Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:quant-ph/0207023 · Optics and Spectroscopy

Resonant energy exchange between atoms in dispersing and absorbing surroundings

Ho Trung Dung, L. Knöll, D. -G. Welsch

Published Jun 1, 2003• 4 citations
arXivHTMLPDF

Abstract

Within the framework of quantization of a macroscopic electromagnetic field, a master equation describing both the resonant dipole-dipole interaction (RDDI) and the resonant atom-field interaction in the presence of dispersing and absorbing macroscopic bodies is derived, with the relevant couplings being expressed in terms of the surroundings-assisted Green’s tensor. It is shown that, under certain conditions, the RDDI can be regarded as being governed by an effective Hamiltonian. The theory, which applies to both weak and strong atom-field coupling, is used to study the resonant energy exchange between two (two-level) atoms initially sharing a single excitation. In particular, it is shown that, in the regime of weak atom-field coupling, there is a time window where the energy transfer follows a transfer-rate law of the type obtained by ordinary second-order perturbation theory. Finally, the spectrum of the light emitted during the energy transfer is studied and the line splittings are discussed.

DOI
10.1134/1.1586732

Related papers

Resonant Energy Exchange between Atoms in Dispersing and Absorbing Surroundings

Dung, H T, Knöll, L, Welsch, D G

Within the framework of quantization of the macroscopic electromagnetic field, a master equation describing both the resonant dipole-dipole interaction (RDDI) and the resonant atom-field interaction (RAFI) in the presence of dispersing and absorbing macroscopic bodies is derived, with the relevant couplings being expressed in terms of the surroundings-assisted Green tensor. It is shown that under certain conditions the RDDI can be regarded as being governed by an effective Hamiltonian. The theory, which applies to both weak and strong atom-field coupling, is used to study the resonant energy exchange between two (two-level) atoms sharing initially a single excitation. In particular, it is shown that in the regime of weak atom-field coupling there is a time window, where the energy transfer follows a transfer-rate law of the type obtained by ordinary second-order perturbation theory. Finally, the spectrum of the light emitted during the energy transfer is studied and the line splittings are discussed.

•Jul 3, 2002•5 citations

Resonant dipole-dipole interaction in the presence of dispersing and absorbing surroundings

Ho Trung Dung, L. Knöll, Dirk‐Gunnar Welsch

Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual- and real-photon exchange in the energy transfer between the atoms. In particular, it is shown that for weak atom-field interaction there is a time window, where the energy transfer follows a rate regime of the type obtained by ordinary second-order perturbation theory. Finally, it is shown that the resonant dipole-dipole interaction can change the singlet line of the emitted light to a doublet spectrum for weak atom-field interaction and the doublet spectrum to a triplet spectrum for strong atom-field interaction.

arXiv:quant-ph/0205056•Physical Review A•Dec 26, 2002•234 citations

Dipole‐dipole coupling in the presence of dispersing and absorbing bodies

D.‐G. Welsch, H.T. Dung, L. Knöll

Abstract An effective Hamiltonian and equations of motion for treating both the resonant dipole‐dipole interaction between two‐level atoms and the resonant atom‐field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. It is shown that the dipole‐dipole interaction and the atom‐field interaction, respectively, are closely related to the real part and the imaginary part of the (classical) Green tensor. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual and real photon exchange in the energy transfer between the atoms. To illustrate the powerfulness of the theory, specific results for the case of the atoms being near a dispersing and absorbing microsphere are presented. In particular, the regimes of weak and strong atom‐field coupling are addressed.

arXiv:quant-ph/0205192•Fortschritte der Physik•Feb 26, 2003•5 citations

Interaction of the quantized electromagnetic field with atoms in the presence of dispersing and absorbing dielectric bodies

Stefan Scheel, D.‐G. Welsch

A general theory of the interaction of the quantized electromagnetic field with atoms, in the presence of dispersing and absorbing dielectric bodies of given Kramers-Kronig consistent permittivities, is developed. It is based on a source-quantity representation of the electromagnetic field, in which the electromagnetic-field operators are expressed in terms of a continuous set of fundamental bosonic fields via the Green tensor of the classical problem. Introducing scalar and vector potentials, the formalism is extended to include in the theory the interaction of the quantized electromagnetic field with additional atoms. Both the minimal-coupling scheme and the multipolar-coupling scheme are considered. The theory replaces the standard concept of mode decomposition, which fails for complex permittivities. It enables us to treat the effects of dispersion and absorption in a consistent way and to give a unified approach to the atom-field interaction, without any restriction to a particular interaction regime in a particular frequency range. All relevant information about the dielectric bodies, such as form and intrinsic dispersion and absorption, is contained in the Green tensor. The application of the theory to the spontaneous decay of an excited atom in the presence of dispersing and absorbing bodies is addressed.

arXiv:quant-ph/0006025•Optics and Spectroscopy•Oct 1, 2001•1 citation

Resonant dipole–dipole interaction in confined and strong-coupling dielectric geometries

Ramy El‐Ganainy, Sajeev John

Using the electromagnetic response function of an electric dipole located within a dielectric geometry, we derive the mathematical equivalence between the classical response and quantum mechanical resonant dipole–dipole interaction between two quantum objects (atoms, quantum dots, etc). Cooperative spontaneous emission likewise emerges from this equivalence. We introduce a practical numerical technique using finite difference time domain for calculating both dipole–dipole interaction and collective spontaneous emission in confined dielectric structures, where strong light–matter coupling might arise. This method is capable of obtaining resonant dipole–dipole interaction over a wide range of frequencies in a single run. Our method recaptures the results of quantum mechanical second order perturbation theory for weak light–matter coupling. In strong coupling situations such as near a photonic band edge, second order Rayleigh–Schrödinger perturbation theory leads to divergences, and instead Brillouin–Wigner perturbation theory is required. This is equivalent to the use of a variational wavefunction to describe the exciton transfer between initial and final states. We introduce a system of coupled classical oscillators, that describes resonant dipole–dipole interaction and vacuum Rabi splitting in the strong-coupling regime, and that provides an effective numerical scheme based on the finite difference time domain method. This includes the effects of quantum entanglement and the correlation of quantum fluctuations. We discuss the crossover to Forster energy transfer when quantum correlations between the dipoles are damped by strong environmental interactions.

New Journal of Physics•Aug 13, 2013•36 citations

Cavity-QED interactions of two correlated atoms

Saeideh Esfandiarpour, Hassan Safari, Robert G. Bennett +1 more

Abstract We consider the resonant van der Waals (vdW) interaction between two correlated identical two-level atoms (at least one of which being excited) within the framework of macroscopic cavity quantum electrodynamics in linear, dispersing and absorbing media. The interaction of both atoms with the body-assisted electromagnetic field of the cavity is assumed to be strong. Our time-independent evaluation is based on an extended Jaynes–Cummings model. For a system prepared in a superposition of its dressed states, we derive the general form of the vdW forces, using a Lorentzian single-mode approximation. We demonstrate the applicability of this approach by considering the case of a planar cavity and showing the position dependence of Rabi oscillations. We also show that in the limiting case of weak coupling, our results reproduce the perturbative ones for the case where the field is initially in vacuum state while the atomic state is in a superposition of two correlated states sharing one excitation.

arXiv:1708.05586•Journal of Physics B Atomic Molecular and Optical Physics•Feb 9, 2018•10 citations
Within the framework of quantization of a macroscopic electromagnetic field, a master equation describing both the resonant dipole-dipole interaction (RDDI) and the resonant atom-field interaction in the presence of dispersing and absorbing macroscopic bodies is derived, with the relevant couplings being expressed in terms of the surroundings-assisted Green’s tensor. It is shown that, under certain conditions, the RDDI can be regarded as being governed by an effective Hamiltonian. The theory, which applies to both weak and strong atom-field coupling, is used to study the resonant energy exchange between two (two-level) atoms initially sharing a single excitation. In particular, it is shown that, in the regime of weak atom-field coupling, there is a time window where the energy transfer follows a transfer-rate law of the type obtained by ordinary second-order perturbation theory. Finally, the spectrum of the light emitted during the energy transfer is studied and the line splittings are discussed.
Within the framework of quantization of the macroscopic electromagnetic field, a master equation describing both the resonant dipole-dipole interaction (RDDI) and the resonant atom-field interaction (RAFI) in the presence of dispersing and absorbing macroscopic bodies is derived, with the relevant couplings being expressed in terms of the surroundings-assisted Green tensor. It is shown that under certain conditions the RDDI can be regarded as being governed by an effective Hamiltonian. The theory, which applies to both weak and strong atom-field coupling, is used to study the resonant energy exchange between two (two-level) atoms sharing initially a single excitation. In particular, it is shown that in the regime of weak atom-field coupling there is a time window, where the energy transfer follows a transfer-rate law of the type obtained by ordinary second-order perturbation theory. Finally, the spectrum of the light emitted during the energy transfer is studied and the line splittings are discussed.
Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual- and real-photon exchange in the energy transfer between the atoms. In particular, it is shown that for weak atom-field interaction there is a time window, where the energy transfer follows a rate regime of the type obtained by ordinary second-order perturbation theory. Finally, it is shown that the resonant dipole-dipole interaction can change the singlet line of the emitted light to a doublet spectrum for weak atom-field interaction and the doublet spectrum to a triplet spectrum for strong atom-field interaction.
Abstract An effective Hamiltonian and equations of motion for treating both the resonant dipole‐dipole interaction between two‐level atoms and the resonant atom‐field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. It is shown that the dipole‐dipole interaction and the atom‐field interaction, respectively, are closely related to the real part and the imaginary part of the (classical) Green tensor. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual and real photon exchange in the energy transfer between the atoms. To illustrate the powerfulness of the theory, specific results for the case of the atoms being near a dispersing and absorbing microsphere are presented. In particular, the regimes of weak and strong atom‐field coupling are addressed.
A general theory of the interaction of the quantized electromagnetic field with atoms, in the presence of dispersing and absorbing dielectric bodies of given Kramers-Kronig consistent permittivities, is developed. It is based on a source-quantity representation of the electromagnetic field, in which the electromagnetic-field operators are expressed in terms of a continuous set of fundamental bosonic fields via the Green tensor of the classical problem. Introducing scalar and vector potentials, the formalism is extended to include in the theory the interaction of the quantized electromagnetic field with additional atoms. Both the minimal-coupling scheme and the multipolar-coupling scheme are considered. The theory replaces the standard concept of mode decomposition, which fails for complex permittivities. It enables us to treat the effects of dispersion and absorption in a consistent way and to give a unified approach to the atom-field interaction, without any restriction to a particular interaction regime in a particular frequency range. All relevant information about the dielectric bodies, such as form and intrinsic dispersion and absorption, is contained in the Green tensor. The application of the theory to the spontaneous decay of an excited atom in the presence of dispersing and absorbing bodies is addressed.
Using the electromagnetic response function of an electric dipole located within a dielectric geometry, we derive the mathematical equivalence between the classical response and quantum mechanical resonant dipole–dipole interaction between two quantum objects (atoms, quantum dots, etc). Cooperative spontaneous emission likewise emerges from this equivalence. We introduce a practical numerical technique using finite difference time domain for calculating both dipole–dipole interaction and collective spontaneous emission in confined dielectric structures, where strong light–matter coupling might arise. This method is capable of obtaining resonant dipole–dipole interaction over a wide range of frequencies in a single run. Our method recaptures the results of quantum mechanical second order perturbation theory for weak light–matter coupling. In strong coupling situations such as near a photonic band edge, second order Rayleigh–Schrödinger perturbation theory leads to divergences, and instead Brillouin–Wigner perturbation theory is required. This is equivalent to the use of a variational wavefunction to describe the exciton transfer between initial and final states. We introduce a system of coupled classical oscillators, that describes resonant dipole–dipole interaction and vacuum Rabi splitting in the strong-coupling regime, and that provides an effective numerical scheme based on the finite difference time domain method. This includes the effects of quantum entanglement and the correlation of quantum fluctuations. We discuss the crossover to Forster energy transfer when quantum correlations between the dipoles are damped by strong environmental interactions.
Abstract We consider the resonant van der Waals (vdW) interaction between two correlated identical two-level atoms (at least one of which being excited) within the framework of macroscopic cavity quantum electrodynamics in linear, dispersing and absorbing media. The interaction of both atoms with the body-assisted electromagnetic field of the cavity is assumed to be strong. Our time-independent evaluation is based on an extended Jaynes–Cummings model. For a system prepared in a superposition of its dressed states, we derive the general form of the vdW forces, using a Lorentzian single-mode approximation. We demonstrate the applicability of this approach by considering the case of a planar cavity and showing the position dependence of Rabi oscillations. We also show that in the limiting case of weak coupling, our results reproduce the perturbative ones for the case where the field is initially in vacuum state while the atomic state is in a superposition of two correlated states sharing one excitation.