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arXiv:quant-ph/0402070 · Physical Review A

Magneto-optical rotation and cross-phase modulation via coherently driven four-level atoms in a tripod configuration

David Petrosyan, Yuri P. Malakyan

Published Aug 30, 2004• 190 citations

Abstract

We study the interaction of a weak probe field, having two orthogonally polarized components, with an optically dense medium of four-level atoms in a tripod configuration. In the presence of a coherent driving laser, electromagnetically induced transparency is attained in the medium, dramatically enhancing its linear as well as nonlinear dispersion while simultaneously suppressing the probe field absorption. We present the semiclassical and fully quantum analysis of the system. We propose an experimentally feasible setup that can induce large Faraday rotation of the probe field polarization and therefore be used for ultrasensitive optical magnetometry. We then study the Kerr nonlinear coupling between the two components of the probe, demonstrating a novel regime of symmetric, extremely efficient cross-phase modulation, capable of fully entangling two single-photon pulses. This scheme may thus pave the way to photon-based quantum information applications, such as deterministic all-optical quantum computation, dense coding, and teleportation.

DOI: 10.1103/physreva.70.023822

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We investigate, both theoretically and experimentally, the cross-Kerr nonlinearity generated in a four-level tripod system in the 87Rb D1 line. The system exhibits simultaneous electromagnetically induced transparency (EIT) windows for two weak (probe and trigger) fields and the enhanced cross-Kerr nonlinearity by EIT. The cross-Kerr nonlinear phase shifts for probe (trigger) field are measured at several different intensities of trigger (probe) field. The results show that large cross-phase modulation (XPM) coefficients can be achieved at low light intensities.

We report experimental observations on the simultaneous electromagnetically induced transparency (EIT) effects for probe and trigger fields (double EIT) as well as the enhanced cross-phase modulation (XPM) between the two fields in a four-level tripod EIT system of the D1 line of 87Rb atoms. The XPM coefficients (larger than 2 x 10(-5) cm2/W) and the accompanying transmissions (higher than 60%) are measured at a slight detuning of the probe field from the exact EIT-resonance condition. The system and enhanced cross-Kerr nonlinearities presented here can be applied to quantum information processes.

We investigate a four-level double-Lambda atomic scheme interacting with four laser fields, a weak probe field, a weak signal field and two driven fields, in a closed-loop configuration. We study the Kerr nonlinearity associated with cross-phase modulation based on electromagnetically induced transparency. Our results show, in this closed-loop system, that the strength of cross-phase modulation and two-photon absorption are dependent critically on the relative phase between the excitation paths. By choosing the parameters appropriately, large cross-phase modulation can be achieved within a wide transparency window, while two-photon absorption is cancelled completely. The strength of cross-phase modulation can be enhanced much more by decreasing the intensities of two driven fields.

We investigate a four-level double-Λ atomic scheme interacting with four laser fields, a weak probe field, a weak signal field and two driven fields, in a closed-loop configuration. We study the Kerr nonlinearity associated with cross-phase modulation based on electromagnetically induced transparency. Our results show, in this closed-loop system, that the strength of cross-phase modulation and two-photon absorption are dependent critically on the relative phase between the excitation paths. By choosing the parameters appropriately, large cross-phase modulation can be achieved within a wide transparency window, while two-photon absorption is cancelled completely. The strength of cross-phase modulation can be enhanced much more by decreasing the intensities of two driven fields.

We investigate the Kerr and magneto-optical effects for a probe laser field with two orthogonally polarized components, propagating in a cold Rydberg atomic gas with an inverted-

\mathsf{Y}

-type level configuration via double electromagnetically induced transparency (EIT). Through an approach beyond both mean-field and ground-state approximations, we make detailed calculations on third-order nonlinear optical susceptibilities and show that the system possesses giant nonlocal self- and cross-Kerr nonlinearities contributed by Rydberg-Rydberg interaction. The theoretical result of the cross-Kerr nonlinearity obtained for

^{85}\mathrm{Rb}

atomic gas is very close to the experimental one reported recently. Moreover, we demonstrate that the probe laser field can acquire a very large magneto-optical rotation via the double EIT, which may be used to design atomic magnetometers with high precision. The results presented here are promising not only for the development of nonlocal nonlinear magneto-optics but also for applications in precision measurement and optical information processing and transmission based on Rydberg atomic gases.

A four-level inverted-Y scheme with an electromagnetically induced transparency (EIT) core is investigated for the enhancement of cross-Kerr effect in rubidium atoms. When detunings of the coupling and control fields are appropriately set, an enhanced EIT window is observed, and the induced phase shift of the probe field due to cross-phase modulation (XPM) is obtained by measuring the dispersive property of the probe transition. The maximal XPM phase shift is about 12° under the current experimental conditions. The experimental measurements agree well with the theoretical calculations. The enhanced XPM phase shift in such an atomic system has applications in quantum nonlinear optics and quantum information science.