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arXiv:2104.10815 · Physical Review A

Giant Kerr nonlinearities and magneto-optical rotations in a Rydberg-atom gas via double electromagnetically induced transparency

Yue Mu, Lu Qin, Zeyun Shi, Guoxiang Huang

Published Apr 12, 2021• 33 citations
arXivHTMLPDF

Abstract

We investigate the Kerr and magneto-optical effects for a probe laser field with two orthogonally polarized components, propagating in a cold Rydberg atomic gas with an inverted-$\mathsf{Y}$-type level configuration via double electromagnetically induced transparency (EIT). Through an approach beyond both mean-field and ground-state approximations, we make detailed calculations on third-order nonlinear optical susceptibilities and show that the system possesses giant nonlocal self- and cross-Kerr nonlinearities contributed by Rydberg-Rydberg interaction. The theoretical result of the cross-Kerr nonlinearity obtained for $^{85}\mathrm{Rb}$ atomic gas is very close to the experimental one reported recently. Moreover, we demonstrate that the probe laser field can acquire a very large magneto-optical rotation via the double EIT, which may be used to design atomic magnetometers with high precision. The results presented here are promising not only for the development of nonlocal nonlinear magneto-optics but also for applications in precision measurement and optical information processing and transmission based on Rydberg atomic gases.

DOI
10.1103/physreva.103.043709

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We investigate the Kerr and magneto-optical effects for a probe laser field with two orthogonally polarized components, propagating in a cold Rydberg atomic gas with an inverted-Y\mathsf{Y}Y-type level configuration via double electromagnetically induced transparency (EIT). Through an approach beyond both mean-field and ground-state approximations, we make detailed calculations on third-order nonlinear optical susceptibilities and show that the system possesses giant nonlocal self- and cross-Kerr nonlinearities contributed by Rydberg-Rydberg interaction. The theoretical result of the cross-Kerr nonlinearity obtained for 85Rb^{85}\mathrm{Rb}85Rb atomic gas is very close to the experimental one reported recently. Moreover, we demonstrate that the probe laser field can acquire a very large magneto-optical rotation via the double EIT, which may be used to design atomic magnetometers with high precision. The results presented here are promising not only for the development of nonlocal nonlinear magneto-optics but also for applications in precision measurement and optical information processing and transmission based on Rydberg atomic gases.
We investigate the optical Kerr nonlinearities of an ensemble of cold Rydberg atoms under the condition of electromagnetically induced transparency (EIT). By using an approach beyond mean-field theory, we show that the system possesses not only enhanced third-order nonlinear optical susceptibility, but also giant fifth-order nonlinear optical susceptibility, which has a cubic dependence on atomic density. Our results demonstrate that both the third-order and the fifth-order nonlinear optical susceptibilities consist of two parts, contributed respectively by photon-atom interaction and Rydberg-Rydberg interaction. The Kerr nonlinearity induced by the Rydberg-Rydberg interaction plays a leading role at high atomic density. We find that the fifth-order nonlinear optical susceptibility in the Rydberg-EIT system may be five orders of magnitude larger than that obtained in traditional EIT systems. The results obtained may have promising applications in light and quantum information processing and transmission at weak-light level.
XXX waves are a special type of wave packet that can maintain their transverse profile of XXX shape during propagation, and they are of much interest for the study of fundamental physics and practical applications. Here we present a scheme to generate nonlinear XXX waves and realize their active control by using a cold gas of Rydberg atoms via electromagnetically induced transparency (EIT). We show that, due to the EIT effect contributed by a control laser field and the strong, nonlocal Kerr nonlinearity contributed by Rydberg-Rydberg interaction between atoms, the system supports high-dimensional, nonlocal, and nonlinear optical XXX waves, which have low propagation loss, ultraslow propagation velocity, and ultralow generation power. We also show that the stability domain of such XXX waves can be greatly enlarged by increasing the nonlocality degree of the Kerr nonlinearity, and their motion trajectory can be manipulated by using an external magnetic field. Our study opens a route for generating and controlling nonlocal ultraslow nonlinear optical XXX waves, which may have promising applications in optical information processing and transmission.
We study the interaction of a weak probe field, having two orthogonally polarized components, with an optically dense medium of four-level atoms in a tripod configuration. In the presence of a coherent driving laser, electromagnetically induced transparency is attained in the medium, dramatically enhancing its linear as well as nonlinear dispersion while simultaneously suppressing the probe field absorption. We present the semiclassical and fully quantum analysis of the system. We propose an experimentally feasible setup that can induce large Faraday rotation of the probe field polarization and therefore be used for ultrasensitive optical magnetometry. We then study the Kerr nonlinear coupling between the two components of the probe, demonstrating a novel regime of symmetric, extremely efficient cross-phase modulation, capable of fully entangling two single-photon pulses. This scheme may thus pave the way to photon-based quantum information applications, such as deterministic all-optical quantum computation, dense coding, and teleportation.
Abstract Rydberg atoms, characterized by their giant polarizability and strong long-range interactions, provide an ideal platform for exploring optical nonlinearities. By coupling light to ensembles of Rydberg atoms, one can map the strong and nonlocal interactions between Rydberg atoms and light fields. A particularly important scheme for realizing such nonlinearity is electromagnetically induced transparency (EIT). This article presents a review of the research progress in nonlinear optics based on Rydberg-EIT systems, particularly nonlinear light propagation in Rydberg atomic gases. We first introduce the fundamental properties of Rydberg atoms and the physical mechanism of EIT-enhanced nonlinearity, emphasizing how the Rydberg blockade effect endows the system with a giant nonlocal Kerr nonlinearity. Subsequently, we discuss some typical nonlinear optical phenomena in such a system with focusing and defocusing nonlocal nonlinearities. In the focusing regime, we discuss spatial solitons, vortex solitons, soliton cloning, soliton molecules, optical bullets, and self-induced transparency solitons. Other topics are also discussed. In the defocusing regime, we analyze pattern formation and shock wave dynamics. Finally, we provide an outlook on the future development of this field toward quantum control, hybrid-system integration, and novel functional devices.
We investigate the formation and control of stationary optical patterns in a cold Rydberg atomic gas via double electromagnetically induced transparency. We show that, through the modulational instability of the plane-wave state of a laser field with two polarization components, the system undergoes a spontaneous symmetry breaking and hence the emergence of plentiful self-organized spatial optical structures, which can be manipulated by the ratio between the cross- and self-Kerr nonlinearities, the nonlocality degree of the Kerr nonlinearities, and the populations initially prepared in the two atomic ground states. Interestingly, a crossover from mixture to separation in space (optical phase separation) of the two polarization components occurs when the ratio between the cross- and self-Kerr nonlinearities exceeds a critical value. We also show that the system supports nonlocal two-component spatial optical solitons and vortices when the parameters of the system are selected suitably. The rich diversity and active controllability of the self-organized optical structures reported here provide a way for realizing novel optical patterns and solitons and their structural phase transitions based on Rydberg atomic gases.
We investigate the linear and nonlinear optical response to an optical pumping of a four-level atomic system with electromagnetically induced transparency (EIT) in a cold Rydberg atomic gas. It is found that the transient behavior (especially, the third- and fifth-order susceptibilities) of the probe field, and the steady-state EIT spectrum of the gas, depend crucially on the Rydberg atoms' interaction. Furthermore, we find that the response speed of the Rydberg interaction with EIT can be as much as six times faster than the EIT without the Rydberg interaction, and that the nonlinear response time of the fifth-order optical susceptibility is longer than that of the third-order susceptibility. It is established that the Rydberg blockade effect plays a significant role in increasing the response speed of the Rydberg with EIT.