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arXiv:quant-ph/0308068 · Physical Review A

Controlling dipole-dipole frequency shifts in a lattice-based optical atomic clock

Darrick E. Chang, Jun Ye, Mikhail D. Lukin

Published Feb 24, 2004• 88 citations
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Abstract

Motivated by the ideas of using cold alkaline-earth atoms trapped in an optical lattice for realization of optical atomic clocks, we investigate theoretically the perturbative effects of atom-atom interactions on a clock transition frequency. These interactions are mediated by the dipole fields associated with the optically excited atoms. We predict resonancelike features in the frequency shifts when constructive interference among atomic dipoles occur. We theoretically demonstrate that by fine tuning the coherent dipole-dipole couplings in appropriately designed lattice geometries, the undesirable frequency shifts can be greatly suppressed.

DOI
10.1103/physreva.69.023810

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Motivated by the ideas of using cold alkaline-earth atoms trapped in an optical lattice for realization of optical atomic clocks, we investigate theoretically the perturbative effects of atom-atom interactions on a clock transition frequency. These interactions are mediated by the dipole fields associated with the optically excited atoms. We predict resonancelike features in the frequency shifts when constructive interference among atomic dipoles occur. We theoretically demonstrate that by fine tuning the coherent dipole-dipole couplings in appropriately designed lattice geometries, the undesirable frequency shifts can be greatly suppressed.
We report a hitherto undiscovered frequency shift for forbidden J = 0-->J = 0 clock transitions excited in atoms confined to an optical lattice. These shifts result from magnetic-dipole and electric-quadrupole transitions, which have a spatial dependence in an optical lattice that differs from that of the stronger electric-dipole transitions. In combination with the residual translational motion of atoms in an optical lattice, this spatial mismatch leads to a frequency shift via differential energy level spacing in the lattice wells for ground state and excited state atoms. We estimate that this effect could lead to fractional frequency shifts as large as 10(-16), which might prevent lattice-based optical clocks from reaching their predicted performance levels. Moreover, these effects could shift the magic wavelength in lattice clocks in three dimensions by as much as 100 MHz, depending on the lattice configuration.
Dipole-dipole interactions lead to frequency shifts that are expected to limit the performance of next-generation atomic clocks. In this work, we compute dipolar frequency shifts accounting for the intrinsic atomic multilevel structure in standard Ramsey spectroscopy. When interrogating the transitions featuring the smallest Clebsch-Gordan coefficients, we find that a simplified two-level treatment becomes inappropriate, even in the presence of large Zeeman shifts. For these cases, we show a net suppression of dipolar frequency shifts and the emergence of dominant nonclassical effects for experimentally relevant parameters. Our findings are pertinent to current generations of optical lattice and optical tweezer clocks, opening a way to further increase their current accuracy, and thus their potential to probe fundamental and many-body physics.
Optical lattice clocks combine the accuracy and stability required for next-generation frequency standards. At the heart of these clocks are carefully engineered optical lattices tuned to a wavelength where the differential AC Stark shift between ground and excited states vanishes—the so called ‘magic’ wavelength. To date, only alkaline-earth-like atoms utilizing clock transitions with total electronic angular momentum J=0 have successfully realized these magic wavelength optical lattices at the level necessary for state-of-the-art clock operation. In this article, we discuss two additional types of clock transitions utilizing states with J≠0, leveraging hyperfine structure to satisfy the necessary requirements for controlling lattice-induced light shifts. We propose realizing (i) clock transitions between same-parity clock states with total angular momentum F=0 and (ii) M1/E2 clock transitions between a state with F=0 and a second state with J=1/2, mF=0. We present atomic species which fulfill these requirements before giving a detailed discussion of both manganese and copper, demonstrating how these transitions provide the necessary suppression of fine structure-induced vector and tensor lattice light shifts for clock operations. Such realization of alternative optical lattice clocks promises to provide a rich variety of new atomic species for neutral atom clock operation, with applications from many-body physics to searches for new physics.
We develop a method of spectroscopy that uses a weak static magnetic field to enable direct optical excitation of forbidden electric-dipole transitions that are otherwise prohibitively weak. The power of this scheme is demonstrated using the important application of optical atomic clocks based on neutral atoms confined to an optical lattice. The simple experimental implementation of this method--a single clock laser combined with a dc magnetic field--relaxes stringent requirements in current lattice-based clocks (e.g., magnetic field shielding and light polarization), and could therefore expedite the realization of the extraordinary performance level predicted for these clocks. We estimate that a clock using alkaline-earth-like atoms such as Yb could achieve a fractional frequency uncertainty of well below 10(-17) for the metrologically preferred even isotopes.
We report on the direct observation of resonant electric dipole-dipole interactions in a cubic array of atoms in the many-excitation limit. The interactions, mediated by single-atom couplings to the shared electromagnetic vacuum, are shown to produce spatially-dependent cooperative Lamb shifts when spectroscopically interrogating the mHz-wide optical clock transition in strontium-87. We show that the ensemble-averaged shifts can be suppressed below the level of evaluated systematic uncertainties for state-of-the-art optical atomic clocks. Additionally, we demonstrate that excitation of the atomic dipoles near a Bragg angle can enhance these effects by nearly an order of magnitude compared to non-resonant geometries. Given the remarkable precision of frequency measurements and the high accuracy of the modeled response, our work demonstrates that such a clock is a novel platform for studies of the quantum many-body physics of spins with long-range interactions mediated by propagating photons.