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arXiv:cond-mat/9911068 · Physical Review Letters

Anomalous Magnetic Splitting of the Kondo Resonance

Joel E. Moore, Xiao-Gang Wen

Published Aug 21, 2000• 95 citations
arXivHTMLPDF

Abstract

The splitting of the Kondo resonance in the density of states of an Anderson impurity in a finite magnetic field is calculated from the exact Bethe-ansatz solution. The result gives an estimate of the electron spectral function for a nonzero magnetic field and the Kondo temperature, with consequences for transport experiments on quantum dots in the Kondo regime. The strong correlations of the Kondo ground state cause a significant low-temperature reduction of the peak splitting. Explicit formulas are found for the shift and broadening of the Kondo peaks. A likely cause of the problems of large- N approaches to spin- 1 / 2 impurities at finite magnetic field is suggested.

DOI
10.1103/physrevlett.85.1722

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The splitting of the Kondo resonance in the density of states of an Anderson impurity in a finite magnetic field is calculated from the exact Bethe-ansatz solution. The result gives an estimate of the electron spectral function for a nonzero magnetic field and the Kondo temperature, with consequences for transport experiments on quantum dots in the Kondo regime. The strong correlations of the Kondo ground state cause a significant low-temperature reduction of the peak splitting. Explicit formulas are found for the shift and broadening of the Kondo peaks. A likely cause of the problems of large- N approaches to spin- 1 / 2 impurities at finite magnetic field is suggested.
This paper is a corrected version of Phys. Rev. B 95, 165404 (2017), which we have retracted because it contained a trivial but fatal sign error that lead to incorrect conclusions. We extend a recently developed Fermi liquid (FL) theory for the asymmetric single-impurity Anderson model [C. Mora et al., Phys. Rev. B 92, 075120 (2015)] to the case of an arbitrary local magnetic field. To describe the system's low-lying quasiparticle excitations for arbitrary values of the bare Hamiltonian's model parameters, we construct an effective low-energy FL Hamiltonian whose FL parameters are expressed in terms of the local level's spin-dependent ground-state occupations and their derivatives with respect to level energy and local magnetic field. These quantities are calculable with excellent accuracy from the Bethe ansatz solution of the Anderson model. Applying this effective model to a quantum dot in a nonequilibrium setting, we obtain exact results for the curvature of the spectral function, cA{c}_{A}cA​, describing its leading $\ensuremath{\sim}{\ensuremath{\varepsilon}}^{2}$ term, and the transport coefficients cV{c}_{V}cV​ and cT{c}_{T}cT​, describing the leading $\ensuremath{\sim}{V}^{2}$ and $\ensuremath{\sim}{T}^{2}$ terms in the nonlinear differential conductance. A sign change in cA{c}_{A}cA​ or cV{c}_{V}cV​ is indicative of a change from a local maximum to a local minimum in the spectral function or nonlinear conductance, respectively, as is expected to occur when an increasing magnetic field causes the Kondo resonance to split into two subpeaks. We find that the fields BA{B}_{A}BA​, BT{B}_{T}BT​, and BV{B}_{V}BV​ at which cA{c}_{A}cA​, cT{c}_{T}cT​, and cV{c}_{V}cV​ change sign, respectively, are all of order TK{T}_{K}TK​, as expected, with BA=BT=BV=0.75073TK{B}_{A}={B}_{T}={B}_{V}=0.75073{T}_{K}BA​=BT​=BV​=0.75073TK​ in the Kondo limit.
By using the full density matrix approach to spectral functions within the numerical renormalization group method, we present a detailed study of the magnetic field induced splittings in the spin-resolved and the total spectral densities of a Kondo correlated quantum dot described by the single level Anderson impurity model. The universal scaling of the splittings with magnetic field is examined by varying the Kondo scale either by a change of local level position at a fixed tunnel coupling or by a change of the tunnel coupling at a fixed level position. We find that the Kondo-peak splitting $\ensuremath{\Delta}/{T}_{K}$ in the spin-resolved spectral function always scales perfectly for magnetic fields B<8TKB<8{T}_{K}B<8TK​ in either of the two TK{T}_{K}TK​-adjusted paths. Scaling is destroyed for fields B>10TKB>10{T}_{K}B>10TK​. On the other hand, the Kondo peak splitting $\ensuremath{\delta}/{T}_{K}$ in the total spectral function does slightly deviate from the conventional scaling theory in whole magnetic field window along the coupling-varying path. Furthermore, we show the scaling analysis suitable for all field windows within the Kondo regime and two specific fitting scaling curves are given from which certain detailed features at low field are derived. In addition, the scaling dimensionless quantity $\ensuremath{\Delta}/2B$ and $\ensuremath{\delta}/2B$ are also studied and they can reach and exceed 1 in the large magnetic field region, in agreement with a recent experiment [T. M. Liu et al., Phys. Rev. Lett. 103, 026803 (2009)].
In a recent work, Zhang and coworkers [Phys. Rev. B 82, 075111 (2010)] studied the Zeeman splitting of the Kondo resonance for the single impurity Anderson model in a finite magnetic field BBB with the numerical renormalization group (NRG) method. They report a discrepancy between the position of the Kondo resonance in the total spectral function and the position in the spin-resolved spectral function at large magnetic fields. Additionally, the position of the Kondo maximum exceeded the Zeeman energy for $B/{T}_{K}\ensuremath{\gtrsim}5\ensuremath{-}10$, where TK{T}_{K}TK​ is the low-energy Kondo scale of the model. In this comment, we argue that both these findings are a result of the specific choice of NRG parameter values. However, we reproduce the crossover in the splitting from Kondo-like behavior to a nonuniversal splitting larger than the Zeeman energy, but this crossover occurs at much larger fields of the order of the charge scale.
We study non-equilibrium electron transport through a quantum impurity coupled to metallic leads using the equation of motion technique at finite temperature T . Assuming that the interactions are taking place solely in the impurity and focusing on the infinite Hubbard limit, we compute the out of equilibrium density of states and the differential conductance G2(T, V ) in order to test several scaling laws. We find that G2(T, V )/G2(T, 0) is a universal function of both eV/TK and T/TK, TK being the Kondo temperature. The effect of an in-plane magnetic field on the splitting of the zero bias anomaly in the differential conductance is also analyzed. For a Zeeman splitting , the computed differential conductance peak splitting depends only on /TK, and for large fields approaches the value of 2. Besides studying the traditional two leads setup, we also consider other configurations that mimic recent experiments, namely, an impurity embedded in a mesoscopic wire and the presence of a third weakly coupled lead. In these cases, a double peak structure of the Kondo resonance is clearly obtained in the differential conductance while the amplitude of the highest peak is shown to decrease as ln(eV/TK). Several features of these results are in qualitative agreement with recent experimental observations reported on quantum dots.
Using different techniques, and Fermi-liquid relationships, we calculate the variation with the applied magnetic field (up to second order) of the zero-temperature equilibrium conductance through a quantum dot described by the impurity Anderson model. We focus on the strong-coupling limit $U\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}$, where UUU is the Coulomb repulsion and $\mathrm{\ensuremath{\Delta}}$ is half the resonant-level width, and consider several values of the dot level energy Ed{E}_{d}Ed​, ranging from the Kondo regime ${\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}$ to the intermediate-valence regime ${\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\sim}\mathrm{\ensuremath{\Delta}}$, where ${\ensuremath{\epsilon}}_{F}$ is the Fermi energy. We have mainly used the density-matrix renormalization group (DMRG) and the numerical renormalization group (NRG) combined with renormalized perturbation theory (RPT). Results for the dot occupancy and magnetic susceptibility from the DMRG and NRG+RPT\mathrm{NRG}+\mathrm{RPT}NRG+RPT are compared with the corresponding Bethe ansatz results for $U\ensuremath{\rightarrow}\ensuremath{\infty}$, showing an excellent agreement once Ed{E}_{d}Ed​ is renormalized by a constant Haldane shift. For $U<3\mathrm{\ensuremath{\Delta}}$ a simple perturbative approach in UUU agrees very well with the other methods. The conductance decreases with the applied magnetic field for dot occupancies ${n}_{d}\ensuremath{\sim}1$ and increases for ${n}_{d}\ensuremath{\sim}0.5$ or ${n}_{d}\ensuremath{\sim}1.5$ regardless of the value of UUU. We also relate the energy scale for the magnetic-field dependence of the conductance with the width of the low-energy peak in the spectral density of the dot.