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European Quantum Electronics Conference (EQEC)

Field quantization in dielectric media and the generalised multipolar hamiltonian

Bryan J. Dalton, S. M. Dutra, E. S. Guerra, P. L. Knight

Published Aug 24, 2005• 0 citations
Publisher

Abstract

Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.

DOI
10.1109/eqec.1994.698269

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Field quantization in dielectric media and the generalized multipolar Hamiltonian

Bryan J. Dalton, E. S. Guerra, P. L. Knight

Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.

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Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.
Canonical quantization of the electromagnetic (EM) field is carried out for the situation where the total charge and current densities are the sum of contributions from neutral dielectric atoms whose effect is to be described purely classically in terms of spatially dependent electric permittivity and magnetic permeability functions, and neutral, stationary radiative atoms whose interaction with the EM field is to be treated quantum mechanically. The coefficients for the expansion of the vector potential in terms of mode functions determined from a generalized Helmholtz equation are chosen as independent generalized coordinates for the EM field. The spatially dependent electric permittivity and magnetic permeability appear in a generalized Helmholtz's equation and the former also occurs in the mode function orthogonality and normalization conditions. The quantum Hamiltonian is derived in a generalized multipolar form rather than the minimal coupling form obtained in other work. The radiative energy is the sum of quantum harmonic oscillator terms, one for each mode. The modes are independent in the present case of exact mode functions associated with the spatially dependent electric permittivity and magnetic permeability, there being no direct mode-mode coupling terms. In the electric dipole approximation the electric interaction energy contribution for each mode and radiative atom is proportional to the scalar product of the dipole operator with the mode function evaluated at the atom, times the annihilation operator, plus the Hermitian adjoint. This form has been widely used in studies of radiative processes for atomic systems in dielectric media, and it is justified here via the canonical quantization procedure. The results apply to the theoretical treatment of numerous quantum optical experiments involving such interactions in the presence of passive, lossless, dispersionless, linear classical optics devices such as resonator cavities, lenses, beam splitters, and so on. An illustrative application of the theory for atomic decay in a one-dimensional Fabry-Perot cavity is given. \textcopyright{} 1996 The American Physical Society.
A macroscopic, canonical quantization of the EM field and radiating atom system in quantum optics and cavity QED involving classical, linear optical devices, based on expanding the vector potential in terms of quasi mode functions is presented. The quasi mode functions approximate the true mode functions for the device, and are obtained by solving the Helmholtz equation for an idealized spatially dependent electric permittivity function describing the device. The Hamiltonian for the EM field and radiating atom system is obtained in multipolar form and the quantum EM field is found to be equivalent to a set of quantum harmonic oscillators, one oscillator per quasi mode. However, unlike true mode theory where the quantum harmonic oscillators are uncoupled, in the quasi mode theory they are coupled and photon exchange processes can occur. Explicit expressions for the coupling constants are obtained. The interaction energy between the radiative atoms and the quantum EM field depends on the amplitudes of the quasi mode functions at the positions of the radiating atoms, similar to that for the true mode approach. The simpler forms for the quasi mode functions enable the atom-field interaction energy to be written in a form in which the atoms are only coupled to certain types of modes—for example cavity quasi modes, which are large inside the optical cavity. In such cases the escape of energy from excited atoms in the cavity can be pictured in quasi mode theory as a two step process—the atom de-excites and creates a photon in a cavity quasi mode, the photon in the cavity quasi mode is then lost and appears as a photon in an external quasi mode. In this process the first step occurs via the atom-cavity quasi mode interaction, the second through coupling between cavity and external quasi modes. This may be contrasted with the true mode approach, where the excited atom loses its energy and the photon is created in one of the true modes. As all true modes have non-zero amplitudes outside as well as inside the cavity, the escape of energy from excited atoms in the cavity is seen as a one step process. An application of the quasi mode theory to the quantum theory of the beam splitter is outlined. The unitary operator used to describe this device is a scattering operator, relating initial and long time values of annihilation, creation operators for pairs of incident and reflected modes, interpreted here as quasi modes.
After giving an outline of the quantization scheme based on the microscopic Hopfield model of a dielectric bulk material, we show how the classical phenomenological Maxwell equations of the electromagnetic field in the presence of dielectric matter of given space- and frequency-dependent complex permittivity can be transferred to quantum theory. Including in the theory the interaction of the medium-assisted field with atomic systems, we present both the minimal-coupling Hamiltonian and the multipolar-coupling Hamiltonian in the Coulomb gauge. To illustrate the concept, we discuss the input--output relations of radiation and the transformation of radiation-field quantum states at absorbing four-port devices, and the spontaneous decay of an excited atom near the surface of an absorbing body and in a spherical micro-cavity with intrinsic material losses. Finally, we give an extension of the quantization scheme to other media such as amplifying media, magnetic media, and nonlinear media.
A general theory of the interaction of the quantized electromagnetic field with atoms, in the presence of dispersing and absorbing dielectric bodies of given Kramers-Kronig consistent permittivities, is developed. It is based on a source-quantity representation of the electromagnetic field, in which the electromagnetic-field operators are expressed in terms of a continuous set of fundamental bosonic fields via the Green tensor of the classical problem. Introducing scalar and vector potentials, the formalism is extended to include in the theory the interaction of the quantized electromagnetic field with additional atoms. Both the minimal-coupling scheme and the multipolar-coupling scheme are considered. The theory replaces the standard concept of mode decomposition, which fails for complex permittivities. It enables us to treat the effects of dispersion and absorption in a consistent way and to give a unified approach to the atom-field interaction, without any restriction to a particular interaction regime in a particular frequency range. All relevant information about the dielectric bodies, such as form and intrinsic dispersion and absorption, is contained in the Green tensor. The application of the theory to the spontaneous decay of an excited atom in the presence of dispersing and absorbing bodies is addressed.
The macroscopic electromagnetic field is quantized in a linear isotropic permeable-dielectric medium by associating a proper damped quantum-mechanical harmonic oscillator with each mode of the radiation field. We introduce a particular form of the Langevin equation with two memory functions and two random impulses to describe the motion of a damped oscillator. A fully canonical approach is used to quantize the damped oscillator, the conjugate momentum is defined and the quantum-mechanical Hamiltonian is introduced. This brings forth a direct method for the quantization of the radiation field and at the same time introduces an effective Hamiltonian operator. Special attention is paid to the vacuum field fluctuation in permeable dielectrics.
Macroscopic canonical quantization of the EM field and radiative atom systems occurring in quantum optics experiments involving linear classical optics devices can be carried out via expansion of the vector potential either in terms of true mode functions for the optical device or in terms of approximate or quasi mode functions. The relationship between the true mode and quasi mode annihilation, creation operators is determined and shown to involve a Bogolubov transformation. Analytic properties are also examined and it is found that the annihilation, creation operators times the square root of the angular frequency are analytic functions of the variables specifying the modes.