Quantum optics provides tools for the accurate control of light using atoms and also for manipulating atomic states using light. These techniques are being used for many applications, including quantum information processing and the generation of exotic quantum states. This thesis contains proposals for implementing a photonic quantum memory and a photon-photon gate, which are essential elements of photonic quantum information processing. Furthermore it proposes a scheme for the creation of many-body entangled states. First a proposal for a new quantum memory protocol, called the atomic frequency sweep quantum memory, is presented. A two-level polariton model is derived that explains the coherent storage and retrieval of light through the manipulation of the atomic resonance frequency. This is followed by a scheme for a deterministic photonic controlled-PHASE gate based on the strong interaction between two stationary collective Rydberg excitations in an atomic ensemble. Distortion effects caused by nonuniform interaction are quantified and compensation techniques for these effects are proposed. Finally a proposal is presented that uses Rydberg dressing for the generation of energy cat states in an atomic medium, i.e. superposition states of all the atoms being in the ground or excited state, where these two states are connected by an optical transition and thus have a significant difference in energy. Considering the fragility of the state, the effects of many different imperfections and decoherence sources are quantified. The resulting cat state would allow testing of energy decoherence models with greatly improved sensitivity.
Quantum optics provides tools for the accurate control of light using atoms and also for manipulating atomic states using light. These techniques are being used for many applications, including quantum information processing and the generation of exotic quantum states. This thesis contains proposals for implementing a photonic quantum memory and a photon-photon gate, which are essential elements of photonic quantum information processing. Furthermore it proposes a scheme for the creation of many-body entangled states. First a proposal for a new quantum memory protocol, called the atomic frequency sweep quantum memory, is presented. A two-level polariton model is derived that explains the coherent storage and retrieval of light through the manipulation of the atomic resonance frequency. This is followed by a scheme for a deterministic photonic controlled-PHASE gate based on the strong interaction between two stationary collective Rydberg excitations in an atomic ensemble. Distortion effects caused by nonuniform interaction are quantified and compensation techniques for these effects are proposed. Finally a proposal is presented that uses Rydberg dressing for the generation of energy cat states in an atomic medium, i.e. superposition states of all the atoms being in the ground or excited state, where these two states are connected by an optical transition and thus have a significant difference in energy. Considering the fragility of the state, the effects of many different imperfections and decoherence sources are quantified. The resulting cat state would allow testing of energy decoherence models with greatly improved sensitivity.
The advances in laser cooling and trapping techniques allow samples of ultra-cold atoms to be created and controlled for the study of quantum physics. In this thesis, we focus on using ensembles of cold atoms to investigate novel quantum effects and their applications in quantum optics. Realization of a scalable intercontinental quantum system, e.g. a global quantum internet, relies on quantum memories with long lifetimes on the order of seconds. We have reduced the differential light shifts of the atomic ground states to a sub-Hz level and achieved a lifetime of 16 seconds. Achieving fast and efficient quantum operations, on the other hand, requires strongly-interacting systems. We explore highly excited Rydberg atoms towards this goal and demonstrate Rydberg excitation blockade, many-body Rabi oscillations, trapping of Rydberg atoms, deterministic single photon source, and atom-photon entanglement. Finally, we integrate the two essential capabilities for quantum information processing, fast quantum state generation and long-term storage, by simultaneously exploiting Rydberg levels for interactions and ground atomic levels for the storage of quantum state. Our work advances the control of coherence properties and interactions in cold atomic ensembles to a new level and opens new opportunities for studies of complex quantum systems.
The field of quantum computation and communication has prospered over the last few decades because of multiple advances in our understanding of trapping and controlling physical quantum systems like neutral atoms, superconducting qubits, trapped ions, quantum dots etc. using light. A lot of research has gone into development of techniques which facilitate trapping and manipulation of ensembles of neutral atoms by studying how the atomic properties of the system respond to properties of light used to control them. In this dissertation we shall explore some applications of light-matter interactions in ensembles of lambda three level neutral atoms for the purpose of entanglement generation and distribution. The first part of this dissertation focuses on the study of a protocol that can be used to generate multi-particle entangled quantum states called the Greenberger-Horne-Zeilinger (GHZ) states in an ensemble of N neutral atoms. Schemes for creation of N particle entangled Greenberger-Horne-Zeilinger (GHZ) states are important for understanding multi-particle non-classical correlations. A theoretical protocol for creation of a multi-particle GHZ state implemented on a target ensemble of N, three-level Rydberg atoms and a single Rydberg atom as a control using Stimulated Raman Adiabatic Passage (STIRAP) is presented. We work in the Rydberg blockade regime for the ensemble atoms induced due to excitation of the control atom to a high lying Rydberg level. It is shown that using STIRAP, atoms from one ground state of the ensemble can be adiabatically transferred with high fidelity to the other multi-particle ground state, depending on the state of the control atom. Measurement of the control atom in a specific basis after this conditional transfer facilitates one-step creation of a N particle GHZ state. A thorough analysis of adiabatic conditions associated with STIRAP for this scheme and the influence of radiative decay from the excited Rydberg levels is presented. The most important and novel feature of this scheme is that it is immune to the decay rate of the excited level in ensemble atoms and provides a robust way of creating GHZ states. In the second part of this dissertation, we study atomic ensemble based quantum interfaces used in quantum repeater protocols for entanglement distribution. Quantum interfaces provide a platform where in the flying photonic qubits used for information and entanglement transfer can interact with a physical system which stores, processes and releases this information back as photons. The Duan-Lukin-Cirac-Zoller (DLCZ) quantum repeater protocol, which was proposed to realize long distance quantum communication, requires usage of quantum memories or quantum interfaces. Atomic ensembles interacting with optical beams based on off-resonant Raman scattering serve as convenient on-demand quantum memories. Here a complete, free space, three-dimensional theory of the associated read and write process for this quantum memory is worked out with the aim of understanding intrinsic retrieval efficiency. We develop a formalism to calculate the transverse mode structure for the signal and the idler photons and use the formalism to study the intrinsic retrieval efficiency under various configurations. The effects of atomic density fluctuations and atomic motion are incorporated by numerically simulating this system for a range of realistic experimental parameters. Results describe the variation in the intrinsic retrieval efficiency as a function of the memory storage time for skewed beam configuration at a finite temperature, which provides valuable information for optimization of the retrieval efficiency in experiments.
It is known that photons are the ideal carriers of quantum information and ensemble of atoms can be acted as the long lived storage and processing units. In the coherently prepared atomic ensemble with the light resonantly interacting with the atoms, various schemes have been proposed to implement quantum state transfer and storage, quantum phase gate, generation of entangled photons, and the long-distance quantum communication [1]. We first proposed the dark-state polaritons in a five-level M-type atomic ensemble in the electro magnetically induced transparency (EIT) [2], Under conditions of the low excitation limit and adiabatic following, the quantum field can be mapped onto the atomic polarization states, forming the shape preserving quantum states of polaritons. Two channels for robust quantum memory are provided. Then, we investigated the nonlinear optical response of a five-level tripod atomic system in the EIT, and proposed a three-qubit phase gate protocol based on the fifth-order nonlinearity [3]. The cross phase modulation among three weak fields induced by the fifth-order nonlinearity in EIT can produce the phase shift of order n, which can be used to realize the three-qubit polarization phase gate. Finally, we proposed a cavity-QED scheme that can effectively generate EPR polarization-entangled photon pairs [4], A four-level tripod atom successively couples to two high-Q optical cavities possessing polarization degeneracy, assisted by a classical π-polarized pump field. The stimulated Raman adiabatic passage process in the atom-cavity system is used to produce the polarization-entangled photon pairs. The proposal is particularly robust against atomic spontaneous decay. The above protocols should have potential applications in quantum information processing.
In this chapter, we present a proposal for the realization of an entangling gate for photons. The protocol works deterministically and is experimentally feasible under realistic conditions. We start outlining the general problem of quantum information processing with photons and describe the current status in this field. Then we introduce the proposed scheme and present its main features. This part is followed by a review of the concepts and procedures employed in our proposal. Finally, we explain the quantum gate, in detail, in the last section of this chapter, where we also briefly discuss the performance of the gate in the presence of imperfections. 26.1.1 Quantum information processing with light Photons play a key role in applications of quantum information because they are ideally suited to transmit quantum states between distant sites. This feature makes them indispensable for the realization of quantum communication protocols and the construction of quantum networks. While being a good flying carrier of information, photons are naturally less adequate for storage than the long-lived matter degrees of freedom. For this reason, matter systems are employed as quantum memories. In order to combine both elements in a quantum network (i.e., photons as flying qubits and atoms as memory devices), light-matter interface schemes have been developed to transfer quantum states of light onto an atomic system. Some of these schemes are based on quantum-nondemolition interactions, electromagnetically induced transparency, and Raman processes. Moreover, Raman processes have been used to entangle two distant atomic ensembles, which is an important step to realize quantum repeaters and, thus to solve the problem of losses and decoherence that exists in a photonic channel. Apart from the transmission and storage of information, in a quantum network it is necessary to process quantum states. However, manipulation of quantum states of light is still challenging, since it requires the ability to create entanglement between photons. This task is difficult because photons are noninteracting particles, in principle. One possibility to entangle photons is to employ materials that possess optical nonlinearities, but so far, there are no materials available whose nonlinearities are strong enough to allow for short gate times. An alternative approach was put forward by Knill et al., which requires only linear optical operations and measurements. However, this scheme is probabilistic and not very efficient in practice. In this chapter, we present a scheme for the realization of a deterministic entangling gate for photons by using an atom lattice. An atom lattice consists of an ensemble of cold atoms loaded in the periodic optical potential created by a standing wave. In order to use the lattice as a quantum register for quantum computation, it is necessary to prepare it in a Mott insulating phase, in which the number of atoms in each site of the potential (i.e., in each of its minima) is approximately constant, and set equal to 1.
This thesis proposes a means of implementing quantum information processing using photonic qubits as information carriers. Electromagnetically-induced transparency (\textsmaller{EIT}) is used to store information encoded in photons into Rydberg excitations in a cloud of cold atoms, where strong dipole-dipole interactions induce interactions between qubits. After a storage time, information is mapped back into photons collectively emitted from the cloud again via \textsmaller{EIT}. A new experimental apparatus is built to implement non-linear Rydberg quantum optics. A high repetition rate is achieved owing to a \textsmaller{2D-MOT} atom source, and high optical resolution for trapping and probing microscopic atomic ensembles is achieved by the use of aspheric lenses inside the vacuum chamber. A new, high resolution computer control scheme is implemented. This thesis demonstrates that, during the holding time, multiple collective Rydberg excitations at a controlled separation interact with each other to imprint a non-uniform phase gradient resulting in anti-correlation of photon emission. Interactions are observed at up to 15 times the wavelength of the photonic qubits. These long range interactions offer a promising approach to scaling all-optical quantum computing. Applying resonant microwave fields during the storage time is demonstrated to offer a competitive method of performing sensitive microwave electrometry. A sensitivity of $12 \pm 7 \uV \percm \perRHz$ is found at a frequency of $7.7\GHz$. The high sensitivity is shown to arise from remnant, Rydberg excitations providing an additional source of atom loss from the atomic ensemble, leading to a suppression of photon storage and retrieval efficiency. An additional stage of microwave driving to sanitise the atomic ensemble for recycling is shown to successfully suppress the atom-loss mechanism. The use of successive microwave pulses is shown to provide a feasible approach to interfacing microwave and optical quantum information processing systems. Information encoded as the presence or absence of a microwave field is translated into information encoded as early or late retrieval of single photons, demonstrating proof of principle for an approach to implementing a proposal for an all-optical controlled-z gate. Externally driven microwave fields are used to provide rapid, low-loss modulation of the signal retrieved from an atomic ensemble, demonstrating the proof of principle of implementing a probabilistic single photon source that can intensity modulate with low-loss at frequencies of at least $27\MHz$, with evidence that modulation may be achievable at rates in excess of $500\MHz$.
The emergence of quantum physics from the page to the lab and the world at large is an exciting development of recent years. The prospects of absolutely secure communication and efficient simulation of physical systems have spurred great human effort into understanding these possibilities and turning them into realities. Photons are the most easily manipulated quantum particles and are a promising candidate for implementing these technologies. Limitations of photons include the difficulty of keeping objects that move at the speed of light, and producing strong interactions between particles that do not normally interact. The work presented in this thesis is motivated by the possibility of overcoming these limitations. The ability to faithfully store and reproduce a quantum state is essential for many quantum information technologies. Quantum memories for light have been developed over the last two decades to provide this ability. The group at the Australian National University developed the gradient echo memory (GEM): A quantum state of light can be controllably stored and released from an atomic ensemble by the use of additional optical fields and magnetic field gradients. This scheme was previously shown to preserve the quantum characteristics of the light. We used the GEM scheme with a cold rubidium ensemble to create the first optical memory that simultaneously beat the no-cloning limit, a benchmark for many of the technologies relying on quantum memories, and the loss rate for a delay line composed of optical fibre. We also created an analogue to a pulsed optical resonator using GEM with a warm rubidium vapour. This was done by replacing the circulating optical field of a resonator with light stored in the memory, and replacing the coupling of light into and out of that circulating mode with storage and recall from the memory. The bandwidth and repetition rate of this resonator were rapidly tunable as they were controlled by external optical and magnetic fields. We worked on implementing GEM with strings of thousands of atoms strongly coupled to the evanescent field of an optical nanofibre. This raised new possibilities for creating a true random access memory that would allow a more flexible use of the multi-mode capacity of GEM. We developed the theory for a novel type of stationary light in the gradient echo memory. Our stationary light scheme relies on the destructive interference of counter-propagating optical fields throughout the memory. The optical intensity scales with optical depth, as with other forms of stationary light. However, as the destructive interference could be set up over a much greater distance, more of the optical depth is available for generating stationary light. Finally, we studied how a control-phase gate for single-photon optical states could be implemented using a nonlinear interaction with stationary light. The stationary light generated by one state modulates the phase of another state stored in the memory. The second state modifies the stationary light, also producing a back-action on the first state and generating the required cross-phase shift.