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arXiv:quant-ph/0307039 · Physical Review A

Decoherence in a driven three-level system

A. R. P. Rau, Weichang Zhao

Published Nov 4, 2003• 21 citations
arXivHTMLPDF

Abstract

Dissipation and decoherence, and the evolution from pure to mixed states in quantum physics, are handled through master equations for the density matrix. Master equations such as the Lindblad equation preserve the trace of this matrix. Viewing them as first-order time-dependent operator equations for the elements of the density matrix, a unitary integration procedure can be adapted to solve for these elements. A simple model for decoherence preserves the Hermiticity of the density matrix. A single, classical Riccati equation is the only one requiring numerical handling to obtain a full solution of the quantum evolution. The procedure is general, valid for any number of levels, but is illustrated here for a three-level system with two driving fields. For various choices of the initial state, we study the evolution of the system as a function of the amplitudes, relative frequencies, and phases of the driven fields and of the strength of the decoherence. The monotonic growth of the entropy is followed as the system evolves from a pure to a mixed state. An example is provided by the $n=3$ states of the hydrogen atom in a time-dependent electric field, such degenerate manifolds affording an analytical solution.

DOI
10.1103/physreva.68.052102

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Dissipation and decoherence, and the evolution from pure to mixed states in quantum physics, are handled through master equations for the density matrix. Master equations such as the Lindblad equation preserve the trace of this matrix. Viewing them as first-order time-dependent operator equations for the elements of the density matrix, a unitary integration procedure can be adapted to solve for these elements. A simple model for decoherence preserves the Hermiticity of the density matrix. A single, classical Riccati equation is the only one requiring numerical handling to obtain a full solution of the quantum evolution. The procedure is general, valid for any number of levels, but is illustrated here for a three-level system with two driving fields. For various choices of the initial state, we study the evolution of the system as a function of the amplitudes, relative frequencies, and phases of the driven fields and of the strength of the decoherence. The monotonic growth of the entropy is followed as the system evolves from a pure to a mixed state. An example is provided by the n=3n=3n=3 states of the hydrogen atom in a time-dependent electric field, such degenerate manifolds affording an analytical solution.
Dissipation and decoherence, and the evolution from pure to mixed states in quantum physics, are handled through master equations for the density matrix. By embedding elements of this matrix in a higher-dimensional Liouville-Bloch equation, the methods of unitary integration are adapted to solve for the density matrix as a function of time, including the nonunitary effects of dissipation and decoherence. The input requires only solutions of classical, initial value time-dependent equations. Results are illustrated for a damped, driven two-level system.
The Lindblad master equation governs the general Markovian evolution of a density operator for an open quantum system. Semiclassical Wigner functions represent density operators in phase space in terms of chords on a classical manifold, so that the amplitude and phase of each chord contribution is classically defined. Inserting such a Wigner function into a phase space version of the master equation, its explicit evolution is derived in the absence of dissipation. There results a simple extension of the unitary evolution of the semiclassical Wigner function, which does not affect the phase of each chord contribution, while dampening its amplitude exponentially. Projecting the Wigner function on to an orthogonal position or momentum basis, the dampening of long chords emerges as the exponential decay of off-diagonal elements of the density matrix.
We consider a three-level atom interacting with two optical and one microwave fields in the adiabatic approximation resulting in a simplified description in the terms of a two-level system. Working within the reduced density operator framework, we assume this two-level system to be affected by two types of environment, described by some ad hoc non-Hermitian Hamiltonian and Gorini-Kossakowski-Sudarshan-Lindblad’s models. We compare the three types of dissipative evolution which can occur: driven by equations for a normalized density matrix, a non-normalized density matrix and a normalized state vector. Using the latter type, we derive an effective Hamiltonian, which encodes information about not only the Hamiltonian part of an original master equation but also its non-Hamiltonian (Liouvillian) part. The Hamiltonian turns out to be dependent on the wavefunction itself: the effects of above-mentioned environments induce, respectively, cubic and quintic nonlinear terms. For evolutions driven by density operators, we study various indicators of quantum purity. It is shown that if a trace of density operator is not conserved then conventional von Neumann entropy can no longer be used as a purity indicator; therefore we introduce the purity-normalized definition of quantum statistical entropy.
A unified quantum-statistical framework is proposed for open three-level atomic systems when two lower-energy states are coupled to a single upper state. We suggest a non-Hermitian generalization of the closed model’s Hamiltonian by the analytical continuation of real-valued parameters related to the energies into a complex domain, as well as by considering some terms previously neglected by the procedure of Hermitian conjugation. We show that such systems can have two types of density operator’s evolution, depending on whether they are expected to be sustainable, or in a process of irreversible decay. This approach not only explains previously heuristically introduced terms in equations of motion for the density matrix but also suggests new terms which predict new dissipative effects. We then consider a special case, namely the evolution of pure states described by a generalized Schrödinger equation, which turns out to be nonlinear with respect to the atomic wavefunctions. As a final step toward unification, in addition to the non-Hermitian Hamiltonian generalization, we also include Markovian quantum jumps by adding the Lindblad dissipator. The resulting equations not only expand the range of applicability of open three-level models, but also suggest that dissipative phenomena in quantum-optical systems in vivo are more diverse and significant than previously believed.
We present a comprehensive analytical and numerical study of time-dependent decoherence in open quantum systems, focusing on a single-qubit model with time-varying Lindblad dissipation rates. Employing a master equation framework, we derive exact solutions for the evolution of off-diagonal density matrix elements and characterize the emergence of robust pointer states. Our findings reveal an initial rapid coherence decay followed by a gradual slowdown, mirroring experimental trends observed in superconducting qubits influenced by quasiparticle dynamics and in photonic cavities subject to fluctuating environments. By incorporating real experimental parameters and validating the model through quantum simulations using QuTiP, we provide a robust quantitative tool for analyzing decoherence in quantum technologies. This extended model addresses limitations in static-rate approximations, offering insights into non-Markovian effects without resolving the measurement problem, and suggests extensions to multi-qubit systems.
In this work, we investigate the quantum coherence and purity in hydrogen atoms under dissipative dynamics, with a focus on the hyperfine structure states arising from the electron-proton spin interaction. Using the Lindblad master equation, we model the time evolution of the density matrix of the system, incorporating both the unitary dynamics driven by the hyperfine Hamiltonian and the dissipative effects due to environmental interactions. Quantum coherence is quantified using the L1 norm and relative entropy measures, while purity is assessed via von Neumann entropy, for initial states, including a maximally entangled Bell state and a separable state. Our results reveal distinct dynamics: for the Bell states, both coherence and purity decay exponentially with a rate proportional to the dissipation parameter, whereas for a kind of separable state, coherence exhibits oscillatory behavior modulated via the hyperfine coupling constant, superimposed on an exponential decay, and accompanied by a steady increase in entropy. Higher dissipation rates accelerate the loss of coherence and the growth of von Neumann entropy, underscoring the environment's role in suppressing quantum superposition and driving the system towards mixed states. These findings enhance our understanding of coherence and purity preservation in atomic systems and offer insights for quantum information applications where robustness against dissipation is critical.