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arXiv:1509.05948 · Physical Review B

Scaling of conductance through quantum dots with magnetic field

Ignacio J. Hamad, C. J. Gazza, J. A. Andrade, Armando A. Aligia, Pablo S. Cornaglia, P. Roura-Bas

Published Nov 9, 2015• 10 citations
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Abstract

Using different techniques, and Fermi-liquid relationships, we calculate the variation with the applied magnetic field (up to second order) of the zero-temperature equilibrium conductance through a quantum dot described by the impurity Anderson model. We focus on the strong-coupling limit $U\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}$, where $U$ is the Coulomb repulsion and $\mathrm{\ensuremath{\Delta}}$ is half the resonant-level width, and consider several values of the dot level energy ${E}_{d}$, ranging from the Kondo regime ${\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}$ to the intermediate-valence regime ${\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\sim}\mathrm{\ensuremath{\Delta}}$, where ${\ensuremath{\epsilon}}_{F}$ is the Fermi energy. We have mainly used the density-matrix renormalization group (DMRG) and the numerical renormalization group (NRG) combined with renormalized perturbation theory (RPT). Results for the dot occupancy and magnetic susceptibility from the DMRG and $\mathrm{NRG}+\mathrm{RPT}$ are compared with the corresponding Bethe ansatz results for $U\ensuremath{\rightarrow}\ensuremath{\infty}$, showing an excellent agreement once ${E}_{d}$ is renormalized by a constant Haldane shift. For $U<3\mathrm{\ensuremath{\Delta}}$ a simple perturbative approach in $U$ agrees very well with the other methods. The conductance decreases with the applied magnetic field for dot occupancies ${n}_{d}\ensuremath{\sim}1$ and increases for ${n}_{d}\ensuremath{\sim}0.5$ or ${n}_{d}\ensuremath{\sim}1.5$ regardless of the value of $U$. We also relate the energy scale for the magnetic-field dependence of the conductance with the width of the low-energy peak in the spectral density of the dot.

DOI
10.1103/physrevb.92.195113

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Using different techniques, and Fermi-liquid relationships, we calculate the variation with the applied magnetic field (up to second order) of the zero-temperature equilibrium conductance through a quantum dot described by the impurity Anderson model. We focus on the strong-coupling limit U\ensuremath≫\ensuremathΔU\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}U\ensuremath≫\ensuremathΔ, where UUU is the Coulomb repulsion and \ensuremathΔ\mathrm{\ensuremath{\Delta}}\ensuremathΔ is half the resonant-level width, and consider several values of the dot level energy Ed{E}_{d}Ed​, ranging from the Kondo regime \ensuremathϵF\ensuremath−Ed\ensuremath≫\ensuremathΔ{\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\gg}\mathrm{\ensuremath{\Delta}}\ensuremathϵF​\ensuremath−Ed​\ensuremath≫\ensuremathΔ to the intermediate-valence regime \ensuremathϵF\ensuremath−Ed\ensuremath∼\ensuremathΔ{\ensuremath{\epsilon}}_{F}\ensuremath{-}{E}_{d}\ensuremath{\sim}\mathrm{\ensuremath{\Delta}}\ensuremathϵF​\ensuremath−Ed​\ensuremath∼\ensuremathΔ, where \ensuremathϵF{\ensuremath{\epsilon}}_{F}\ensuremathϵF​ is the Fermi energy. We have mainly used the density-matrix renormalization group (DMRG) and the numerical renormalization group (NRG) combined with renormalized perturbation theory (RPT). Results for the dot occupancy and magnetic susceptibility from the DMRG and NRG+RPT\mathrm{NRG}+\mathrm{RPT}NRG+RPT are compared with the corresponding Bethe ansatz results for U\ensuremath→\ensuremath∞U\ensuremath{\rightarrow}\ensuremath{\infty}U\ensuremath→\ensuremath∞, showing an excellent agreement once Ed{E}_{d}Ed​ is renormalized by a constant Haldane shift. For U<3\ensuremathΔU<3\mathrm{\ensuremath{\Delta}}U<3\ensuremathΔ a simple perturbative approach in UUU agrees very well with the other methods. The conductance decreases with the applied magnetic field for dot occupancies nd\ensuremath∼1{n}_{d}\ensuremath{\sim}1nd​\ensuremath∼1 and increases for nd\ensuremath∼0.5{n}_{d}\ensuremath{\sim}0.5nd​\ensuremath∼0.5 or nd\ensuremath∼1.5{n}_{d}\ensuremath{\sim}1.5nd​\ensuremath∼1.5 regardless of the value of UUU. We also relate the energy scale for the magnetic-field dependence of the conductance with the width of the low-energy peak in the spectral density of the dot.
In a recent work [Merker, Kirchner, Mu\~noz, and Costi, Phys. Rev. B 87, 165132 (2013)], the authors compared the results of numerical renormalization group (NRG) and a perturbative approach for the dependence on temperature TTT and magnetic field BBB of the conductance through a quantum dot described by the impurity Anderson model, for small TTT and BBB. We show that the equation used to extract the dependence on BBB from NRG results is incorrect out of the particle-hole symmetric case. As a consequence, in the Kondo regime, the correct NRG results have a weaker dependence on BBB and the disagreement between both approaches increases.
Single-particle dynamics of the Anderson impurity model in the presence of a magnetic field H are considered, using a recently developed local moment approach that encompasses all energy scales, field and interaction strengths. For strong coupling in particular, the Kondo scaling regime is recovered. Here the frequency (ω/ω K ) and field ( H /ω K ) dependence of the resultant universal scaling spectrum is obtained in large part analytically, and the field-induced destruction of the Kondo resonance investigated. The scaling spectrum is found to exhibit the slow logarithmic tails recently shown to dominate the zero-field scaling spectrum. At the opposite extreme of the Fermi level, it gives asymptotically exact agreement with results for statics known from the Bethe ansatz. Good agreement is also found with the frequency and field-dependence of recent numerical renormalization group calculations. Differential conductance experiments on quantum dots in the presence of a magnetic field are likewise considered, and appear to be well accounted for by the theory. Some new exact results for the problem are also established.
We generalize Nozi\`eres' Fermi-liquid theory for the low-energy behavior of the Kondo model to that of the single-impurity Anderson model. In addition to the electrons' phase shift at the Fermi energy, the low-energy Fermi-liquid theory is characterized by four Fermi-liquid parameters: the two given by Nozi\`eres that enter to first order in the excitation energy, and two additional ones that enter to second order and are needed away from particle-hole symmetry. We express all four parameters in terms of zero-temperature physical observables, namely the local charge and spin susceptibilities and their derivatives with respect to the local level position. We determine these in terms of the bare parameters of the Anderson model using Bethe ansatz and numerical renormalization group (NRG) calculations. Our low-energy Fermi-liquid theory applies throughout the crossover from the strong-coupling Kondo regime via the mixed-valence regime to the empty-orbital regime. From the Fermi-liquid theory, we determine the conductance through a quantum dot symmetrically coupled to two leads in the regime of small magnetic field, low temperature, and small bias voltage, and compute the coefficients of the $\ensuremath{\sim}{B}^{2}, \ensuremath{\sim}{T}^{2}$, and $\ensuremath{\sim}{V}^{2}$ terms exactly in terms of the Fermi-liquid parameters. The coefficients of T2,V2{T}^{2}, {V}^{2}T2,V2, and B2{B}^{2}B2 are found to change sign during the Kondo to empty-orbital crossover. The crossover becomes universal in the limit that the local interaction is much larger than the level width. For completeness, we also compute the shot noise and discuss the resulting Fano factor.
This paper is a corrected version of Phys. Rev. B 95, 165404 (2017), which we have retracted because it contained a trivial but fatal sign error that lead to incorrect conclusions. We extend a recently developed Fermi liquid (FL) theory for the asymmetric single-impurity Anderson model [C. Mora et al., Phys. Rev. B 92, 075120 (2015)] to the case of an arbitrary local magnetic field. To describe the system's low-lying quasiparticle excitations for arbitrary values of the bare Hamiltonian's model parameters, we construct an effective low-energy FL Hamiltonian whose FL parameters are expressed in terms of the local level's spin-dependent ground-state occupations and their derivatives with respect to level energy and local magnetic field. These quantities are calculable with excellent accuracy from the Bethe ansatz solution of the Anderson model. Applying this effective model to a quantum dot in a nonequilibrium setting, we obtain exact results for the curvature of the spectral function, cA{c}_{A}cA​, describing its leading $\ensuremath{\sim}{\ensuremath{\varepsilon}}^{2}$ term, and the transport coefficients cV{c}_{V}cV​ and cT{c}_{T}cT​, describing the leading $\ensuremath{\sim}{V}^{2}$ and $\ensuremath{\sim}{T}^{2}$ terms in the nonlinear differential conductance. A sign change in cA{c}_{A}cA​ or cV{c}_{V}cV​ is indicative of a change from a local maximum to a local minimum in the spectral function or nonlinear conductance, respectively, as is expected to occur when an increasing magnetic field causes the Kondo resonance to split into two subpeaks. We find that the fields BA{B}_{A}BA​, BT{B}_{T}BT​, and BV{B}_{V}BV​ at which cA{c}_{A}cA​, cT{c}_{T}cT​, and cV{c}_{V}cV​ change sign, respectively, are all of order TK{T}_{K}TK​, as expected, with BA=BT=BV=0.75073TK{B}_{A}={B}_{T}={B}_{V}=0.75073{T}_{K}BA​=BT​=BV​=0.75073TK​ in the Kondo limit.
We study the single-impurity Anderson model out of equilibrium under the influence of a bias voltage ϕ and a magnetic field B . We investigate the interplay between the shift ( ) of the Kondo peak in the spin-resolved density of states (DOS) and the one ( ) of the conductance anomaly. In agreement with experiments and previous theoretical calculations we find that, while the latter displays a rather linear behavior with an almost constant slope as a function of B down to the Kondo scale, the DOS shift first features a slower increase reaching the same behavior as only for . Our auxiliary master equation approach yields highly accurate nonequilibrium results for the DOS and for the conductance all the way from within the Kondo up to the charge fluctuation regime, showing excellent agreement with a recently introduced scheme based on a combination of numerical renormalization group with time-dependent density matrix renormalization group.
We present a comprehensive Fermi liquid description for thermoelectric transport and current noise, applicable to multilevel quantum dots (QD) and magnetic alloys (MA) without electron-hole or time-reversal symmetry. Our formulation for the low-energy transport is based on an Anderson model with NNN discrete impurity levels, and is asymptotically exact at low energies, up to the next-leading order terms in power expansions with respect to temperature TTT and bias voltage eVeVeV. The expansion coefficients can be expressed in terms of the Fermi liquid parameters, which include the three-body correlation functions defined with respect to the equilibrium ground state in addition to the linear susceptibilities and the occupation number Nd{N}_{d}^{}Nd​ of impurity electrons. We apply this formulation to the SU(N)\mathrm{SU}(N)SU(N) symmetric QD and MA, and calculate the correlation functions for N=4N=4N=4 and 6, using numerical renormalization group approach. The three-body correlations are shown to be determined by a single parameter over a wide range of electron fillings $1\ensuremath{\lesssim}{N}_{d}^{}\ensuremath{\lesssim}N\ensuremath{-}1$ for strong Coulomb interactions UUU, and they also exhibit the plateau structures due to the SU(N)\mathrm{SU}(N)SU(N) Kondo effects at integer values of Nd{N}_{d}^{}Nd​. We find that the Lorenz number $L=\ensuremath{\kappa}/(T\ensuremath{\sigma})$ for QD and MA, defined as the ratio of the thermal conductivity $\ensuremath{\kappa}$ to the electrical conductivity $\ensuremath{\sigma}$, deviates from the universal Wiedemann-Franz value ${\ensuremath{\pi}}^{2}/(3{e}^{2})$ as the temperature increases from T=0T=0T=0, showing the T2{T}^{2}T2 dependence, the coefficient for which depends on the three-body correlations away from half filling. Furthermore, we find that the current noise for the SU(4) quantum dots and that for SU(6) show a pronounced difference at the quarter Nd/N=1/4{N}_{d}^{}/N=1/4Nd​/N=1/4 and 3/43/43/4 fillings. In particular, the linear noise for N=4N=4N=4 exhibits a flat peak while the peak for N=6N=6N=6 shows a round shape, reflecting the fact that, at these filling points, the SU(N)\mathrm{SU}(N)SU(N) Kondo effects occur for $N\ensuremath{\equiv}0$ (mod 4), whereas the intermediate-valence fluctuations occur for $N\ensuremath{\equiv}2$ (mod 4). We also demonstrate the role of three-body correlations on the nonlinear current noise and the other transport coefficients.