This thesis reports an optical dipole trap for atomic calcium. The dipole trap is loaded from a magneto-optical trap (MOT) of calcium atoms cooled near the Doppler limit (~1 mK). The dipole trap is formed by a large-frame argon ion laser focused to 20 microns into the center of the MOT. This laser runs single-line at 488 nm with a maximum power of 10.6 watts. These parameters result in a trap of 125 mK for calcium atoms in the 4s3d 1D2 state. The 488 nm light also photo-ionizes the trapped atoms due to a near-resonant transition to the 4s4f 1F3 level. These ions leave the trap and are detected to determine the trap decay rate. By measuring this decay rate as a function of 488 nm intensity, we determine the 1F3 photo-ionization cross section at this wavelength to be approximately 230 Mb.
We present studies of resonance-enhanced photoionization for isotope-selective loading of
Ca+ into a Paul trap. The ${4s}^{2}{}^{1}{S}_{0}\ensuremath{\leftrightarrow}4s4p{}^{1}{P}_{1}$ transition of neutral calcium is driven by a 423 nm laser and the atoms are photoionized by a second laser at 389 nm. Isotope selectivity is achieved by using crossed atomic and laser beams to reduce the Doppler width significantly below the isotope shifts in the 423 nm transition. The loading rate of ions into the trap is studied under a range of experimental parameters for the abundant isotope
40Ca+. Using the fluorescence of the atomic beam at 423 nm as a measure of the Ca number density, we estimate a lower limit for the absolute photoionization cross section of 170(60) Mb. We achieve loading and laser cooling of all the naturally occurring isotopes, without the need for enriched sources. Laser heating/cooling is observed to enhance the isotope selectivity. In the case of the rare species
43Ca+ and
46Ca+, which have not previously been laser cooled, the loading is not fully isotope selective, but we show that pure crystals of
43Ca+ may nevertheless be obtained. We find that for loading
40Ca+ the 389 nm laser may be replaced by an incoherent source.
We report on a system for atomic beam deceleration and magneto-optical trapping of calcium atoms that uses the 1S0–1P1 transition, in which a single laser is used to trap and slow the atoms. The slower laser beam is focused near the magneto-optical trap’s center, which has a waist size much smaller than the atomic cloud such that its influence on the trapped atoms is greatly reduced. We also investigate the theoretical possibility of cooling by use of a two-photon (4s2)1S0–(4s5s)1S0 transition. Excitation near resonance with the 1P1 level results in an equilibrium temperature seven times smaller than the Doppler limit of the 1S0–1P1 transition.
We demonstrate an efficient scheme for continuous trap loading based upon spatially selective optical pumping. We discuss the case of
1S0 calcium atoms in an optical dipole trap (ODT), however, similar strategies should be applicable to a wide range of atomic species, which do not permit efficient conventional trap loading. Our starting point is a moderately cold $(\ensuremath{\approx}300\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{K})$ and dense $(\ensuremath{\approx}9\ifmmode\times\else\texttimes\fi{}{10}^{9}\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3})$ reservoir of metastable
3P2 atoms in a magneto-optic trap (triplet MOT). A focused
532nm laser beam produces a strongly elongated optical potential for
1S0 atoms with up to $350\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{K}$ well depth. A weak focused laser beam at
430nm, carefully superimposed upon the ODT beam, selectively pumps the
3P2 atoms inside the capture volume to the singlet state, where they are confined by the ODT. The triplet MOT perpetually refills the capture volume with
3P2 atoms, thus providing a continuous stream of cold atoms into the ODT at a rate of ${10}^{7}\phantom{\rule{0.3em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$. Limited by evaporation loss, in
200ms we typically load $5\ifmmode\times\else\texttimes\fi{}{10}^{5}$ atoms with $3.5\ifmmode\times\else\texttimes\fi{}{10}^{10}\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$ peak density and axial and radial temperatures of 300 and $85\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{K}$, respectively. After terminating the loading we observe evaporation during
50ms, typically leaving us with
105 atoms with nearly equal radial and axial temperatures close to $40\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{K}$ and a peak density of $5\ifmmode\times\else\texttimes\fi{}{10}^{11}\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$. A simple model is presented, which identifies the relevant physical mechanisms of the loading and decay dynamics. We point out that a comparable scheme could be employed to load a dipole trap with
3P0 atoms.
We report the measurement of the absolute photoionization cross section for the
6P3/2 state of cesium. Cross sections were determined by measuring the photoionization rate of cesium atoms confined in a magneto-optical trap. The photoionization rate was measured by monitoring the decay of trap fluorescence during exposure to ionizing laser radiation. The measurements were made in the wavelength range 457.9 to 501.7 nm using several lines from an Ar-ion laser. Our results are compared to other experimental measurements as well as to existing theories.