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arXiv:quant-ph/0408018 · Physical Review A

Decoherence in collective quantum memories for photons

Claudia K. A. Mewes, Michael Fleischhauer

Published Aug 18, 2005• 33 citations
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Abstract

The influence of decoherence on quantum memories for photons based on atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states, corresponding to single photons or nonclassical states of light, the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states, which have the same projection onto the relevant quasiparticle mode (dark-state polariton). Several decoherence processes resulting from uncorrelated individual reservoir couplings are analyzed in detail: single-atom spin flips and dephasing, atom loss, and motion of atoms. Furthermore, it is shown that the sensitivity to collective decoherence processes that affect all polariton modes with comparable strength does also not increase with the number of atoms.

DOI
10.1103/physreva.72.022327

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The influence of decoherence on quantum memories for photons based on atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states, corresponding to single photons or nonclassical states of light, the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states, which have the same projection onto the relevant quasiparticle mode (dark-state polariton). Several decoherence processes resulting from uncorrelated individual reservoir couplings are analyzed in detail: single-atom spin flips and dephasing, atom loss, and motion of atoms. Furthermore, it is shown that the sensitivity to collective decoherence processes that affect all polariton modes with comparable strength does also not increase with the number of atoms.
An ideal and reversible transfer technique for the quantum state between light and metastable collective states of matter is presented and analyzed in detail. The method is based on the control of photon propagation in coherently driven three-level atomic media, in which the group velocity is adiabatically reduced to zero. Form-stable coupled excitations of light and matter (``dark-state polaritons'') associated with the propagation of quantum fields in electromagnetically induced transparency are identified, their basic properties discussed and their application for quantum memories for light analyzed.
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In this thesis, we explore the quantum dynamics of light interactions with optically thick collections of atoms. We provide a theoretical description of several recent experiments in which some key operations necessary for the implementation of quantum communication networks are demonstrated. Collective Raman scattering from an atomic ensemble is shown to produce probabilistic entanglement between the polarization of a scattered photon and an associated collective atomic excitation. The predicted correlations agree with experimental observations. We also propose a method to use cascade transitions to produce entanglement between a photon with a frequency in the telecom range (ideal for transmission over optical fibers) and a near infrared photon (ideal for storage in an atomic ensemble), and a description of the experimental demonstration is provided. We also propose and describe the implementation of a deterministic source of single photons.\n\nIn addition, we generalize the theory of dark-state polaritons in ensembles of three level Lambda atoms to account for the nuclear spin degeneracy of alkali atoms. This generalized theory provides a description of the first demonstration of single photon storage and retrieval from atomic ensembles. Additionally, in the presence of a uniform magnetic field, we predict the occurrence of collapses and revivals of the photon retrieval efficiency as a function of storage time within the ensemble. These predictions are in very good agreement with subsequent experimental observations. We also exploit the ability of photon storage to entangle remote atomic qubits.
Quantum optics provides tools for the accurate control of light using atoms and also for manipulating atomic states using light. These techniques are being used for many applications, including quantum information processing and the generation of exotic quantum states. This thesis contains proposals for implementing a photonic quantum memory and a photon-photon gate, which are essential elements of photonic quantum information processing. Furthermore it proposes a scheme for the creation of many-body entangled states. First a proposal for a new quantum memory protocol, called the atomic frequency sweep quantum memory, is presented. A two-level polariton model is derived that explains the coherent storage and retrieval of light through the manipulation of the atomic resonance frequency. This is followed by a scheme for a deterministic photonic controlled-PHASE gate based on the strong interaction between two stationary collective Rydberg excitations in an atomic ensemble. Distortion effects caused by nonuniform interaction are quantified and compensation techniques for these effects are proposed. Finally a proposal is presented that uses Rydberg dressing for the generation of energy cat states in an atomic medium, i.e. superposition states of all the atoms being in the ground or excited state, where these two states are connected by an optical transition and thus have a significant difference in energy. Considering the fragility of the state, the effects of many different imperfections and decoherence sources are quantified. The resulting cat state would allow testing of energy decoherence models with greatly improved sensitivity.
We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters' inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitter ensembles. When two different ensembles of emitters are coupled to the resonator, they support a peculiar collective dark state, which is also very attractive for the storage of quantum information.