Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:cond-mat/0405274

Quantum phase transitions and magnetization of an integrable spin ladder with new parameters in bridging to real compounds

Zu‐Jian Ying, I. Roditi, Huan-Qiang Zhou

Published May 13, 2004• 0 citations
arXivHTMLPDF

Abstract

We study the field-induced quantum phase transitions (QPT) and the relevant magnetic properties of a spin-1/2 two-leg integrable spin ladder (ISL), of which the system parameters in bridging to the real compounds are determined by setting the extra interactions in the Hamiltonian of the ISL relative to the Heisenberg spin ladder to vanish in the expectation in the ground state (GS). Such an ISL analytically has the correct leading terms of both the critical fields of the two QPT's as in the real strongly-coupled compounds: gμ_BH_{c1}=J_{\perp}-J_{\parallel} and gμ_BH_{c2}=J_{\perp}+2J_{\parallel} in terms of the experimental leg (J_{\parallel}) and rung (J_{\perp}) interactions. The symmetric magnetization inflection point is located at gμ_BH_{IP}=J_{\perp}+J_{\parallel}/2. The magnetizations for the GS and at finite temperatures, as well as the susceptibility, show good agreements in various comparisons with the finite-site exact diagonalization, the transfer-matrix renormalization group numerical result, the perturbation theory, and the compounds (5IAP)_2CuBr_4\cdot 2H_2O, Cu_2(C_5H_{12}N_2)_2Cl_4 and (C_5H_{12}N)_2CuBr_4.

DOI
10.48550/arxiv.cond-mat/0405274

Related papers

Integrable models and quantum spin ladders: comparison between theory and experiment for the strong coupling ladder compounds

Murray T. Batchelor, X. W. Guan, N. Oelkers +1 more

This article considers recent advances in the investigation of the thermal and magnetic properties of integrable spin ladder models and their applicability to the physics of strong coupling ladder compounds. For this class of compounds the rung coupling J ⊥ is much stronger than the coupling J ∥ along the ladder legs. The ground state properties of the integrable two-leg spin- and the mixed spin-() ladder models at zero temperature are analysed by means of the Thermodynamic Bethe Ansatz (TBA). Solving the TBA equations yields exact results for the critical fields and critical behaviour. The thermal and magnetic properties of the models are discussed in terms of the recently introduced High Temperature Expansion (HTE) method, which is reviewed in detail. In the strong coupling region the integrable spin- ladder model exhibits three quantum phases: (i) a gapped phase in the regime , (ii) a fully polarized phase for , and (iii) a Luttinger liquid magnetic phase in the regime H c1<H<H c2. The critical behaviour in the vicinity of the critical points H c1 and H c2 is of Pokrovsky-Talapov type. The temperature-dependent thermal and magnetic properties are directly evaluated from the exact free energy expression and compared to known experimental results for the strong coupling ladder compounds (5IAP)2CuBr4· 2H2O, Cu2(C5H12N2)2Cl4, (C5H12N)2CuBr4, BIP-BNO and [Cu2(C2\O 2)(C10H8N2)2)](NO3)2. Similar analysis of the mixed spin-() ladder model reveals a rich phase diagram, with a and a full saturation magnetization plateau within the strong antiferromagnetic rung coupling regime. For weak rung coupling, the fractional magnetization plateau is diminished and a new quantum phase transition occurs. The phase diagram can be directly deduced from the magnetization curve obtained from the exact result derived from the TBA and HTE. The results are applied to the mixed ferrimagnetic ladder compound PNNBNO. The thermodynamics of the spin-orbital model with different single-ion anisotropies is also discussed. For this model single-ion anisotropy can trigger different quantum phase transitions within the spin and orbital degrees of freedom, with magnetization plateaux arising from different spin and orbit Landé g-factors.

arXiv:cond-mat/0512489•Advances In Physics•May 1, 2007•63 citations

Magnetization properties of some quantum spin ladders

Kunj Tandon, Siddhartha Lal, Swapan Kumar Pati +2 more

The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-$1/2$ ladder, and a two-legged spin-$1/2$ ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an $\mathrm{XXZ}$ spin-$1/2$ chain in a magnetic field; the second-order terms give corrections to the $\mathrm{XXZ}$ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.

arXiv:cond-mat/9806111•Physical review. B, Condensed matter•Jan 1, 1999•63 citations

Spin- 12 Heisenberg ladder: Variation of entanglement and fidelity measures close to quantum critical points

Amit Tribedi, Indrani Bose

We consider a two-chain, spin-$\frac{1}{2}$ antiferromagnetic Heisenberg spin ladder in an external magnetic field $H$. The spin ladder is known to undergo second-order quantum phase transitions (QPTs) at two critical values ${H}_{c1}$ and ${H}_{c2}$ of the magnetic field. There are now known examples of strongly coupled (where the rung exchange interaction is much stronger than the nearest-neighbor intrachain exchange interaction) organic ladder compounds in which QPTs have been experimentally observed. In this paper, we investigate whether well-known bipartite entanglement meaures such as one-site von Neumann entropy, two-site von Neumann entropy, and concurrence develop special features close to the quantum critical points. As suggested by an earlier theorem, the first derivatives of the measures with respect to magnetic field are expected to diverge as $H\ensuremath{\rightarrow}{H}_{c1}$ and $H\ensuremath{\rightarrow}{H}_{c2}$. Based on numerical diagonalization data and a mapping of the strongly coupled ladder Hamiltonian onto the $XXZ$ chain Hamiltonian, for which several analytical results are known, we find that the derivatives of the entanglement measures diverge as $H\ensuremath{\rightarrow}{H}_{c2}$ but remain finite as $H\ensuremath{\rightarrow}{H}_{c1}$. The reason for this discrepancy is analyzed. We further calculate two recently proposed quantum information theoretic measures, the reduced fidelity and reduced fidelity susceptibility, and show that these measures provide appropriate signatures of the QPTs occuring at the critical points $H={H}_{c1}$ and $H={H}_{c2}$.

arXiv:0812.4106•Physical Review A•Jan 30, 2009•23 citations

Critical properties of S=12 Heisenberg ladders in magnetic fields

Mamoru Usami, Sei-ichiro Suga

The critical properties of the $S=1/2$ Heisenberg two-leg ladders are investigated in a magnetic field. Combining the exact diagonalization method and the finite-size-scaling analysis based on conformal field theory, we calculate the critical exponents of spin correlation functions numerically. For a strong interchain coupling, magnetization dependence of the critical exponents shows characteristic behavior depending on the sign of the interchain coupling. We also calculate the critical exponents for the $S=1/2$ Heisenberg two-leg ladder with a diagonal interaction, which is thought of as a model Hamiltonian of the organic spin ladder compound ${\mathrm{Cu}}_{2}(1,4\ensuremath{-}\mathrm{d}\mathrm{i}\mathrm{a}\mathrm{z}\mathrm{a}\mathrm{c}\mathrm{y}\mathrm{c}\mathrm{l}\mathrm{o}\mathrm{h}\mathrm{e}\mathrm{p}\mathrm{t}\mathrm{a}\mathrm{n}\mathrm{e}{)}_{2}{\mathrm{Cl}}_{4}.$ Numerical results are compared with experimental results of temperature dependence of the NMR relaxation rate ${1/T}_{1}.$

arXiv:cond-mat/9809088•Physical review. B, Condensed matter•Dec 1, 1998•37 citations

Exact solutions in a S=12 quantum spin ladder model with pair and quartic interactions

Jeremiah H. Barry, Mark W. Meisel

The effects of multispin interactions upon quantum spin ladders are investigated theoretically. A two-leg $S=\frac{1}{2}$ quantum spin ladder is taken to have intrarung (inter-rung) quadratic (biquadratic) Heisenberg exchange-type interactions and is placed in a uniform magnetic field. Due to the commutability properties of the Hamiltonian, the magnetic canonical partition function of the model is exactly calculable by a method of rung transfer matrix. Exact solutions are then derived for thermodynamic quantities like free and internal energies, magnetization, and magnetic susceptibilities (initial and nonlinear). The zero-temperature results comprise exact solutions in the complete interaction parameter space for the ground-state energy and degeneracy, zero-field spin gap, loci of quantum phase transitions, and the critical magnetic field.

Physical review. B, Condensed matter•Aug 1, 1998•3 citations

Magnetic-Field Effects on Two-Leg Heisenberg Antiferromagnetic Ladders: Thermodynamic Properties

Xiaoqun Wang, Lu Yu

Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in a magnetic field. Based on different magnetization behaviors, we found a disordered spin liquid, the Luttinger liquid, spin-polarized phases, and a classical regime. Our calculations in the Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu2(C5H12N2)2Cl4 are due to a quasi-one-dimensional effect rather than three-dimensional ordering.

arXiv:cond-mat/9906399•Physical Review Letters•Jun 5, 2000•80 citations
We study the field-induced quantum phase transitions (QPT) and the relevant magnetic properties of a spin-1/2 two-leg integrable spin ladder (ISL), of which the system parameters in bridging to the real compounds are determined by setting the extra interactions in the Hamiltonian of the ISL relative to the Heisenberg spin ladder to vanish in the expectation in the ground state (GS). Such an ISL analytically has the correct leading terms of both the critical fields of the two QPT's as in the real strongly-coupled compounds: gμ_BH_{c1}=J_{\perp}-J_{\parallel} and gμ_BH_{c2}=J_{\perp}+2J_{\parallel} in terms of the experimental leg (J_{\parallel}) and rung (J_{\perp}) interactions. The symmetric magnetization inflection point is located at gμ_BH_{IP}=J_{\perp}+J_{\parallel}/2. The magnetizations for the GS and at finite temperatures, as well as the susceptibility, show good agreements in various comparisons with the finite-site exact diagonalization, the transfer-matrix renormalization group numerical result, the perturbation theory, and the compounds (5IAP)2CuBr_4\cdot 2H_2O, Cu_2(C_5H{12}N_2)2Cl_4 and (C_5H{12}N)_2CuBr_4.
This article considers recent advances in the investigation of the thermal and magnetic properties of integrable spin ladder models and their applicability to the physics of strong coupling ladder compounds. For this class of compounds the rung coupling J ⊥ is much stronger than the coupling J ∥ along the ladder legs. The ground state properties of the integrable two-leg spin- and the mixed spin-() ladder models at zero temperature are analysed by means of the Thermodynamic Bethe Ansatz (TBA). Solving the TBA equations yields exact results for the critical fields and critical behaviour. The thermal and magnetic properties of the models are discussed in terms of the recently introduced High Temperature Expansion (HTE) method, which is reviewed in detail. In the strong coupling region the integrable spin- ladder model exhibits three quantum phases: (i) a gapped phase in the regime , (ii) a fully polarized phase for , and (iii) a Luttinger liquid magnetic phase in the regime H c1<H<H c2. The critical behaviour in the vicinity of the critical points H c1 and H c2 is of Pokrovsky-Talapov type. The temperature-dependent thermal and magnetic properties are directly evaluated from the exact free energy expression and compared to known experimental results for the strong coupling ladder compounds (5IAP)2CuBr4· 2H2O, Cu2(C5H12N2)2Cl4, (C5H12N)2CuBr4, BIP-BNO and [Cu2(C2\O 2)(C10H8N2)2)](NO3)2. Similar analysis of the mixed spin-() ladder model reveals a rich phase diagram, with a and a full saturation magnetization plateau within the strong antiferromagnetic rung coupling regime. For weak rung coupling, the fractional magnetization plateau is diminished and a new quantum phase transition occurs. The phase diagram can be directly deduced from the magnetization curve obtained from the exact result derived from the TBA and HTE. The results are applied to the mixed ferrimagnetic ladder compound PNNBNO. The thermodynamics of the spin-orbital model with different single-ion anisotropies is also discussed. For this model single-ion anisotropy can trigger different quantum phase transitions within the spin and orbital degrees of freedom, with magnetization plateaux arising from different spin and orbit Landé g-factors.
The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-1/21/21/2 ladder, and a two-legged spin-1/21/21/2 ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an XXZ\mathrm{XXZ}XXZ spin-1/21/21/2 chain in a magnetic field; the second-order terms give corrections to the XXZ\mathrm{XXZ}XXZ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.
We consider a two-chain, spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg spin ladder in an external magnetic field HHH. The spin ladder is known to undergo second-order quantum phase transitions (QPTs) at two critical values Hc1{H}_{c1}Hc1​ and Hc2{H}_{c2}Hc2​ of the magnetic field. There are now known examples of strongly coupled (where the rung exchange interaction is much stronger than the nearest-neighbor intrachain exchange interaction) organic ladder compounds in which QPTs have been experimentally observed. In this paper, we investigate whether well-known bipartite entanglement meaures such as one-site von Neumann entropy, two-site von Neumann entropy, and concurrence develop special features close to the quantum critical points. As suggested by an earlier theorem, the first derivatives of the measures with respect to magnetic field are expected to diverge as $H\ensuremath{\rightarrow}{H}_{c1}$ and $H\ensuremath{\rightarrow}{H}_{c2}$. Based on numerical diagonalization data and a mapping of the strongly coupled ladder Hamiltonian onto the XXZXXZXXZ chain Hamiltonian, for which several analytical results are known, we find that the derivatives of the entanglement measures diverge as $H\ensuremath{\rightarrow}{H}_{c2}$ but remain finite as $H\ensuremath{\rightarrow}{H}_{c1}$. The reason for this discrepancy is analyzed. We further calculate two recently proposed quantum information theoretic measures, the reduced fidelity and reduced fidelity susceptibility, and show that these measures provide appropriate signatures of the QPTs occuring at the critical points H=Hc1H={H}_{c1}H=Hc1​ and H=Hc2H={H}_{c2}H=Hc2​.
The critical properties of the S=1/2S=1/2S=1/2 Heisenberg two-leg ladders are investigated in a magnetic field. Combining the exact diagonalization method and the finite-size-scaling analysis based on conformal field theory, we calculate the critical exponents of spin correlation functions numerically. For a strong interchain coupling, magnetization dependence of the critical exponents shows characteristic behavior depending on the sign of the interchain coupling. We also calculate the critical exponents for the S=1/2S=1/2S=1/2 Heisenberg two-leg ladder with a diagonal interaction, which is thought of as a model Hamiltonian of the organic spin ladder compound ${\mathrm{Cu}}_{2}(1,4\ensuremath{-}\mathrm{d}\mathrm{i}\mathrm{a}\mathrm{z}\mathrm{a}\mathrm{c}\mathrm{y}\mathrm{c}\mathrm{l}\mathrm{o}\mathrm{h}\mathrm{e}\mathrm{p}\mathrm{t}\mathrm{a}\mathrm{n}\mathrm{e}{)}_{2}{\mathrm{Cl}}_{4}.$ Numerical results are compared with experimental results of temperature dependence of the NMR relaxation rate 1/T1.{1/T}_{1}.1/T1​.
The effects of multispin interactions upon quantum spin ladders are investigated theoretically. A two-leg S=12S=\frac{1}{2}S=21​ quantum spin ladder is taken to have intrarung (inter-rung) quadratic (biquadratic) Heisenberg exchange-type interactions and is placed in a uniform magnetic field. Due to the commutability properties of the Hamiltonian, the magnetic canonical partition function of the model is exactly calculable by a method of rung transfer matrix. Exact solutions are then derived for thermodynamic quantities like free and internal energies, magnetization, and magnetic susceptibilities (initial and nonlinear). The zero-temperature results comprise exact solutions in the complete interaction parameter space for the ground-state energy and degeneracy, zero-field spin gap, loci of quantum phase transitions, and the critical magnetic field.
Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in a magnetic field. Based on different magnetization behaviors, we found a disordered spin liquid, the Luttinger liquid, spin-polarized phases, and a classical regime. Our calculations in the Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu2(C5H12N2)2Cl4 are due to a quasi-one-dimensional effect rather than three-dimensional ordering.