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arXiv:physics/0003109

The ZEKE-effect in cold Rydberg gases

Dutta, S. K., D. Feldbaum, Georg A. Raithel

Published Mar 31, 2000• 2 citations
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Abstract

Cold, dense Rydberg gases produced in a cold-atom trap are investigated using spectroscopic methods and time-resolved electron counting. On the discrete Rydberg resonances we observe large trap losses and long lasting electron emission from the Rydberg gas (>30ms). Our observations are explained by quasi-elastic l-mixing collisions between Rydberg atoms and slow electrons that lead to the population of long-lived high-angular-momentum Rydberg states. These atoms thermally ionize slowly and with large probabilities, leading to the observed effects.

DOI
10.48550/arxiv.physics/0003109

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•Jan 1, 2003•0 citations
Cold, dense Rydberg gases produced in a cold-atom trap are investigated using spectroscopic methods and time-resolved electron counting. On the discrete Rydberg resonances we observe large trap losses and long lasting electron emission from the Rydberg gas (>30ms). Our observations are explained by quasi-elastic l-mixing collisions between Rydberg atoms and slow electrons that lead to the population of long-lived high-angular-momentum Rydberg states. These atoms thermally ionize slowly and with large probabilities, leading to the observed effects.
Cold, dense Rydberg gases produced in a cold-atom trap are investigated using spectroscopic methods and time-resolved electron counting. Optical excitation on the discrete Rydberg resonances reveals long-lasting electron emission from the Rydberg gas ( >20 ms). Our observations are explained by lm-mixing collisions between Rydberg atoms and slow electrons that lead to the population of long-lived high-angular-momentum Rydberg states. These atoms thermally ionize slowly and with large probabilities.
There is considerable interest in the dynamics of ultracold plasmas and ultracold Rydberg gases. Ultracold plasmas are typically formed by photo-excitation of ultracold atoms to an energy region near (both above and below) an ionization threshold. Excitation to bound, highly-excited Rydberg states can lead to formation of a plasma via several processes, including collisions between Rydberg atoms. Three-body recombination in an ultracold plasma can also result in the production of ultracold Rydberg atoms. Understanding the dynamics of ultracold Rydberg gases is therefore important for understanding the dynamics of ultracold plasmas. In this dissertation, we have investigated the formation and survival of a particular class of Rydberg atoms. These atoms are known as ZEKE state Rydberg atoms, where the term ZEKE is derived from "Zero Kinetic Energy." ZEKE Rydberg states are high angular momentum and high angular momentum projection excited states which can be formed by laser excitation in the presence of electric fields. Without the electric fields, these states would be optically dark. We have investigated ZEKE Rydberg states in ultracold argon in an energy region just below the second ionization threshold of the atoms in our magneto-optical trap. Here, low angular momentum states decay very quickly (< 1 ns) by auto-ionization through a core spin flip due to the Rydberg electron-core interaction. This interaction has been significantly reduced due to the dilution of low l and m states as a result of l and m mixing during excitation. Hence, ZEKE Rydberg states live orders of magnitude longer than low angular momentum states. We are reporting on our experimental investigation of these states in the ultracold regime and prospects for future studies in which external control of these states may be used to control ultracold plasma dynamics.
Using state-selective field ionization, the state distributions of Rydberg atoms in cold Rydberg gases are measured for various initially excited Rydberg levels, populations, and evolution times. We provide direct experimental evidence for lll-changing collisions that we previously observed indirectly [S. K. Dutta, D. Feldbaum, A. Walz-Flannigan, J. R. Guest, and G. Raithel, Phys. Rev. Lett. 86, 3993 (2001)]. We also observe nnn-mixing and find that its effects are largely in agreement with recent theoretical work on nnn-changing collisions between electrons and Rydberg atoms, thus enabling an estimation of the electron temperature. Unexpectedly large populations of atoms are found in states with principal quantum numbers much lower than that of the initially excited atoms. We explain this observation by collisions between high-lll Rydberg atoms, which are highly polar and can collide due to static electric-dipole forces between them.
We have observed the evolution of cold Rydberg gases and ultracold plasmas in an environment that allows for the control of interactions of the blackbody radiation temperature from 4K to 300K. The work in this thesis describes the influence of initial densities, populations, excitation state, evolution time and thermal background temperature on the evolution of cold Rydberg gases as well as directly excited ultracold plasmas. With some initial ionization, cold-Rydberg-atom gases easily develop a positive space charge that traps electrons for times on the order of tens of mus. This acts as a catalyst for electron-Rydberg atom collisions, increasing the collision probabilities by orders of magnitude and profoundly altering the final state of the Rydberg gas. Using state-selective field ionization, we have provided direct proof that these collisions cause changes in l-states, and we have seen the first experimental evidence that they also lead to inelastic n-changing collisions, as predicted by theory. We have also found evidence for Rydberg-Rydberg collisions, enabled by the attractive electric-dipole forces between atoms in high-l states and possibly by van-der-Waal's interactions at very high-n . Thermal interactions are seen to influence the formation of a plasma from a cold Rydberg gas. Plasmas form more easily in the presence of a 300K radiation field than at 4K, due to the contribution of thermal ionization to the plasma formation. The background temperature also appears to affect the electron temperature in both the directly excited plasma and the plasma spontaneously formed from a cold Rydberg gas. In Rydberg atom gases that have undergone partial ionization, electron temperatures were estimated using the dependence of n-changing collisions on the electron temperature.
Dense samples of cold Rydberg atoms have previously been observed to spontaneously evolve to a plasma, despite the fact that each atom may be bound by as much as $100\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1}$. Initially, ionization is caused by blackbody photoionization and Rydberg-Rydberg collisions. After the first electrons leave the interaction region, the net positive charge traps subsequent electrons. As a result, rapid ionization starts to occur after $1\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{s}$ caused by electron-Rydberg collisions. The resulting cold plasma expands slowly and persists for tens of microseconds. While the initial report on this process identified the key issues described above, it failed to resolve one key aspect of the evolution process. Specifically, redistribution of population to Rydberg states other than the one initially populated was not observed, a necessary mechanism to maintain the energy balance in the system. Here we report new and expanded observations showing such redistribution and confirming theoretical predictions concerning the evolution to a plasma. These measurements also indicate that, for high nnn states of purely cold Rydberg samples, the initial ionization process which leads to electron trapping is one involving the interactions between Rydberg atoms.
We have studied the development of gases of ultra-cold Rydberg atoms in Magneto Optic Traps, and discovered that such gases exhibit a range of density-dependent phenomena. In particular, we have found that at the densities of ∼ 10 7 cm -3 the Rydberg atoms spontaneously evolve into long-lived high angular momentum states. These states slowly decay due to microwave background radiation over tens of milliseconds. We have numerically simulated the effects leading to such behavior, and investigated numerically the l- and n-mixing collisions of Rydberg atoms with electrons in the range of 10 meV. These calculations show that the l- and n-mixing cross-sections follow the n 5 scaling law, expected from simple Stark map considerations, but also depend on the velocities of the colliding electrons, reflecting the adiabaticity of the atom-electron interactions. We have developed a novel technique of measuring the electric fields inside plasmas by using Rydberg excitation spectroscopy of embedded atoms, based on the disappearance of regions of zero oscillator strength in the presence of such fields. We have applied this technique to study the evolution of ultra-cold non-neutral plasmas excited from the MOT, and have found that it expands over 1 mus. We have simulated such an expansion by considering only Coulomb repulsion between the constituent ions, and have found that such a model is consistent with the experimental observations.