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arXiv:cond-mat/9806111 · Physical review. B, Condensed matter

Magnetization properties of some quantum spin ladders

Kunj Tandon, Siddhartha Lal, Swapan Kumar Pati, S. Ramasesha, Diptiman Sen

Published Jan 1, 1999• 63 citations
arXivHTMLPDF

Abstract

The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-$1/2$ ladder, and a two-legged spin-$1/2$ ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an $\mathrm{XXZ}$ spin-$1/2$ chain in a magnetic field; the second-order terms give corrections to the $\mathrm{XXZ}$ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.

DOI
10.1103/physrevb.59.396

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The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-1/21/21/2 ladder, and a two-legged spin-1/21/21/2 ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an XXZ\mathrm{XXZ}XXZ spin-1/21/21/2 chain in a magnetic field; the second-order terms give corrections to the XXZ\mathrm{XXZ}XXZ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.
Using the density-matrix renormalization-group technique we investigate the low-energy properties and the magnetization-plateau behavior in a two-leg mixed spin ladder consisting of a spin-1/2 chain coupled with a spin-1 chain. The calculated results show that the system is in the same universality class as the spin-3/2 chain when the interchain coupling is strongly ferromagnetic, but the similarity between the two systems is less clear under other coupling conditions. We have identified two types of magnetization-plateau phases. The calculation of the magnetization distribution on the spin-1/2 and the spin-1 chains on the ladder shows that one plateau phase is related to the partially magnetized valence-bond-solid state, and the other plateau state contains strongly coupled S=1S=1S=1 and s=1/2s=1/2s=1/2 spins on the rung.
Abstract In this paper we consider ladders with two, three, and four coupled Ising spin chains, characterized by interchain and intrachain couplings, to study in detail their magnetic behaviour for different ratios of the interaction constants and different values of magnetic field, by using a transfer matrix method and a complex algorithm, realizing the diagonalization and the differentiation. We have proposed a combined algorithm to realize also the generation of the elements of the transfer matrix for more complicated ladder configurations. The problem of Ising ladders is straightforward with a crossover between a 2D high‐temperature region and a 1D low‐temperature region when the 2D correlation length equals the width. To emphasize the fact that there is no finite magnetization in absence of the magnetic field, we study also analytically this case for the ladder with two coupled Ising chains. In presence of the magnetic field, for very weak magnetic fields (of the order 10−8, in reduced units) the magnetization goes from the value one to the value zero in a narrow interval of nonzero temperatures, where also the susceptibility exhibits a very high peak. This narrow interval, increasing the number of chains, is displaced towards higher temperatures. Also, in the case of interchain antiferromagnetic couplings, the formation of interchain spin pairs becomes clear.
We study the quantum critical behavior in the antiferromagnetic Heisenberg chain and two-leg Heisenberg ladder resulting from the application of an external magnetic field. In each of these systems a finite-temperature crossover line between two different ferromagnetic phases ends with a quantum critical point at zero temperature. Using the bond-mean-field theory, we calculate the field dependence of the magnetization and the mean-field spin bond parameters in both systems. For the Heisenberg chain, we recover the existing exact results and show in addition that the saturation of the zero-temperature magnetization at the field hc=2J{h}_{c}=2Jhc​=2J is accompanied by a quantum phase transition, where the bond parameter vanishes. Here JJJ is the exchange coupling constant along the chain. For the two-leg ladder, we also recover the known results, like the two magnetization plateaus, and show that at the upper critical field, which corresponds to the appearance of the saturation magnetization plateau, the chain and rung spin bond parameters vanish. The identification of the order parameters that govern the field-induced quantum criticality in the systems we study here constitutes an original contribution. Because no long-range order, which breaks symmetry, characterizes the bond order, the latter could be a proposal for the so-called hidden order. We calculate analytically the bond parameters in both systems as functions of the field in the low- and high-field limits at zero temperature. At nonzero temperatures, the calculation of the magnetization and bond parameters is carried out by solving the mean-field equations numerically.
The effect of antiferromagnetic interchain coupling in alternating spin-(1,1/2) chains is studied by means of spin-wave theory and density-matrix renormalization group (DMRG). In particular, two limiting cases are investigated, the two-leg ladder and its two-dimensional (2D) generalization. Results of the ground-state properties like energy, spin gap, magnetizations, and correlation functions are reported for the whole range of the interchain coupling ${J}_{\ensuremath{\perp}}.$ For the 2D case the spin-wave results predict a smooth dimensional crossover from 1D to 2D keeping the ground state always ordered. For the ladder system, the DMRG results show that any ${J}_{\ensuremath{\perp}}>0$ drives the system to a gapped ground state. Furthermore the behavior of the correlation functions closely resemble the uniform spin-1/2 ladder. For ${J}_{\ensuremath{\perp}}$ lower than 0.3, however, the gap behaves quadratically as $\ensuremath{\Delta}\ensuremath{\sim}{0.6J}_{\ensuremath{\perp}}^{2}.$ Finally, it is argued that the behavior of the spin gap for an arbitrary number of mixed coupled spin chains is analogous to that of the uniform spin-1/2 chains.
We study the ground state phase diagram of a frustrated spin-1/2 four-leg tube in an external magnetic field. We explore the parameter space of this model in the regime of all-antiferromagnetic exchange couplings by means of three different approaches: density matrix renormalization group (DMRG), a low-energy effective Hamiltonian (LEH) and a Hartree variational approach (HVA). We find that in the limit of weakly interacting plaquettes, singlet and triplet states play an important role in the formation of magnetization plateaux. We study the transition regions numerically and analytically, and find that they are described, at first order in a strong- coupling expansion, by an XXZ spin-1/2 chain in a magnetic field. These results are consistent with the DMRG and HVA calculations.
We study the field-induced quantum phase transitions (QPT) and the relevant magnetic properties of a spin-1/2 two-leg integrable spin ladder (ISL), of which the system parameters in bridging to the real compounds are determined by setting the extra interactions in the Hamiltonian of the ISL relative to the Heisenberg spin ladder to vanish in the expectation in the ground state (GS). Such an ISL analytically has the correct leading terms of both the critical fields of the two QPT's as in the real strongly-coupled compounds: gμ_BH_{c1}=J_{\perp}-J_{\parallel} and gμ_BH_{c2}=J_{\perp}+2J_{\parallel} in terms of the experimental leg (J_{\parallel}) and rung (J_{\perp}) interactions. The symmetric magnetization inflection point is located at gμ_BH_{IP}=J_{\perp}+J_{\parallel}/2. The magnetizations for the GS and at finite temperatures, as well as the susceptibility, show good agreements in various comparisons with the finite-site exact diagonalization, the transfer-matrix renormalization group numerical result, the perturbation theory, and the compounds (5IAP)_2CuBr_4\cdot 2H_2O, Cu_2(C_5H_{12}N_2)_2Cl_4 and (C_5H_{12}N)_2CuBr_4.