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arXiv:quant-ph/0506117 · Bulletin of the American Physical Society

Cavity quantum electrodynamics with surface plasmons

Darrick E. Chang, Anders Søndberg Sørensen, Philip Hemmer, Mikhail D. Lukin

Published May 20, 2005• 0 citations
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Abstract

We describe a technique that enables strong, coherent coupling between individual optical emitters and electromagnetic excitations in conducting nanowires. The excitations in the wire are optical plasmons that are localized to sub-wavelength dimensions, and under realistic conditions optical emission can be almost entirely directed into the propagating plasmon modes via a mechanism analogous to cavity quantum electrodynamics. We describe an application of this technique involving efficient generation of single photons on demand, in which the plasmon on the nanowire is efficiently out-coupled to a dielectric waveguide. Finally, realistic sources of imperfections are analyzed.

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We describe a technique that enables strong, coherent coupling between individual optical emitters and electromagnetic excitations in conducting nanowires. The excitations in the wire are optical plasmons that are localized to sub-wavelength dimensions, and under realistic conditions optical emission can be almost entirely directed into the propagating plasmon modes via a mechanism analogous to cavity quantum electrodynamics. We describe an application of this technique involving efficient generation of single photons on demand, in which the plasmon on the nanowire is efficiently out-coupled to a dielectric waveguide. Finally, realistic sources of imperfections are analyzed.
We introduce a unified theoretical framework for single-plasmon transport in one-dimensional nanowires, bridging the quantized electromagnetic Green's tensor formalism with effective non-Hermitian Hamiltonian models. This approach naturally incorporates propagating surface plasmon polaritons, high-order modes dissipative channels, and intrinsic losses. We investigate both the stationary regime and the spatio-temporal dynamics of a single-plasmon pulse travelling through an atomic chain coupled to a dispersive nanowire. We analyze modal contributions to reflection and transmission spectra for quantum emitter coupled to a silver nanowire, a configuration proposed as a single-plasmon transistor, and we demonstrate that optimized multi-emitter systems offer significant advantages. In case of one quantum emitter coupled to a silver nanowire at telecom wavelengths, we predict a single-plasmon transmittivity down to 7\% under realistic conditions, and an atomic qubit population of 12\%. Extension to multi-emitter systems using a Löwdin orthogonalization procedure enables a consistent treatment of collective interactions. We show that optimized positioning with just five emitters enhances plasmon modulation, achieving a transmittivity of 2\% but also reduces coupling losses to one-third compared to the single-emitter case. Our results establish a robust foundation for analyzing and designing plasmonic waveguide quantum electrodynamics systems.
Abstract Quantum nanophotonics places nanoscale structuring in direct dialogue with photonic quantum information—compressing functionality to the few-nanometre, few-femtosecond frontier while retaining energy efficiency, speed and room-temperature operation. We highlight nanoplasmonic cavity-QED architectures in which extreme mode confinement delivers strong coupling under ambient conditions, enabling ultrafast single-photon emission and near-field multipartite entanglement using industry-grade near-field transducers that nanofocus guided light at practical efficiencies. We set these advances against the arc from early plasmonic cQED proposals and single-emitter Purcell studies to modern time-domain measurements that resolve sub-picosecond polariton/Rabi dynamics—establishing a clear route from concept to device. In parallel, we point to low-loss, high-index Mie resonators whose spectrally sharp electric and magnetic modes afford narrow-band coherent control, filtering and radiation-pattern engineering, and which naturally co-integrate in hybrid metal–dielectric stacks that combine ultrastrong local coupling with low-loss routing and storage. Finally, we discuss quantum nanoplasmonic coherent perfect absorption (qnCPA)—a waveguide-fed, non-perturbing protocol that selectively prepares and protects plasmon–emitter dressed states via dissipation-assisted, unidirectional feeding. Together with macroscopic QED and quantum quasinormal-mode quantization, which regularize open, lossy resonators and clarify when loss can be a resource, these developments chart robust, chip-scale routes to room-temperature quantum technologies.
A bright source of on-demand entangled photons is needed for quantum networks. A single quantum dot in a site-selected nanowire waveguide is a promising candidate for realizing such sources. However, such sources are associated with poor single-photon indistinguishability, limiting their applicability in quantum networks. A common approach for enhancing the single-photon indistinguishability in quantum dot-based entangled photon sources is to implement a broadband optical cavity. Achieving a high-Purcell cavity while retaining the advantages of the nanowire, such as directional emission, a broad operational bandwidth, and high light extraction efficiency, has been a significant challenge. Here, we propose a nanowire cavity based on quasi-bound states in the continuum formed by the strong coupling of two resonant optical modes. We numerically predict this design to support a cavity mode with 4 nm bandwidth and a Purcell enhancement of $\sim$17. This cavity mode enables a directional far-field emission profile (88% overlap with a Gaussian) with a light extraction efficiency of $\sim$74%. Our solution opens up a route for generating entangled photon pairs with enhanced extraction efficiency and single-photon indistinguishability for the practical realization of quantum networks.
Surface plasmon polaritons are charge density waves of electrons in a metal, which are coupled to an electromagnetic field at a metal-dielectric interface. The electro- magnetic field associated with surface plasmons is confined, resulting in increased field intensities near the interface. Optical emitters placed near a metal film interact strongly with the surface plasmon modes present, not only modifying the radiation rates, but also the radiation profile. These emitters may be used to store and process information, and understanding their behaviour in the presence of a lossy metal film is important in determining the advantages and limitations of using surface plasmons. In this thesis, we wish to understand how we can optically control atoms by exploring two physical phenomena: first, the influence of surface plasmons on collective effects in an ensemble of emitters. Secondly, the single photon excitation of an emitter near a metal film. In the first case, we analyze the collective radiative behaviour of multiple classical emitters near a metal film that radiatively couple to the far-field through surface plasmon modes. We demonstrate that the contributions of dipolar image charges within the metal film significantly affect the cooperative emission of nearby sources, generating sub- and super-radiant emission that can be controlled with a suitably detuned external driving field. In the second case, we determine the excitation probability of an atom near a metal film by a single photon pulse that is time reversed. Using a quantum electro- dynamic description of absorbing dielectrics, we show that non-radiative decay will limit the excitation probability to about half of the maximum that could be achieved in the absence of losses.