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arXiv:quant-ph/0107039 · Journal of Modern Optics

Field quantization, photons and non-Hermitean modes

S. A. Brown, Bryan J. Dalton

Published Jun 1, 2002• 7 citations
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Abstract

Field quantization in unstable optical systems is treated by expanding the vector potential in terms of non-Hermitean (Fox-Li) modes. We define non-Hermitean modes and their adjoints in both the cavity and external regions and make use of the important bi-orthogonality relationships that exist within each mode set. We employ a standard canonical quantization procedure involving the introduction of generalized coordinates and momenta for the electromagnetic (EM) field. Three-dimensional systems are treated, making use of the paraxial and monochromaticity approximations for the cavity non-Hermitean modes. We show that the quantum EM field is equivalent to a set of quantum harmonic oscillators (QHOs), associated with either the cavity or the external region non-Hermitean modes, and thus confirming the validity of the photon model in unstable optical systems. Unlike in the conventional (Hermitean mode) case, the annihilation and creation operators we define for each QHO are not Hermitean adjoints. It is shown that the quantum Hamiltonian for the EM field is the sum of non-commuting cavity and external region contributions, each of which can be expressed as a sum of independent QHO Hamiltonians for each non-Hermitean mode, except that the external field Hamiltonian also includes a coupling term responsible for external non-Hermitean mode photon exchange processes. The non-commutativity of certain cavity and external region annihilation and creation operators is associated with cavity energy gain and loss processes, and may be described in terms of surface integrals involving cavity and external region non-Hermitean mode functions on the cavity-external region boundary. Using the essential states approach and the rotating wave approximation, our results are applied to the spontaneous decay of a two-level atom inside an unstable cavity. We find that atomic transitions leading to cavity non-Hermitean mode photon absorption are associated with a different coupling constant to that for transitions leading to photon emission, a feature consequent on the use of non-Hermitean mode functions. We show that under certain conditions the spontaneous decay rate is enhanced by the Petermann factor.

DOI
10.1080/09500340110095625

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Field quantization in unstable optical systems is treated by expanding the vector potential in terms of non-Hermitean (Fox-Li) modes. We define non-Hermitean modes and their adjoints in both the cavity and external regions and make use of the important bi-orthogonality relationships that exist within each mode set. We employ a standard canonical quantization procedure involving the introduction of generalized coordinates and momenta for the electromagnetic (EM) field. Three-dimensional systems are treated, making use of the paraxial and monochromaticity approximations for the cavity non-Hermitean modes. We show that the quantum EM field is equivalent to a set of quantum harmonic oscillators (QHOs), associated with either the cavity or the external region non-Hermitean modes, and thus confirming the validity of the photon model in unstable optical systems. Unlike in the conventional (Hermitean mode) case, the annihilation and creation operators we define for each QHO are not Hermitean adjoints. It is shown that the quantum Hamiltonian for the EM field is the sum of non-commuting cavity and external region contributions, each of which can be expressed as a sum of independent QHO Hamiltonians for each non-Hermitean mode, except that the external field Hamiltonian also includes a coupling term responsible for external non-Hermitean mode photon exchange processes. The non-commutativity of certain cavity and external region annihilation and creation operators is associated with cavity energy gain and loss processes, and may be described in terms of surface integrals involving cavity and external region non-Hermitean mode functions on the cavity-external region boundary. Using the essential states approach and the rotating wave approximation, our results are applied to the spontaneous decay of a two-level atom inside an unstable cavity. We find that atomic transitions leading to cavity non-Hermitean mode photon absorption are associated with a different coupling constant to that for transitions leading to photon emission, a feature consequent on the use of non-Hermitean mode functions. We show that under certain conditions the spontaneous decay rate is enhanced by the Petermann factor.
A macroscopic, canonical quantization of the EM field and radiating atom system in quantum optics and cavity QED involving classical, linear optical devices, based on expanding the vector potential in terms of quasi mode functions is presented. The quasi mode functions approximate the true mode functions for the device, and are obtained by solving the Helmholtz equation for an idealized spatially dependent electric permittivity function describing the device. The Hamiltonian for the EM field and radiating atom system is obtained in multipolar form and the quantum EM field is found to be equivalent to a set of quantum harmonic oscillators, one oscillator per quasi mode. However, unlike true mode theory where the quantum harmonic oscillators are uncoupled, in the quasi mode theory they are coupled and photon exchange processes can occur. Explicit expressions for the coupling constants are obtained. The interaction energy between the radiative atoms and the quantum EM field depends on the amplitudes of the quasi mode functions at the positions of the radiating atoms, similar to that for the true mode approach. The simpler forms for the quasi mode functions enable the atom-field interaction energy to be written in a form in which the atoms are only coupled to certain types of modes—for example cavity quasi modes, which are large inside the optical cavity. In such cases the escape of energy from excited atoms in the cavity can be pictured in quasi mode theory as a two step process—the atom de-excites and creates a photon in a cavity quasi mode, the photon in the cavity quasi mode is then lost and appears as a photon in an external quasi mode. In this process the first step occurs via the atom-cavity quasi mode interaction, the second through coupling between cavity and external quasi modes. This may be contrasted with the true mode approach, where the excited atom loses its energy and the photon is created in one of the true modes. As all true modes have non-zero amplitudes outside as well as inside the cavity, the escape of energy from excited atoms in the cavity is seen as a one step process. An application of the quasi mode theory to the quantum theory of the beam splitter is outlined. The unitary operator used to describe this device is a scattering operator, relating initial and long time values of annihilation, creation operators for pairs of incident and reflected modes, interpreted here as quasi modes.
Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.
Specific forms of the travelling and trapped vector mode functions for a three-dimensional Fabry-Perot cavity are developed from the general results of the preceding paper, with parameters describing the output cavity mirror chosen for a typical high Q cavity case. Cavity and external quasi-mode functions associated with the quasi-mode theory of macroscopic canonical quantization are then obtained via an idealized choice of output mirror parameters. The coupling constants describing photon exchange processes between the single cavity quasi-mode associated with each Fabry-Perot resonance and various external quasi-modes are calculated, and their slow dependence on the external quasi-mode frequency shows that the conditions for irreversible Markovian damping of the cavity quasi-mode are satisfied. For radiative atoms placed in the cavity the coupling constants for energy exchange processes with sideways travelling external quasi-modes also vary slowely, so that Markovian spontaneous emission damping occurs for the radiative atoms. However, their coupling with the isolated cavity quasi-modes is associated with reversible photon exchanges as represented via one photon Rabi frequencies. The standard model in cavity quantum electrodynamics, in which the basic processes are described by a cavity damping rate, a radiative atom spontaneous decay rate and an atom-cavity mode coupling constant has now been justified in terms of the quasi-mode theory of macroscopic canonical quantization.
Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.
In the present and the accompanying paper a justification of the standard model of cavity quantum electrodynamics is given in terms of a quasi-mode theory of macroscopic canonical quantization. The coupling of the cavity quasi-mode to external quasi-modes is treated for the representative case of the three-dimensional Fabry-Perot cavity. The general form of the travelling and trapped mode functions for this cavity are derived in this paper and the mode-mode coupling constants are calculated in the accompanying paper. The slow dependence of the coupling constants with the mode frequency difference demonstrates that the conditions for Markovian damping of the cavity quasimode are satisfied. As also discussed in the accompanying paper, the interaction of radiative atoms with cavity quasi-modes is associated with reversible energy exchanges between atom and cavity and represented by Rabi coupling constants. The interaction of radiative atoms located within the cavity with sideways travelling external quasi-modes involves slowly varying coupling constants and is associated with irreversible spontaneous emission dampling. The basic processes represented in the standard cavity quantum electrodynamics model and the associated coupling constant and decay rates thereby follow from the quasi-mode theory.
The quantum theory of a one-dimensional optical cavity is developed with emphasis on the presence of output coupling. First the resonant mode is defined and calculated classically. Then the field is decomposed into a sequence of modes by introducing an imaginary boundary at a large distance. The mode functions are proved to be orthogonal with respect to an integration with the dielectric constant as a weighting factor. The Hamiltonian of the field is shown to be equivalent to that of a collection of independent harmonic oscillators, the mass of which is a function of the frequency of oscillation. This equivalent of mass appears on normalizing the mode functions and proves to carry information on the structure of the cavity. Quantization of the field is carried out, and the commutation relation for the electric fields inside and outside the cavity is derived. The commutator is composed of an infinite set of derivatives of $\ensuremath{\delta}$ functions, which discloses the effect of the presence of output coupling and that of the small size of the cavity on the radiation field. Also, the commutator is shown to have some properties common with the classical resonant mode, i.e., the property of exponential decay and its rate.