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arXiv:quant-ph/0109135 · Physical Review Letters

Generating Entangled Two-Photon States with Coincident Frequencies

Vittorio Giovannetti, Lorenzo Maccone, Jeffrey H. Shapiro, Franco N. C. Wong

Published Apr 17, 2002• 114 citations
arXivHTMLPDF

Abstract

It is shown that parametric down-conversion, with a short-duration pump pulse and a long nonlinear crystal that is appropriately phase matched, can produce a frequency-entangled biphoton state whose individual photons are coincident in frequency. Quantum interference experiments which distinguish this state from the familiar time-coincident biphoton state are described.

DOI
10.1103/physrevlett.88.183602

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It is shown that parametric down-conversion, with a short-duration pump pulse and a long nonlinear crystal that is appropriately phase matched, can produce a frequency-entangled biphoton state whose individual photons are coincident in frequency. Quantum interference experiments which distinguish this state from the familiar time-coincident biphoton state are described.
We demonstrate a new class of frequency-entangled states generated via spontaneous parametric down-conversion under extended phase-matching conditions. Biphoton entanglement with coincident signal and idler frequencies is observed over a broad bandwidth in periodically poled KTiOPO4. We demonstrate high visibility in Hong-Ou-Mandel interferometric measurements under pulsed pumping without spectral filtering, which indicates excellent frequency indistinguishability between the down-converted photons. The coincident-frequency entanglement source is useful for quantum information processing and quantum measurement applications.
Spectral and temporal coincidence and single-particle photon wave packets are described and their widths and durations are found. The degree of entanglement is characterized by the experimentally measurable parameter R defined as the ratio of the coincidence and single-particle spectral widths. In the frequency representation, this parameter is found as a function of the pump-pulse duration. This function is shown to have a minimum and even in the minimum, at rather natural conditions, the parameter R is found to be very high (R=73>>1). The Schmidt number K is found for both short and long pump pulses and interpolated for arbitrary pulse durations. All functional dependences of R and K are found to be identical and numerical difference between them is shown to be not exceeding 20%. Two-time temporal wave function of a biphoton state is investigated in details, and a rather significant difference between the cases of short and long pump pulses is found to occur. In the case of long pulses, the temporal parameter R is defined as the ratio of durations of the single-particle and coincidence signals, and the defined in such a way parameter R is shown to be very close to the Schmidt number K.
We consider a new method for the generation of polarization-frequency entangled states of photon pairs. We use a frequency-nondegenerate regime of spontaneous parametric down conversion where the photon pairs (biphotons) are produced with identical polarizations, propagate mostly in the same direction, but differ in frequency. Entanglement is achieved by a coherent superposition of pairs emitted from two nonlinear crystals, with the polarization of the biphotons from the first crystal being changed by a transformer placed between the two crystals. We show that this scheme allows the degree of entanglement to be controlled by the choice of biphoton frequencies.
A ${\ensuremath{\chi}}^{(2)}$ nonlinear optical crystal is pumped by two temporally well-distinguishable femtosecond laser pulses to generate entangled photon pairs in the process of spontaneous parametric down-conversion. We have observed first- and second-order interference between amplitudes generated from the first and the second pump pulse as a function of the time delay between the two pump pulses. The criteria for first- and second-order interference are found to be very different, which reflect the quantum entanglement nature of the state of spontaneous parametric down-conversion.
We investigate quantum interference effects of entangled two-photon states generated in a nonlinear crystal pumped by femtosecond pulses. Attention is devoted to the effects of the pump-pulse profile (pulse duration and chirp) as well as those originating in second-order dispersion, both in the nonlinear crystal and in the optical elements through which the down-converted photons propagate. The characteristics of the pump pulse, along with the dispersion, influence on the visibility and the symmetry of the coincidence-count interference pattern. Nonlocal dispersion cancellation occurs in some cases.