission of classical oscillating dipoles. By deriving the second-order autocorrelation function, we show that extraordinary two-photon correlations are obtained, ranging from strong antibunching to superbunching. These features are enhanced by disorder in the emitter positions, and the control parameter is the number of excitations in the system. We observe the appearance of bunching and antibunching when the light is scattered by the atoms predominantly coherently, i.e., mimicking classical Rayleigh scattering, whereas thermal photon statistics is obtained when the light is scattered via spontaneous decay, a well-known quantum effect. The underlying mechanism is the interplay between coherent scattering, which exhibits spatial fluctuations due to interference, and dissipation in the form of isotropic spontaneous decay.
We report the experimental verification of nonclassical correlations for an unfiltered spontaneous four-wave mixing process in an ensemble of cold two-level atoms, confirming theoretical predictions by Du et al. in 2007 for the violation of a Cauchy-Schwarz inequality in the system, and obtaining R=(1.98±0.03)≰1. Quantum correlations are observed in a nanoseconds timescale in the interference between the central exciting frequency and sidebands dislocated by the detuning to the atomic resonance. They prevail over the noise background coming from Rayleigh scattering from the same optical transition. These correlations are fragile with respect to processes that disturb the phase of the atomic excitation, but are robust to variations in number of atoms and to increasing light intensities.