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The Journal of Chemical Physics

Phase induced current in presence of nonequilibrium bath: A quantum approach

Satyabrata Bhattacharya, Pinaki Chaudhury, Sudip Chattopadhyay, Jyotipratim Ray Chaudhuri

Published Sep 25, 2008• 4 citations
Publisher

Abstract

Based on a system-reservoir nonlinear coupling model, where the associated bath is externally driven by a fluctuating force, we present a microscopic approach to quantum state-dependent diffusion and multiplicative noises in terms of a quantum (Markovian) Langevin equation in overdamped limit when the associated bath is in nonequilibrium state. We then explore the possibility of observing a quantum current when the bath is modulated by white noise, the phenomena which is absent in the classical regime.

DOI
10.1063/1.2981053

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Based on a system-reservoir nonlinear coupling model, where the associated bath is externally driven by a fluctuating force, we present a microscopic approach to quantum state-dependent diffusion and multiplicative noises in terms of a quantum (Markovian) Langevin equation in overdamped limit when the associated bath is in nonequilibrium state. We then explore the possibility of observing a quantum current when the bath is modulated by white noise, the phenomena which is absent in the classical regime.
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We consider a microscopic model of an inhomogeneous environment where an arbitrary quantum system is locally coupled to a harmonic bath via a finite-range interaction. We show that in the overdamped regime the position distribution obeys a classical Kramers-Moyal equation that involves an infinite number of higher-order derivatives, implying that the finite bath correlation length leads to non-Gaussian Markovian noise. We analytically solve the equation for a harmonically bound particle and analyze its non-Gaussian diffusion as well as its steady-state properties.
We analyze the phase diffusion, quantum fluctuations and their spectral features of a one-dimensional Bose-Josephson junction (BJJ) nonlinearly coupled to a bosonic heat bath. The phase diffusion is considered by taking into account of random modulations of the BJJ modes causing a phase loss of initial coherence between the ground and excited states, whereby the frequency modulation is incorporated in the system-reservoir Hamiltonian by an interaction term linear in bath operators but nonlinear in system (BJJ) operators. We examine the dependence of the phase diffusion coefficient on the on-site interaction and temperature in the zero- and π-phase modes and demonstrate its phase transition-like behavior between the Josephson oscillation and the macroscopic quantum self-trapping (MQST) regimes in the π-phase mode. Based on the thermal canonical Wigner distribution, which is the equilibrium solution of the associated quantum Langevin equation for phase, coherence factor is calculated to study phase diffusion for the zero- and π-phase modes. We investigate the quantum fluctuations of the relative phase and population imbalance in terms of fluctuation spectra which capture an interesting shift in Josephson frequency induced by frequency fluctuation due to nonlinear system-reservoir coupling, as well as the on-site interaction-induced splitting in the weak dissipative regime.
We explore the noise-induced barrier crossing dynamics of a Brownian particle in the high temperature quantum regime under large damping. We assume the associated heat bath not to be in thermal equilibrium; it is rather driven by an externally applied random force which exposes the system particles to a nonequilibrium environment. We propose a system + reservoir model to study the stochastic Langevin dynamics. We also construct the corresponding Fokker–Planck equation in the said regime and solve it to explore the bistable kinetics. We investigate the role of different parameters in shaping the nature of such a bistable kinetics in detail and hence allowing one to get some insight into the very complicated dynamics of quantum dissipative system(s). Finally, we analyze the semiclassical rate vis-a-vis the classical analog.
We address the issue of a system that has been tacitly made thermodynamically open by externally driving the associated heat bath in an attempt to gain better insight regarding many physical situations that are akin to this problem. This work embodies the study of the quantum effects in the rate of decay from a metastable state of a Brownian particle which is in contact with a correlated noise-driven bath. We do this by initiating from a suitable system-reservoir model to derive the operator-valued Langevin equation. This further leads us to the corresponding c-number analog that includes quantum effects in leading order. Suitable mathematical treatment culminates in the quantum Fokker-Planck equation, the solution to which yields the rate expression. Finally, we put this to thorough numerical analysis.
Abstract The very notion of a current fluctuation is problematic in the quantum context. We study that problem in the context of nonequilibrium statistical mechanics, both in a microscopic setup and in a Markovian model. Our answer is based on a rigorous result that relates the weak coupling limit of fluctuations of reservoir observables under a global unitary evolution with the statistics of the so-called quantum trajectories. These quantum trajectories are frequently considered in the context of quantum optics, but they remain useful for more general nonequilibrium systems. In contrast with the approaches found in the literature, we do not assume that the system is continuously monitored. Instead, our starting point is a relatively realistic unitary dynamics of the full system