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arXiv:quant-ph/0504062 · Physical Review A

Pure-state single-photon wave-packet generation by parametric down-conversion in a distributed microcavity

Michael G. Raymer, Jaewoo Noh, Konrad Banaszek, Ian A. Walmsley

Published Aug 29, 2005• 68 citations
arXivHTMLPDF

Abstract

We propose an optical parametric down-conversion (PDC) scheme that does not suffer a trade-off between the state purity of single-photon wave packets and the rate of packet production. This is accomplished by modifying the PDC process by using a microcavity to engineer the density of states of the optical field at the PDC frequencies. The high-finesse cavity mode occupies a spectral interval much narrower than the bandwidth of the pulsed pump laser field, suppressing the spectral correlation, or entanglement, between signal and idler photons. Spectral filtering of the field occurs prior to photon creation rather than afterward as in most other schemes. Operator-Maxwell equations are solved to find the Schmidt-mode decomposition of the two-photon states produced. Greater than 99% pure-state packet production is predicted to be achievable.

DOI
10.1103/physreva.72.023825

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We propose an optical parametric down-conversion (PDC) scheme that does not suffer a trade-off between the state purity of single-photon wave packets and the rate of packet production. This is accomplished by modifying the PDC process by using a microcavity to engineer the density of states of the optical field at the PDC frequencies. The high-finesse cavity mode occupies a spectral interval much narrower than the bandwidth of the pulsed pump laser field, suppressing the spectral correlation, or entanglement, between signal and idler photons. Spectral filtering of the field occurs prior to photon creation rather than afterward as in most other schemes. Operator-Maxwell equations are solved to find the Schmidt-mode decomposition of the two-photon states produced. Greater than 99% pure-state packet production is predicted to be achievable.
This paper presents an experiment on single-photon spectrum generation using an optical parametric oscillator device with cavity-enhanced parametric down-conversion. A PPKTP crystal inside a cavity far below threshold is pumped in order to create signal-idler photon pairs. Triple-resonance of pump, signal, and idler fields are achieved using a compensating KTP crystal. Long-term stability, ultra-high brightness (14000 biphotons/s per mW), and MHz signal bandwidth behind a single-mode fiber on the cesium D1 line (894.3 nm) are attained by locking the cavity length of the pump via the Hansch-Couillaud method. The spectral width of the parametric fluorescence is also derived using the signal-to-idler cross-correlation measurements, and has been found to be < 3 MHz.
Pair creation by spontaneous parametric down-conversion (SPDC) has become a reliable source for single-photon states, used in many kinds of quantum information experiments and applications. In order to be spectrally pure, the two photons within a generated pair should be as frequency-uncorrelated as possible. For this purpose most experiments use narrow bandpass filters, having to put up with a drastic decrease in count rates. This article elaborates (theoretically and by numerical evaluation) the alternative method to engineer a setup such that the SPDC-generated quantum states are intrinsically pure. Using pulsed pump lasers and periodically poled crystals this approach makes bandpass filtering obsolete and allows for significantly higher output intensities and therefore count rates in the detectors. After numerically scanning all common wavelength regimes, polarisation configurations and three different non-linear crystals, we present a broad variety of setups which allow for an implementation of this method.
Parametric down-conversion (PDC) forms one of the basic building blocks for quantum optical experiments. However, the intrinsic multimode spectral-temporal structure of pulsed PDC often poses a severe hindrance for the direct implementation of the heralding of pure single photon states or, for example, continuous-variable entanglement distillation experiments. To get rid of multimode effects narrowband frequency filtering is frequently applied to achieve a single-mode behaviour. To date, the theoretical models of filtered PDC, however, only account for filtering in the low gain regime, where only a few photon-pairs are emitted at any single point in time. In this paper we extend these theoretical descriptions and present a rigorous theoretical model for filtered type-II PDC. Our theoretical investigations reveal that filtering a multimode type-II PDC state, followed by a careful optimization of the measurement basis, effectively achieves a single-mode behaviour and further enables the generation of single-mode EPR-entanglement. Considering the ever increasing brightness of PDC sources our developed theoretical framework, enables the accurate description of filtered PDC in quantum optical experiments.
We explore a promising method of generating pure heralded single photons. Our approach is based on parametric down-conversion in a periodically-poled waveguide. However, unlike conventional downconversion sources, the photon pairs are counter-propagating: one travels with the pump beam in the forward direction while the other is backpropagating towards the laser source. Our calculations reveal that these downconverted two-photon states carry minimal spectral correlations within each photon-pair. This approach offers the possibility to employ a new range of downconversion processes and materials like PPLN (previously considered unsuitable due to its unfavorable phasematching properties) to produce heralded pure single photons over a broad frequency range.
We study theoretically the joint spectral properties of photon-pairs produced through spontaneous four-wave mixing (SFWM) with two spectrally distinct pump pulses in optical fibers. We show that, due to the group velocity difference between the pulses, the signature of the interaction can be significantly different from spontaneous parametric down-conversion or SFWM with a single pump pulse. Specifically, we study the case where temporal walk-off between the pumps enables a gradual turn-on and turn-off of the interaction. By utilizing this property, we develop a new approach towards tailoring the spectral correlations within the generated photon pairs, demonstrating the ability to produce factorable photon-pair states, and hence heralded single photons in a pure wave-packet. We show that the use of two pumps is advantageous over single-pump SFWM approaches towards this goal: the usage of the dual-pump configuration enables, in principle, the creation of completely factorable states without any spectral filtering, even in media for which single-pump SFWM tailoring techniques are unsatisfactory, such as standard polarization-maintaining fiber.