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arXiv:quant-ph/0501118 · Laser Physics

Radiative Corrections to Multi-Level Mollow-Type Spectra

Ulrich D. Jentschura, Evers, Joerg, Christoph H. Keitel

Published Jan 21, 2005• 4 citations
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Abstract

This paper is concerned with two rather basic phenomena: the incoherent fluorescence spectrum of an atom driven by an intense laser field and the coupling of the atom to the (empty) modes of the radiation field. The sum of the many-photon processes gives rise to the inelastic part of the atomic fluorescence, which, for a two-level system, has a well-known characteristic three-peak structure known as the Mollow spectrum. From a theoretical point of view, the Mollow spectrum finds a natural interpretation in terms of transitions among laser-dressed states which are the energy eigenstates of a second-quantized two-level system strongly coupled to a driving laser field. As recently shown, the quasi-energies of the laser-dressed states receive radiative corrections which are nontrivially different from the results which one would expect from an investigation of the coupling of the bare states to the vacuum modes. In this article, we briefly review the basic elements required for the analysis of the dynamic radiative corrections, and we generalize the treatment of the radiative corrections to the incoherent part of the steady-state fluorescence to a three-level system consisting of 1S, 3P and 2S states.

DOI
10.48550/arxiv.quant-ph/0501118

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This paper is concerned with two rather basic phenomena: the incoherent fluorescence spectrum of an atom driven by an intense laser field and the coupling of the atom to the (empty) modes of the radiation field. The sum of the many-photon processes gives rise to the inelastic part of the atomic fluorescence, which, for a two-level system, has a well-known characteristic three-peak structure known as the Mollow spectrum. From a theoretical point of view, the Mollow spectrum finds a natural interpretation in terms of transitions among laser-dressed states which are the energy eigenstates of a second-quantized two-level system strongly coupled to a driving laser field. As recently shown, the quasi-energies of the laser-dressed states receive radiative corrections which are nontrivially different from the results which one would expect from an investigation of the coupling of the bare states to the vacuum modes. In this article, we briefly review the basic elements required for the analysis of the dynamic radiative corrections, and we generalize the treatment of the radiative corrections to the incoherent part of the steady-state fluorescence to a three-level system consisting of 1S, 3P and 2S states.
The incoherent inelastic part of the resonance fluorescence spectrum of a laser-driven atom is known as the Mollow spectrum [B. R. Mollow, Phys. Rev. 188, 1969 (1969)]. Starting from this level of description, we discuss theoretical foundations of high-precision spectroscopy using the resonance fluorescence light of strongly laser-driven atoms. Specifically, we evaluate the leading relativistic and radiative corrections to the Mollow spectrum, up to the relative orders of ${(Z\ensuremath{\alpha})}^{2}$ and $\ensuremath{\alpha}{(Z\ensuremath{\alpha})}^{2}$, respectively, and Bloch-Siegert shifts as well as stimulated radiative corrections involving off-resonant virtual states. Complete results are provided for the hydrogen $1S\text{\ensuremath{-}}2{P}_{1∕2}$ and $1S\text{\ensuremath{-}}2{P}_{3∕2}$ transitions; these include all relevant correction terms up to the specified order of approximation and could directly be compared to experimental data. As an application, the outcome of such experiments would allow for a sensitive test of the validity of the dressed-state basis as the natural description of the combined atom-laser system.
We discuss radiative corrections to an atomic two-level system subject to an intense driving laser field. It is shown that the Lamb shift of the laser-dressed states, which are the natural state basis of the combined atom-laser system, cannot be explained in terms of the Lamb shift received by the atomic bare states which is usually observed in spectroscopic experiments. In the final part, we propose an experimental scheme to measure these corrections based on the incoherent resonance fluorescence spectrum of the driven atom.
We calculate the steady-state spectrum of resonance fluorescence from a two-level atom coupled to a single cavity mode and driven by a strong, in general off-resonance, external field. In the strong-coupling limit, each Mollow triplet component is split into a multiplet, whose detailed structure depends on the atom–cavity coupling, the cavity and spontaneous emission decay constants, and the photon-number distribution of the cavity mode. The dressed states for this system are identified, and the spectral features are interpreted in terms of transitions among these dressed states. In particular, we find that the central component of the central multiplet can have a strongly subnatural linewidth.
We present a perturbative derivation of the fluorescence spectrum for a three-level atom driven by a classical radiation field. The energies of the three atomic levels are equal to \ensuremath{\Elzxh}${\mathrm{\ensuremath{\omega}}}_{\mathrm{i}}$ (i=1, 2, and 3) with ${\mathrm{\ensuremath{\omega}}}_{3}$\ensuremath{\gtrsim}${\mathrm{\ensuremath{\omega}}}_{2}$\ensuremath{\gtrsim}${\mathrm{\ensuremath{\omega}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{32}$\ensuremath{\gg}${\mathrm{\ensuremath{\omega}}}_{21}$ (${\mathrm{\ensuremath{\omega}}}_{\mathit{ij}}$=${\mathrm{\ensuremath{\omega}}}_{\mathit{i}}$-${\mathrm{\ensuremath{\omega}}}_{\mathit{j}}$). The radiation field, having a frequency \ensuremath{\Omega}\ensuremath{\gtrsim}${\mathrm{\ensuremath{\omega}}}_{31}$, can be considered to drive the 2-3 transition only. Spontaneous emission from the ground state, via a normally counter-rotating atom-vacuum interaction term in the Hamiltonian, conserves energy when a photon is subsequently absorbed from the laser field. The spectrum is explained in terms of a Raman process, and in terms of an interaction between the laser field and the coupled atom-vacuum field system. Connection is made with a dressed-atom description of the problem. \textcopyright{} 1996 The American Physical Society.
Summary form only given. The problem of an atom driven by a strong laser was first investigated theoretically in 1969 by B.R. Mollow. He discovered that the resonance fluorescence spectrum has a three-peaked structure with the central peak being more pronounced than the two side peaks. The common Mollow triplet fluorescence pattern can be altered in many ways, by making adjustments to the system. The system can be placed in a squeezed vacuum, the atom can be placed in a cavity, or a bichromatic field can be used instead of a monochromatic laser. These alterations all have an effect on the resulting resonance fluorescence and probe absorption spectra. Other interesting modifications occur when the atom interacts with a stochastic field as well as a laser. The previous approaches were numerical. Here we also obtain analytic solutions (in certain limits) which provide additional insight.
The dressed atom approach provides a tool to investigate the dynamics of an atom-laser system by fully retaining the quantum nature of the coherent mode. In its standard derivation, the internal atom-laser evolution is described within the rotating-wave approximation, which determines a doublet structure of the spectrum and the peculiar fluorescence triplet in the steady state. However, the rotating wave approximation may fail to apply to atomic systems subject to femtosecond light pulses, light-matter systems in the strong-coupling regime or sustaining permanent dipole moments. This work aims to demonstrate how the general features of the steady-state radiative cascade are affected by the interaction of the dressed atom with propagating radiation modes. Rather than focusing on a specific model, we analyze how these features depend on the parameters characterizing the dressed eigenstates in arbitrary atom-laser dynamics, given that a set of general hypotheses is satisfied. Our findings clarify the general conditions in which a description of the radiative cascade in terms of transition between dressed states is self-consistent. We provide a guideline to determine the properties of photon emission for any atom-laser interaction model, which can be particularly relevant when the model should be tailored to enhance a specific line. We apply the general results to the case in which a permanent dipole moment is a source of low-energy emission, whose frequency is of the order of the Rabi coupling.