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arXiv:quant-ph/0207133 · Journal of the Optical Society of America B

Doppler cooling to the recoil limit by means of sharp atomic transitions with controlled quenching

Véronique Zehnlé, Jean Claude Garreau

Published May 1, 2003• 3 citations
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Abstract

We develop an analytical approach to Doppler cooling of atoms by one- or two-photon transitions when the natural width of the excited level is so small that the process leads to a Doppler temperature comparable with the recoil temperature. In such a limit the usual Fokker–Planck equation for Doppler cooling does not correctly describe the cooling process. We propose a generalization of the Fokker–Planck approach and derive a new model that is able to reproduce the numerical results correctly, even very close to the recoil limit. Two cases of practical interest, one-photon Doppler cooling of strontium and two-photon Doppler cooling of hydrogen, are considered. We also treat the possibility of adding a controlled quenching of the sharp line to optimize the cooling process.

DOI
10.1364/josab.20.000931

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We develop an analytical approach to Doppler cooling of atoms by one- or two-photon transitions when the natural width of the excited level is so small that the process leads to a Doppler temperature comparable with the recoil temperature. In such a limit the usual Fokker–Planck equation for Doppler cooling does not correctly describe the cooling process. We propose a generalization of the Fokker–Planck approach and derive a new model that is able to reproduce the numerical results correctly, even very close to the recoil limit. Two cases of practical interest, one-photon Doppler cooling of strontium and two-photon Doppler cooling of hydrogen, are considered. We also treat the possibility of adding a controlled quenching of the sharp line to optimize the cooling process.
We propose and analyze the possibility of performing two-photon continuous-wave Doppler cooling of hydrogen atoms using the $1S\ensuremath{-}2S$ transition. ``Quenching'' of the 2S2S2S level (by coupling with the 2P2P2P state) is used to increase the cycling frequency, and to control the equilibrium temperature. Theoretical and numerical studies of the heating effect due to Doppler-free two-photon transitions evidence an increase of the temperature by a factor of 2. The equilibrium temperature decreases with the effective (quenching-dependent) width of the excited state and can thus be adjusted up to values close to the recoil temperature.
We present a quantum theory of one-dimensional laser cooling of free atoms using a transition with a J = 0 ground state and a J = 1 excited state. This treatment is valid both for broad lines (recoil energy small compared with the energy width ℏ Γ of the excited level) and for narrow lines. For broad lines we recover the well-known cooling limit for a two-level transition (∼ℏΓ/2), whereas for a narrow line the cooling limit is found to be of the order of the recoil energy. The stationary momentum distribution is obtained for both cases and is found to be close to the one obtained by Monte Carlo simulations.
Based on the numerical solution of the quantum kinetic equation for the atomic density matrix, which makes it possible to accurately take into account the recoil effects in the interaction of atoms with field photons, we have studied the limits of laser cooling of atoms using closed optical transitions characterised by different recoil parameters (the ratio of the recoil energy to the natural linewidth). It is shown that for optical transitions with an insufficiently small recoil parameter, the polarisation effects, which lead to the possibility of sub-Doppler laser cooling, lose their efficiency and do not ensure an attainment of the temperature below the Doppler limit. The analysis performed allows one to outline the boundaries of the sub-Doppler theory of laser cooling of atoms.
The laser cooling of atoms with a narrow-line optical transition, i.e., in regimes of quantum nature of laser-light interactions resulting in a significant recoil effect, is studied. It is demonstrated that a minimum laser-cooling temperature for two-level atoms in a standing wave reached for red detuning close to three recoil frequencies is vastly different from the theory used for a semiclassical description of Doppler cooling. A set of dimensionless parameters uniquely characterizing the time evolution and the steady state of different atoms with narrow-line optical transitions in the laser field is introduced. The results can be used for analysis of optimal conditions for laser cooling of atoms with narrow lines such as Ca, Sr, and Mg, which are of great interest for atomic clocks.