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arXiv:physics/9902028 · The European Physical Journal D

Modified Bloch equations in the presence of a nonstationary bath

Jyotipratim Ray Chaudhuri, Suman Kumar Banik, Bimalendu Deb, Deb Shankar Ray

Published Jan 1, 1999• 8 citations
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Abstract

Based on the system-reservoir description, we propose a simple solvable microscopic model for a nonequilibrium bath. This captures the essential features of a nonstationary quantum Markov process. We establish an appropriate generalization of the fluctuation-dissipation relation pertaining to this process and explore the essential modifications of the Bloch equations to reveal the nonexponential decay of the Bloch vector components and transient spectral broadening in resonance fluorescence. We discuss a simple experimental scheme to verify the theoretical results.

DOI
10.1007/pl00021626

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Based on the system-reservoir description, we propose a simple solvable microscopic model for a nonequilibrium bath. This captures the essential features of a nonstationary quantum Markov process. We establish an appropriate generalization of the fluctuation-dissipation relation pertaining to this process and explore the essential modifications of the Bloch equations to reveal the nonexponential decay of the Bloch vector components and transient spectral broadening in resonance fluorescence. We discuss a simple experimental scheme to verify the theoretical results.
We extend the quantum theory of dissipation in the context of system-reservoir model, where the reservoir in question is kept in a nonequilibrium condition. Based on a systematic separation of time scales involved in the dynamics, appropriate generalizations of the fluctuation-dissipation and Einstein's relations have been pointed out. We show that the Wigner-Weisskopf decay of the system mode results in a rate constant which depending on the relaxation of nonequilibrium bath is dynamically modified. We also calculate the time-dependent spectra of a cavity mode with a suitable gain when the cavity is kept in contact with a nonequilibrium bath.
We extend the quantum theory of dissipation in the context of a system-reservoir model, where the reservoir in question is kept in a non-equilibrium condition. Based on a systematic separation of time scales involved in the dynamics, appropriate generalizations of the fluctuation-dissipation and Einstein's relations have been pointed out. We show that the Wigner-Weisskopf decay of the system mode results in a rate constant which, depending on the relaxation of a non-equilibrium bath, is dynamically modified. We also calculate the time-dependent spectra of a cavity mode with a suitable gain when the cavity is kept in contact with a non-equilibrium bath.
For a spin-12\frac{1}{2}21​ coupled to a Gaussian heat bath in the presence of an external magnetic field, we generalize the Bloch equations to the non-Markovian case. Using this generalization as the base, we show that the time-varying component of the magnetic field parallel to its constant part is absorbed by the spin system, especially at high temperatures of the heat bath. For the spectral density and dispersion of longitudinal spin fluctuations, we obtain expressions that are in good agreement with known results.
Understanding the non-Markovian dynamics of dissipative processes induced by memory effects of the environment is a fundamental subject of open quantum systems. Because of the complexity of open quantum systems, e.g., the multiple energy scales involving that of the system, the environment, and their mutual coupling, it is generally a challenging task to characterize the relationship among the parameters of the system dynamics and the reservoir spectra. For the two-level spontaneous emission model within structured environments, it was shown in a recent literature (Opt. Lett. 38, 3650) that a functional relation could be established between the asymptotically non-decaying population and the spectral density of the reservoir as the system undergoes a long-time evolution. It hence renders a distinct perspective to look into the character of long-lived quantum coherence in the corresponding non-Markovian process. This article is devoted to further investigate the phenomena of limit cycle oscillations possibly occurring in such non-Markovian dissipative systems in a long-time evolution. For a two-level system subjected to an environment with Ohmic class spectra, due to the presence of a unique bound-state mode of the system, the evolution trajectory of the given initial states will converge to a limit cycle in the Bloch space. The dependence of the radius and the location of the limit cycle on the spectral density function of the reservoir are manifested by virtue of the described functional relation. For the model subjected to a photonic crystal environment with multiple bands, our studies reveal that, owing to the presence of two or more bound states, the evolution trajectory of the system will converge to a toric curve of a paraboloid in the Bloch space and the phenomena of periodic or quasi-periodic oscillations could exhibit. While the equation of the parabolic curve is fully determined by the initial values of the state vector in the Bloch space, our results reveal that the scope of the evolution trajectory inside the toric curve is related to the spectral density of the reservoir and their quantified relation is distinctly characterized. Finally, the asymptotic dynamics of the correlations of a two-qubit system is discussed when it is subjected locally to the non-Markovian dissipative process.
We describe an analytically solvable model of quantum decoherence in a nonequilibrium environment. The model considers the effect of a bath driven from equilibrium by, for example, an ultrafast excitation of a quantum chromophore. The nonequilibrium response of the environment is represented by a nonstationary random function corresponding to the fluctuating transition frequency between two quantum states coupled to the surroundings. The nonstationary random function is characterized by a Fourier series with the phase of each term starting initially with a definite value across the ensemble but undergoing random diffusion with time. The decay of the off-diagonal density matrix element is shown to depend significantly on the particular pattern of initial phases of the terms in the Fourier series, or equivalently, the initial phases of bath modes coupled to the quantum subsystem. This suggests the possibility of control of quantum decoherence by the detailed properties of an environment that is driven from thermal equilibrium.
Based on a system-reservoir nonlinear coupling model, where the associated bath is externally driven by a fluctuating force, we present a microscopic approach to quantum state-dependent diffusion and multiplicative noises in terms of a quantum (Markovian) Langevin equation in overdamped limit when the associated bath is in nonequilibrium state. We then explore the possibility of observing a quantum current when the bath is modulated by white noise, the phenomena which is absent in the classical regime.