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arXiv:quant-ph/0403128 · Physical Review A

Casimir-Polder forces: A nonperturbative approach

Stefan Yoshi Buhmann, L. Knöll, Dirk‐Gunnar Welsch, Ho Trung Dung

Published Nov 29, 2004• 171 citations
arXivHTMLPDF

Abstract

Within the frame of macroscopic QED in linear, causal media, we study the radiation force of Casimir-Polder type acting on an atom which is positioned near dispersing and absorbing magnetodielectric bodies and initially prepared in an arbitrary electronic state. It is shown that minimal and multipolar coupling lead to essentially the same lowest-order perturbative result for the force acting on an atom in an energy eigenstate. To go beyond perturbation theory, the calculations are based on the exact center-of-mass equation of motion. For a nondriven atom in the weak-coupling regime, the force as a function of time is a superposition of force components that are related to the electronic density matrix elements at a chosen time. Even the force component associated with the ground state is not derivable from a potential in the ususal way, because of the position dependence of the atomic polarizability. Further, when the atom is initially prepared in a coherent superposition of energy eigenstates, then temporally oscillating force components are observed, which are due to the interaction of the atom with both electric and magnetic fields.

DOI
10.1103/physreva.70.052117

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Within the frame of macroscopic QED in linear, causal media, we study the radiation force of Casimir-Polder type acting on an atom which is positioned near dispersing and absorbing magnetodielectric bodies and initially prepared in an arbitrary electronic state. It is shown that minimal and multipolar coupling lead to essentially the same lowest-order perturbative result for the force acting on an atom in an energy eigenstate. To go beyond perturbation theory, the calculations are based on the exact center-of-mass equation of motion. For a nondriven atom in the weak-coupling regime, the force as a function of time is a superposition of force components that are related to the electronic density matrix elements at a chosen time. Even the force component associated with the ground state is not derivable from a potential in the ususal way, because of the position dependence of the atomic polarizability. Further, when the atom is initially prepared in a coherent superposition of energy eigenstates, then temporally oscillating force components are observed, which are due to the interaction of the atom with both electric and magnetic fields.
The Casimir-Polder force on a single atom in the presence of microscopic magneto-electric bodies is studied within the framework of macroscopic quantum electrodynamics. In the first part, time-independent perturbation theory is used show that the static Casimir-Polder force on a ground-state atom in the presence of an arbitrary arrangement of bodies can be expressed in terms of the atom's polarisability and the scattering part of the Green tensor characterising the bodies. This result is used to verify the origin of the force and to study various bodies of simple shapes. In the second part, a genuinely dynamical approach is developed by starting from the operator Lorentz force. It is found that the dynamics of the force on initially excited atoms is governed by irreversible spontaneous decay in the case of weak atom-field coupling, while Rabi oscillations may arise for strong atom-field coupling.
The potential of long-range interaction between two dissimilar atoms, one of which is excited, drops as 1/R 2 with the distance for the Casimir-Polder limit of large distances in comparison with the wave-length of atom transitions (E.A. Power and T. Thirunamachandran, Phys. Rev. A 51, 3660 (1995)). It is shown that such a dependence, obtained with the help of perturbation technique, results in a divergence for the interaction potential between an excited atom and a medium of dilute gas. We develop a nonperturbative method based upon quantum Green’s functions (Yu. Sherkunov, Phys. Rev. A 72, 052703 (2005)) to calculate the interaction potential for an excited atom and a ground-state atom embedded in a dielectric medium, taking into account the absorption of photons in the dielectric medium. The exponential suppression of the interaction between the atoms is demonstrated. The force acting on an excited atom near the interface of dilute gas medium is calculated. The result is no more divergent. The force between gas media in Casimir-Polder regime is calculated as well.
The time-dependent Casimir-Polder force arising during the time evolution of an initially bare two-level atom, interacting with the radiation field and placed near a perfectly conducting wall, is considered. Initially the electromagnetic field is supposed to be in the vacuum state and the atom in its ground state. The analytical expression of the force as a function of time and atom-wall distance is evaluated from the time-dependent atom-field interaction energy. Physical features and limits of validity of the results are discussed in detail.
We consider the dynamical atom-surface Casimir-Polder force in the nonequilibrium configuration of an atom near a perfectly conducting wall, initially prepared in an excited state with the field in its vacuum state. We evaluate the time-dependent Casimir-Polder force on the atom and find that it shows an oscillatory behavior from attractive to repulsive both in time and in space. We also investigate the asymptotic behavior in time of the dynamical force and of related local field quantities, showing that the static value of the force, as obtained by a time-independent approach, is recovered for times much longer than the time scale of the atomic self-dressing but shorter than the atomic decay time. We then discuss the evolution of global quantities such as atomic and field energies and their asymptotic behavior. We also compare our results for the dynamical force on the excited atom with analogous results recently obtained for an initially bare ground-state atom. We show that new relevant features are obtained in the case of an initially excited atom, for example, much larger values of the dynamical force with respect to the static one, allowing for an easier way to single out and observe the dynamical Casimir-Polder effect.
We study the influence of thermal Casimir-Polder forces on the near-surface trapping of cold polar molecules, with emphasis on LiH and YbF near a Au surface at room temperature. We show that even for a molecule initially prepared in its electronic and rovibrational ground state, the Casimir-Polder force oscillates with the molecule-wall separation. The nonresonant force and the evanescent part of the resonant force almost exactly cancel at high temperature which results in a saturation of the (attractive) force in this limit. This implies that the Casimir-Polder force on a fully thermalized molecule can differ dramatically from that obtained using a naive perturbative expansion of the Lifshitz formula based on the molecular ground-state polarizability. A dynamical calculation reveals how the spatial oscillations die out on a typical time scale of several seconds as thermalization of the molecule with its environment sets in.
Abstract We investigate the dynamical Casimir-Polder force between an atom and a conducting wall during the time evolution of the system from a partially dressed state. This state is obtained by a sudden change of the atomic position with respect to the plate. To evaluate the time-dependent atom-plate Casimir-Polder force we solve the Heisenberg equations for the field and atomic operators by an iterative technique. We find that the dynamical atom-plate Casimir-Polder interaction exhibits oscillation in time, and can be attractive or repulsive depending on time and the atom-wall distance. We also investigate the time dependence of global observables, such as the field and atomic Hamiltonians, and discuss some interesting features of the dynamical process bringing the interaction energy to the equilibrium configuration.