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arXiv:quant-ph/0203072 · Physical Review A

Decoherence of collective atomic spin states due to inhomogeneous coupling

C. P. Sun, S. Yi, Li You

Published Jun 26, 2003• 28 citations
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Abstract

We investigate the decoherence of a superposition of symmetric collective internal states of an atomic ensemble due to inhomogeneous coupling to external control fields. For asymptotically large system, we find $\sqrt{N}$ as the characteristic decoherence rate scale with N being the total number of atoms. Our results shed new light on attempts for realizing quantum information processing and storage with atomic ensembles.

DOI
10.1103/physreva.67.063815

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We investigate the decoherence of a superposition of symmetric collective internal states of an atomic ensemble due to inhomogeneous coupling to external control fields. For asymptotically large system, we find N\sqrt{N}N​ as the characteristic decoherence rate scale with N being the total number of atoms. Our results shed new light on attempts for realizing quantum information processing and storage with atomic ensembles.
An ensemble of multilevel atoms is a good candidate for a quantum information storage device. The information is encrypted in the collective ground state atomic coherence, which, in the absence of external excitation, is decoupled from the vacuum and therefore decoherence free. However, in the process of manipulation of atoms with light pulses (writing, reading), one inadvertently introduces a coupling to the environment, i.e., a source of decoherence. The dissipation process is often treated as an independent process for each atom in the ensemble, an approach which fails at large atomic optical depths where cooperative effects must be taken into account. In this paper, the cooperative behavior of spin decoherence and population transfer for a system of two, driven multilevel atoms is studied. Not surprisingly, an enhancement in the decoherence rate is found, when the atoms are separated by a distance that is small compared to an optical wavelength; however, it is found that this rate increases even further for somewhat larger separations for atoms aligned along the direction of the driving field's propagation vector. A treatment of the cooperative modification of optical pumping rates and an effect of polarization swapping between atoms is also discussed, lending additional insight into the origin of the collective decay.
The influence of decoherence on quantum memories for photons based on atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states, corresponding to single photons or nonclassical states of light, the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states, which have the same projection onto the relevant quasiparticle mode (dark-state polariton). Several decoherence processes resulting from uncorrelated individual reservoir couplings are analyzed in detail: single-atom spin flips and dephasing, atom loss, and motion of atoms. Furthermore, it is shown that the sensitivity to collective decoherence processes that affect all polariton modes with comparable strength does also not increase with the number of atoms.
When the dynamics of a spin ensemble are expressible solely in terms of symmetric processes and collective spin operators, the symmetric collective states of the ensemble are preserved. These many-body states, which are invariant under particle relabeling, can be efficiently simulated since they span a subspace whose dimension is linear in the number of spins. However, many open system dynamics break this symmetry, most notably when ensemble members undergo identical, but local, decoherence. In this paper, we extend the definition of symmetric collective states of an ensemble of spin-1∕21∕21∕2 particles in order to efficiently describe these more general collective processes. The corresponding collective states span a subspace that grows quadratically with the number of spins. We also derive explicit formulas for expressing arbitrary, identical, local decoherence in terms of these states. We then investigate the open system dynamics of experimentally relevant nonclassical collective atomic states, including superposition and spin squeezed states, subject to various symmetric but local decoherence models.
The symmetric collective states of an atomic spin ensemble (i.e., many-body states that are invariant under particle exchange) are not preserved by decoherence that acts identically but individually on members of the ensemble. We develop a class of collective states in an ensemble of N spin-1/2 particles that is invariant under symmetric local decoherence and find that the dimension of the Hilbert space spanned by these collective states scales only as N^2. We then investigate the open system dynamics of experimentally relevant non-classical collective atomic states, including Schroedinger cat and spin squeezed states, subject to various symmetric but local decoherence models.
Atomic ensembles, comprising clouds of atoms addressed by laser fields, provide an attractive system for both the storage of quantum information and the coherent conversion of quantum information between atomic and optical degrees of freedom. We describe a scheme for full-scale quantum computing with atomic ensembles, in which qubits are encoded in symmetric collective excitations of many atoms. We consider the most important sources of error—imperfect exciton–photon coupling and photon losses—and demonstrate that the scheme is extremely robust against these processes: the required photon emission and collection efficiency threshold is ≳86%. Our scheme uses similar methods to those already demonstrated experimentally in the context of quantum repeater schemes and yet has information processing capabilities far beyond those proposals.
The enhanced collective coupling to weak quantum fields may turn atomic or spin ensembles into an important component in quantum information processing architectures. Inhomogeneous broadening can, however, significantly reduce the coupling and the lifetime of the collective excitation that represent the quantum information. In this paper we show that the width and shape of the inhomogeneous broadening have a striking influence on the dynamics of the cavity-ensemble system and may lead to narrowing of the linewidth of the collective states. We underpin our findings with the examples of a Gaussian and a Lorentzian profile of the inhomogeneity.