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arXiv:quant-ph/0401130 · Physical Review Letters

Stability of Atomic Clocks Based on Entangled Atoms

Axel André, Anders Søndberg Sørensen, Mikhail D. Lukin

Published Jun 7, 2004• 157 citations
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Abstract

We analyze the effect of realistic noise sources for an atomic clock consisting of a local oscillator that is actively locked to a spin-squeezed (entangled) ensemble of N atoms. We show that the use of entangled states can lead to an improvement of the long-term stability of the clock when the measurement is limited by decoherence associated with instability of the local oscillator combined with fluctuations in the atomic ensemble's Bloch vector. Atomic states with a moderate degree of entanglement yield the maximal clock stability, resulting in an improvement that scales as N(1/6) compared to the atomic shot noise level.

DOI
10.1103/physrevlett.92.230801

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We analyze the effect of realistic noise sources for an atomic clock consisting of a local oscillator that is actively locked to a spin-squeezed (entangled) ensemble of N atoms. We show that the use of entangled states can lead to an improvement of the long-term stability of the clock when the measurement is limited by decoherence associated with instability of the local oscillator combined with fluctuations in the atomic ensemble's Bloch vector. Atomic states with a moderate degree of entanglement yield the maximal clock stability, resulting in an improvement that scales as N(1/6) compared to the atomic shot noise level.
We show that the stability of an optical atomic clock can only be improved by spin squeezed states for ensembles below a critical particle number. This limitation results from a trade-off between measurement noise and instabilities due to limited laser coherence. Our results apply to the case of cyclic Ramsey interrogations on a single atomic ensemble with dead time between each measurement. The combination of analytical models for projection noise, dead time noise (Dick effect) and laser phase noise allows quantitative predictions of the critical particle number and the optimal clock stability for a given dead time and laser noise. Our analytical predictions are confirmed by numerical simulations of the closed servo loop of an optical atomic clock.
The ultimate stability of atomic clocks is limited by the quantum noise of the atoms. To reduce this noise it has been suggested to use entangled atomic ensembles with reduced atomic noise. Potentially this can push the stability all the way to the limit allowed by the Heisenberg uncertainty relation, which is denoted the Heisenberg limit. In practice, however, entangled states are often more prone to decoherence, which may prevent reaching this performance. Here we present an adaptive measurement protocol that in the presence of a realistic source of decoherence enables us to get near-Heisenberg-limited stability of atomic clocks using entangled atoms. The protocol may thus realize the full potential of entanglement for quantum metrology despite the detrimental influence of decoherence.
Optical atomic clocks are a driving force for precision measurements due to the high accuracy and stability demonstrated in recent years. While further improvements to the stability have been envisioned by using entangled atoms, squeezing the quantum mechanical projection noise, evaluating the overall gain must incorporate essential features of an atomic clock. Here, we investigate the benefits of spin squeezed states for clocks operated with typical Brownian frequency noise-limited laser sources. Based on an analytic model of the closed servo-loop of an optical atomic clock, we report here quantitative predictions on the optimal clock stability for a given dead time and laser noise. Our analytic predictions are in good agreement with numerical simulations of the closed servo-loop. We find that for usual cyclic Ramsey interrogation of single atomic ensembles with dead time, even with the current most stable lasers spin squeezing can only improve the clock stability for ensembles below a critical atom number of about one thousand in an optical Sr lattice clock. Even with a future improvement of the laser performance by one order of magnitude the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers.
Optical atomic clocks are a driving force for precision measurements due to the high accuracy and stability demonstrated in recent years. While further improvements to the stability have been envisioned by using entangled atoms, squeezing the quantum mechanical projection noise, evaluating the overall gain must incorporate essential features of an atomic clock. Here, we investigate the benefits of spin squeezed states for clocks operated with typical Brownian frequency noise-limited laser sources. Based on an analytic model of the closed servo-loop of an optical atomic clock, we report here quantitative predictions on the optimal clock stability for a given dead time and laser noise. Our analytic predictions are in good agreement with numerical simulations of the closed servo-loop. We find that for usual cyclic Ramsey interrogation of single atomic ensembles with dead time, even with the current most stable lasers spin squeezing can only improve the clock stability for ensembles below a critical atom number of about one thousand in an optical Sr lattice clock. Even with a future improvement of the laser performance by one order of magnitude the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers. © 2020, The Author(s).
The stability of several clock protocols based on 2 to 20 entangled atoms is evaluated numerically by a simulation that includes the effect of decoherence due to classical oscillator noise. In this context the squeezed states discussed by André, Sørensen and Lukin [PRL 92, 239801 (2004)] offer reduced instability compared to clocks based on Ramsey's protocol with unentangled atoms. When more than 15 atoms are simulated, the protocol of Bužek, Derka and Massar [PRL 82, 2207 (1999)] has lower instability. A large-scale numerical search for optimal clock protocols with two to eight qubits yields improved clock stability compared to Ramsey spectroscopy, and for two to three qubits performance matches the analytical protocols. In the simulations, a laser local oscillator decoheres due to flicker-frequency (1/f) noise. The oscillator frequency is repeatedly corrected, based on projective measurements of the qubits, which are assumed not to decohere with one another.
Improving the clock stability is of fundamental importance for the development of quantum-enhanced metrology. One of the main limitations arises from the randomly fluctuating local oscillator (LO) frequency, which introduces ``phase slips'' for long interrogation times and hence the failure of the frequency-feedback loop. Here we propose a strategy to improve the stability of atomic clocks by interrogating two atomic ensembles sharing the same LO. The two ensembles are prepared in coherent spin states pointing along orthogonal directions in the Bloch sphere. While standard Ramsey interrogation can only determine phases unambiguously in the interval $[\ensuremath{-}\ensuremath{\pi}/2,\ensuremath{\pi}/2]$, the joint interrogation allows for an extension to $[\ensuremath{-}\ensuremath{\pi},\ensuremath{\pi}]$, resulting in a relaxed restriction of the Ramsey time and improvement of absolute clock stability. Theoretical predictions are supported by ab initio numerical simulation for white and correlated LO noise. While our basic protocol uses uncorrelated atoms, we further extended it to include spin-squeezing and further improving the scaling of clock stability with the number of atoms. Our protocol can be readily tested in current state-of-the-art experiments.