A unified quantum-statistical framework is proposed for open three-level atomic systems when two lower-energy states are coupled to a single upper state. We suggest a non-Hermitian generalization of the closed model’s Hamiltonian by the analytical continuation of real-valued parameters related to the energies into a complex domain, as well as by considering some terms previously neglected by the procedure of Hermitian conjugation. We show that such systems can have two types of density operator’s evolution, depending on whether they are expected to be sustainable, or in a process of irreversible decay. This approach not only explains previously heuristically introduced terms in equations of motion for the density matrix but also suggests new terms which predict new dissipative effects. We then consider a special case, namely the evolution of pure states described by a generalized Schrödinger equation, which turns out to be nonlinear with respect to the atomic wavefunctions. As a final step toward unification, in addition to the non-Hermitian Hamiltonian generalization, we also include Markovian quantum jumps by adding the Lindblad dissipator. The resulting equations not only expand the range of applicability of open three-level models, but also suggest that dissipative phenomena in quantum-optical systems in vivo are more diverse and significant than previously believed.
A unified quantum-statistical framework is proposed for open three-level atomic systems when two lower-energy states are coupled to a single upper state. We suggest a non-Hermitian generalization of the closed model’s Hamiltonian by the analytical continuation of real-valued parameters related to the energies into a complex domain, as well as by considering some terms previously neglected by the procedure of Hermitian conjugation. We show that such systems can have two types of density operator’s evolution, depending on whether they are expected to be sustainable, or in a process of irreversible decay. This approach not only explains previously heuristically introduced terms in equations of motion for the density matrix but also suggests new terms which predict new dissipative effects. We then consider a special case, namely the evolution of pure states described by a generalized Schrödinger equation, which turns out to be nonlinear with respect to the atomic wavefunctions. As a final step toward unification, in addition to the non-Hermitian Hamiltonian generalization, we also include Markovian quantum jumps by adding the Lindblad dissipator. The resulting equations not only expand the range of applicability of open three-level models, but also suggest that dissipative phenomena in quantum-optical systems in vivo are more diverse and significant than previously believed.
Within the framework of the quantum-statistical approach, utilizing both non-Hermitian Hamiltonian and Lindblad’s jump operators, one can derive various generalizations of the von Neumann equation for reduced density operators, also known as hybrid master equations. If one considers the evolution of pure states only, i.e., disregarding the coherence between states and spontaneous transitions from pure to mixed states, then one can resort to quantum-mechanical equations of the Schrödinger type. We derive them from the hybrid master equations and study their main properties, which indicate that our equations have a larger range of applicability compared to other generalized Schrödinger equations proposed hitherto. Among other features, they can describe not only systems which remain in the stationary eigenstates of the Hamiltonian as time passes, but also those which evolve from those eigenstates. As an example, we consider a simple but important model, a quantum harmonic oscillator driven by both Hamiltonian and non-Hamiltonian terms, and derive its classical limit, which turns out to be the damped harmonic oscillator. Using this model, we demonstrate that the effects of dissipative environments of different types can cancel each other, thus resulting in an effectively dissipation-free classical system. Another discussed phenomenon is whether a non-trivial quantum system can reduce to a classical system in free motion, i.e., without experiencing any classical Newtonian forces. This uncovers a large class of quantum-mechanical non-Hamiltonian systems whose dynamics are not determined by conventional mechanics’ potentials and forces, but rather come about through quantum statistical effects caused by the system’s environment.
We consider a three-level atom interacting with two optical and one microwave fields in the adiabatic approximation resulting in a simplified description in the terms of a two-level system. Working within the reduced density operator framework, we assume this two-level system to be affected by two types of environment, described by some ad hoc non-Hermitian Hamiltonian and Gorini-Kossakowski-Sudarshan-Lindblad’s models. We compare the three types of dissipative evolution which can occur: driven by equations for a normalized density matrix, a non-normalized density matrix and a normalized state vector. Using the latter type, we derive an effective Hamiltonian, which encodes information about not only the Hamiltonian part of an original master equation but also its non-Hamiltonian (Liouvillian) part. The Hamiltonian turns out to be dependent on the wavefunction itself: the effects of above-mentioned environments induce, respectively, cubic and quintic nonlinear terms. For evolutions driven by density operators, we study various indicators of quantum purity. It is shown that if a trace of density operator is not conserved then conventional von Neumann entropy can no longer be used as a purity indicator; therefore we introduce the purity-normalized definition of quantum statistical entropy.
We compare two approaches to open quantum systems, namely, the non-Hermitian dynamics and the Lindblad master equation. In order to deal with more general dissipative phenomena, we propose the unified master equation that combines the characteristics of both of these approaches. This allows us to assess the differences between them as well as to clarify which observed features come from the Lindblad or the non-Hermitian part, when it comes to experiment. Using a generic two-mode single-atom laser system as a practical example, we analytically solve the dynamics of the normalized density matrix operator. We study the two-level model in a number of cases (depending on parameters and types of dynamics), compute different observables and study their physical properties. It turns out that one can not only able to describe the different types of damping in dissipative quantum optical systems but also mimic the undamped anharmonic oscillatory phenomena which happen in quantum systems with more than two levels (while staying within the framework of the analytically simple two-mode approximation).
The Lindblad (GKLS) master equation, which represents the mathematical form for the general evolution of a density matrix, is a versatile and widely-used tool in open quantum systems. In contrast with the typical approach of imposing additional conditions on the system, such as weak coupling or energy conservation, we explore the structure of the equation with no assumptions. We demonstrate that general quantum dynamics can be expressed through a combination of free evolution, exchanges of some physical quantities (generalised charges), not necessarily commuting with the Hamiltonian, between the system and the bath, and pure dephasing. This result comprises a novel perspective on quantum master equations, employing physical processes as elemental parts. We use it to explore the dynamics and stationary states of a two-level system and show that strong coupling, particle exchange, and non-Abelian effects all share the same physical origin. Moreover, we demonstrate that the generalised Gibbs state for all three cases contains a non-commutation term, which has not been previously considered.
Non-Hermitian Hamiltonians and Lindblad operators are some of the most important generators of dynamics for describing quantum systems interacting with different kinds of environments. The first type differs from conservative evolution by an anti-Hermitian term that causes particle decay, while the second type differs by a dissipation operator in Lindblad form that allows energy exchange with a bath. However, although under some conditions the two types of maps can be used to describe the same observable, they form a disjoint set. In this work, we propose a generalized generator of dynamics of the form Lmixed(z,ρS)=−i[H,ρS]+∑i(z+Γc,iΓc,iFiρSFi†−21{Fi†Fi,ρS}+) that depends on a general energy z, and has a tunable parameter Γc that determines the degree of particle density lost. It has as its limits non-Hermitian (Γc→0) and Lindbladian dynamics (Γc→∞). The intermediate regime evolves density matrices such that 0≤Tr(ρS)≤1. We derive our generator with the help of an ancillary continuum manifold acting as a sink for particle density. The evolution describes a system that can exchange both particle density and energy with its environment. We illustrate its features for a two level system and a five M level system with a coherent population trapping point.
Abstract In the conventional quantum mechanics of conserved systems, Hamiltonian is assumed to be a Hermitian operator. However, when it comes to quantum systems in presence of dissipation and/or noise, including open quantum optical systems, the strict hermiticity requirement is nor longer necessary. In fact, it can be substantially relaxed: the non-Hermitian part of a Hamiltonian is allowed, in order to account for effects of dissipative environment, whereas its Hermitian part would be describing subsystem’s energy. Within the framework of the standard approach to dissipative phenomena based on a master equation for the reduced density operator, we propose a replacement of the hermiticity condition by a more general condition of commutativity between Hermitian and anti-Hermitian parts of a Hamiltonian. As an example, we consider a dissipative two-mode quantum system coupled to a single-mode electromagnetic wave, where we demonstrate that the adjoint-commutativity condition does simplify the parametric space of the model.