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Quantum Electronics and Laser Science Conference

Quantum interference using ultrafast spontaneous parametric down-conversion

Mete Atatüre, Alexander V. Sergienko, Bradley M. Jost, E.A. Saleh, Malvin Carl Teich

Published Jan 20, 2003• 0 citations
Publisher

Abstract

Summary form only given. Pairs of entangled photons display a complex quantum state that cannot be represented through a product of single-particle states. The spontaneous parametric down-conversion (SPDC) process, that takes place when a laser pulse pumps a second-order nonlinear crystal has become recently a convenient source of such nonclassical states of light in quantum optics experiments. Nonstationary effects are mainly observed when the pump pulse temporal duration is significantly shorter than the characteristic interaction time in the nonlinear crystal. We introduce a nonstationary theory of SPDC to describe the results of fourth-order quantum-interference experiments when no spectral filtering is applied to the down-converted fields. Experiments involving nonlinear SPDC crystals with three different lengths were performed. The ultraviolet laser pulses were obtained from a Ti:sapphire femtosecond laser with a second-harmonic generator. These pulses were used to pump nonlinear crystals to initiate the process of nonstationary spdc and generate orthogonally-polarized photon pairs. These pairs then went into a polarization interferometer, and the coincidence counts of the detectors at the two output ports of the interferometer were recorded.

DOI
10.1109/qels.1999.807310

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Summary form only given. Pairs of entangled photons display a complex quantum state that cannot be represented through a product of single-particle states. The spontaneous parametric down-conversion (SPDC) process, that takes place when a laser pulse pumps a second-order nonlinear crystal has become recently a convenient source of such nonclassical states of light in quantum optics experiments. Nonstationary effects are mainly observed when the pump pulse temporal duration is significantly shorter than the characteristic interaction time in the nonlinear crystal. We introduce a nonstationary theory of SPDC to describe the results of fourth-order quantum-interference experiments when no spectral filtering is applied to the down-converted fields. Experiments involving nonlinear SPDC crystals with three different lengths were performed. The ultraviolet laser pulses were obtained from a Ti:sapphire femtosecond laser with a second-harmonic generator. These pulses were used to pump nonlinear crystals to initiate the process of nonstationary spdc and generate orthogonally-polarized photon pairs. These pairs then went into a polarization interferometer, and the coincidence counts of the detectors at the two output ports of the interferometer were recorded.
The generation of entangled states of three or more photons through the nonlinear process of spontaneous parametric down-conversion requires the use of a femtosecond pump to provide an indistinguishability of photon pairs generated from different nonlinear crystals. We demonstrate experimentally that the quantum interference between two photons generated in each of the nonlinear crystals will degrade significantly as the duration of the femtosecond pump pulse becomes shorter than the coherence time of the signal and idler photons. Spectral postselection using narrow-band filters compensates this effect at the expense of the photon flux available for detection.
A ${\ensuremath{\chi}}^{(2)}$ nonlinear optical crystal is pumped by two temporally well-distinguishable femtosecond laser pulses to generate entangled photon pairs in the process of spontaneous parametric down-conversion. We have observed first- and second-order interference between amplitudes generated from the first and the second pump pulse as a function of the time delay between the two pump pulses. The criteria for first- and second-order interference are found to be very different, which reflect the quantum entanglement nature of the state of spontaneous parametric down-conversion.
Theory and experiment of two-photon lquotlquotlquotdirectrquotrquotrquot interference for type-II spontaneous parametric down-conversion with an ultrafast pulse laser pump
Fourth-order spatial interference of entangled photon pairs generated in the process of spontaneous parametric down-conversion pumped by a femtosecond pulse laser has been performed for the first time. In theory, it takes into account the transverse correlation between the two photons and is used to calculate the dependence of the visibility of the interference pattern obtained in Young’s double-slit experiment. In this experiment, a short focal length lens and two narrow band interference filters were adopted to eliminate the effects of the broadband pump laser and improve the visibility of the interference pattern under the condition of nearly collinear light and degenerate phase matching.
Two spatially separated type-I nonlinear crystals are pumped by femtosecond laser pulses to create entangled photon pairs in the process of spontaneous parametric down-conversion. The two-photon entangled state exhibits high-visibility quantum interference for both polarization and space-time variables without the need of stringent spectral postselection by using narrow-band filters. The visibility is insensitive to the thickness of the crystals, unlike in the case of pulse pumped type-II parametric down-conversion; therefore the intensity can be easily increased by using thick nonlinear crystals. This method will be indispensable in experiments that require a pulsed source of entangled photon pairs, such as generation of multiphoton entangled states, quantum teleportation, and quantum communications.
Pair creation by spontaneous parametric down-conversion (SPDC) has become a reliable source for single-photon states, used in many kinds of quantum information experiments and applications. In order to be spectrally pure, the two photons within a generated pair should be as frequency-uncorrelated as possible. For this purpose most experiments use narrow bandpass filters, having to put up with a drastic decrease in count rates. This article elaborates (theoretically and by numerical evaluation) the alternative method to engineer a setup such that the SPDC-generated quantum states are intrinsically pure. Using pulsed pump lasers and periodically poled crystals this approach makes bandpass filtering obsolete and allows for significantly higher output intensities and therefore count rates in the detectors. After numerically scanning all common wavelength regimes, polarisation configurations and three different non-linear crystals, we present a broad variety of setups which allow for an implementation of this method.
Summary form only given. By far the most efficient source of two-particle entangled state is spontaneous parametric downconversion (SPDC). Especially, cw laser pumped type-II SPDC has been widely treated as a good source of entangled photon pairs, since one can easily prepare a polarization Bell state. However, femtosecond pulse pumped type-II SPDC shows poor quantum interference visibility when a thick crystal is used. To restore the visibility, one has to use narrow-band spectral filters at the expense of available photon flux. We demonstrate a scheme for high-visibility two-photon interference with thick (3.4 mm.) type-II BaB/sub 2/O/sub 4/ (BBO) crystals in femtosecond pulse pumped SPDC. Polarization Bell states can be prepared using this method without spectral and amplitude post-selection.