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arXiv:quant-ph/0407094 · Optics and Spectroscopy

Collective states in highly symmetric atomic configurations and single-photon traps

Hanno Hammer

Published Aug 1, 2005• 3 citations
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Abstract

We study correlated states in circular and linear-chain configurations of identical two-level atoms containing the energy of a single quasi-resonant photon in the form of a collective excitation, where the collective behavior is mediated by exchange of transverse photons between the atoms. For a circular atomic configuration containing N atoms, the collective energy eigenstates can be determined by group-theoretical means making use of the fact that the configuration possesses a cyclic symmetry group Z N . For these circular configurations, the carrier spaces of the various irreducible representations of the symmetry group are at most two-dimensional, so that the effective Hamiltonian on the radiationless subspace of the system can be diagonalized analytically. As a consequence, the radiationless energy eigenstates carry a Z N quantum number p = 0, 1, …, N, which is analogous to the angular momentum quantum number l = 0, 1, … carried by particles propagating in a central potential, such as a hydrogen-like system. Just as the hydrogen s states are the only electronic wave functions that can occupy the central region of the Coulomb potential, the quasi-particle corresponding to a collective excitation of the circular atomic sample can occupy the central atom only for vanishing Z N quantum number p. When a central atom is present, the p = 0 state splits into two, showing level crossing at certain radii; in the regions between these radii, damped oscillations between two “ extreme” p = 0 states occur, where the excitation occupies either the outer atoms or the central atom only. For large numbers of atoms in a maximally subradiant state, a critical interatomic distance of λ/2 emerges both in the linear-chain and in the circular configuration of atoms. The spontaneous decay rate of the linear configuration exhibits a jumplike “critical” behavior for next-neighbor distances close to a half-wavelength. Furthermore, both the linear-chain and the circular configurations exhibit exponential photon trapping once the next-neighbor distance becomes less than a half-wavelength, with the suppression of spontaneous decay being particularly pronounced in the circular system. In this way, circular configurations containing sufficiently many atoms may be natural candidates for single-photon traps.

DOI
10.1134/1.2034622

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Apr 18, 2008•1 citation
We study correlated states in circular and linear-chain configurations of identical two-level atoms containing the energy of a single quasi-resonant photon in the form of a collective excitation, where the collective behavior is mediated by exchange of transverse photons between the atoms. For a circular atomic configuration containing N atoms, the collective energy eigenstates can be determined by group-theoretical means making use of the fact that the configuration possesses a cyclic symmetry group Z N . For these circular configurations, the carrier spaces of the various irreducible representations of the symmetry group are at most two-dimensional, so that the effective Hamiltonian on the radiationless subspace of the system can be diagonalized analytically. As a consequence, the radiationless energy eigenstates carry a Z N quantum number p = 0, 1, …, N, which is analogous to the angular momentum quantum number l = 0, 1, … carried by particles propagating in a central potential, such as a hydrogen-like system. Just as the hydrogen s states are the only electronic wave functions that can occupy the central region of the Coulomb potential, the quasi-particle corresponding to a collective excitation of the circular atomic sample can occupy the central atom only for vanishing Z N quantum number p. When a central atom is present, the p = 0 state splits into two, showing level crossing at certain radii; in the regions between these radii, damped oscillations between two “ extreme” p = 0 states occur, where the excitation occupies either the outer atoms or the central atom only. For large numbers of atoms in a maximally subradiant state, a critical interatomic distance of λ/2 emerges both in the linear-chain and in the circular configuration of atoms. The spontaneous decay rate of the linear configuration exhibits a jumplike “critical” behavior for next-neighbor distances close to a half-wavelength. Furthermore, both the linear-chain and the circular configurations exhibit exponential photon trapping once the next-neighbor distance becomes less than a half-wavelength, with the suppression of spontaneous decay being particularly pronounced in the circular system. In this way, circular configurations containing sufficiently many atoms may be natural candidates for single-photon traps.
Correlated excitations in a plane circular configuration of identical atoms with parallel dipole moments are investigated. The collective energy eigenstates, which are formally identical to Frenkel excitons, can be computed together with their level shifts and decay rates by decomposing the atomic state space into carrier spaces for the irreducible representations of the symmetry group ZN{\mathbb{Z}}_{N}ZN​ of the circle. It is shown that the index ppp of these representations can be used as a quantum number analogously to the orbital angular momentum quantum number lll in hydrogenlike systems. Just as the hydrogen sss states are the only electronic wave functions which can occupy the central region of the Coulomb potential, the quasiparticle corresponding to a collective excitation of the atoms in the circle can occupy the central atom only for vanishing ZN{\mathbb{Z}}_{N}ZN​ quantum number ppp. If a central atom is present, the p=0p=0p=0 state splits into two and shows level crossing at certain radii; in the regions between these radii, damped quantum beats between two ``extreme'' p=0p=0p=0 configurations occur. The physical mechanisms behind super- and subradiance at a given radius are discussed. It is shown that, beyond a certain critical number of atoms in the circle, the lifetime of the maximally subradiant state increases exponentially with the number of atoms in the configuration, making the system a natural candidate for a single-photon trap.
We investigate collective behaviour that appears in open, many-body systems of two- and four-level atoms. Here, ``open" refers to the system interacting with an external environment that causes dissipation. We derive a general open quantum master equation to describe the system dynamics only, independent of this environment. We identify processes such as coherent exchange of virtual photons and modified decay rates caused by long-range interactions between all pairs of atoms that scale with distance by inverse power laws. We explore excitation transport within a one-dimensional chain of atoms where the atomic transition dipoles are coupled to the free radiation field. When the interatomic spacing is smaller than or comparable to the wavelength of light associated with the photon emitted from a given transition, virtual photon exchange interactions facilitate excitation transport through the chain. Atomic systems coupled to an environment display dissipative dynamics, however subradiant transport is exhibited from a variety of initial states; spontaneous emission from the chain occurs at a rate much slower than that for an individual atom. In particular, we find a region within the decay spectrum that consists entirely of subradiant states with a corresponding linear dispersion relation in the interaction energy. Identifying this subspace allows for the dispersionless transport of wave packets over long distances with near-zero decay. Moreover, the group velocity of the wave packet and direction of the transport can be controlled via an external uniform magnetic field while preserving its subradiant character. We discuss a number of experimental considerations to justify the feasibility and robustness of this protocol. Initial state preparation is outlined, utilising external laser driving to excite the system into the single excitation sector. Furthermore, we consider positional disorder by explicitly accounting for the external atomic degrees of freedom -- position and momentum -- which allows us to model the positions of all atoms by a motional state representing the occupation of a lattice well with a given width. These discussions are made in the low-temperature limit, where the atomic motion is essentially frozen, and we identify that subradiant transport is indeed robust. Finally, we explore the experimental limits of interatomic spacing and imperfect filling within an experimentally achievable optical lattice. We calculate the photon emission rate -- an experimentally measurable quantity -- and compare the emission spectra to our analysis. By limiting parameters to those achieved experimentally, we observe a reduction, yet not an absence, of collective behaviour. The simplicity and versatility of this system, together with the robustness of subradiance against disorder, makes it relevant for a range of applications such as lossless energy transport and long-time light storage. The lifetime of an atomic excitation could be increased by a factor of thousands to millions for a chain of atoms under the conditions that we explore in this thesis.
We consider a pair of identical two-level atoms interacting with a scalar field in one dimension, separated by a distance x21{x}_{21}x21​. We obtain collective decaying states, belonging to a complex spectral representation of the Hamiltonian. The imaginary parts of the eigenvalues give the decay rates, and the real parts give the average energy of the collective states. In one dimension there is strong interference between the fields emitted by the atoms, producing cooperative effects even when the atoms are far apart. The decay rates and the energy oscillate with the distance x21{x}_{21}x21​. Depending on x21{x}_{21}x21​, the decay rates will either decrease, vanish, or increase as compared with the one-atom decay rate. We have sub- and superradiance at periodic intervals. Our model may be used to study two-cavity electron waveguides. The vanishing of the collective decay rates then suggests the possibility of obtaining stable configurations, where an electron is trapped inside the two cavities.
Sub- and superradiant dynamics of spontaneously decaying atoms are manifestations of collective many-body systems. We study the internal dynamics and the radiation properties of two atoms in free space. Interesting results are obtained when the atoms are separated by less than half a wavelength of the atomic transition, where the dipole-dipole interaction gives rise to new coherent effects, such as (a) coherence between two intermediate collective states, (b) oscillations in the two-photon correlation G(2){G}^{(2)}G(2), (c) emission of two photons by one atom, and (d) the loss of directional correlation. We compare the population dynamics during the two-photon emission process with the dynamics of single-photon emission in the cases of a $\ensuremath{\Lambda}$ and a V scheme. We compute the temporal correlation and angular correlation of two successively emitted photons using the G(2){G}^{(2)}G(2) for different values of atomic separation. We find antibunching when the atomic separation is a quarter wavelength $\ensuremath{\lambda}∕4$. Oscillations in the temporal correlation provide a useful feature for measuring subwavelength atomic separation. Strong directional correlation between two emitted photons is found for atomic separation larger than a wavelength. We also compare the directionality of a photon spontaneously emitted by the two atoms prepared in phased-symmetric and phased-antisymmetric entangled states ${\ensuremath{\mid}\ifmmode\pm\else\textpm\fi{}⟩}_{{\mathbf{k}}_{0}}={e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{1}}\ensuremath{\mid}{a}_{1},{b}_{2}⟩\ifmmode\pm\else\textpm\fi{}{e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{2}}\ensuremath{\mid}{b}_{1},{a}_{2}⟩$ by a laser pulse with wave vector k0{\mathbf{k}}_{0}k0​. Photon emission is directionally suppressed along k0{\mathbf{k}}_{0}k0​ for the phased-antisymmetric state. The directionality ceases for interatomic distances less than $\ensuremath{\lambda}∕2$.
The nonperturbative theory of the cooperative spontaneous emission from a two level atom trapped in one-dimentional damped nanocavity with a single resonance mode is presented. The time-dependent spectral properties and nonlinear dynamics of a separate photon emission by the micro-molecular-like system "excited atom coupled to a resonance decaying mode" have been analyzed. The investigation has been carried out by solving the Schrödinger equation in the interaction picture with the help of the Green functions method in the Heitler-Ma's form. The formalism was supplemented with the novel algorithm in operating causal singular functions and with fundamentals of the theory of quasi-stationary systems. The proposed theory accounts automatically of both reabsorptions of emitted photon and its simultaneous escaping out of the cavity. Solutions of the wave equation were found without using intermediate virtual states and series expansions. In accordance with the theory of quasi-stationary systems the field of mode decaying exponentially in the empty nanocavity was represented with the Lorenz-shaped packet of stationary photonic states (quasi-modes). The electro-dipolar interaction between the atom and the mode field was adopted to be switched on suddenly. The expressions and plots of emission probabilities spectral densities together with photon emission probability dynamics as functions of time for various ratios Γ/4g of photon escaping rate Γ and coupling constant g are presented. For Γ/4g <1 the transient emission spectrum reveals the presence of two symmetrical side-bands and of the central peak, the latter decaying in time at the rate ∝ Γ/2 so that the final spectrum is a doublet. In this case the photon emission probability is described by decaying oscillations. On the contrary for Γ/4g ≥ 1 the spectrum is a singlet and the emission occurs in exponentially decaying ways.