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arXiv:cond-mat/9804151 · Acta Physica Polonica B

Quantum Antiferromagnets in a Magnetic Field

Daniel Loss, Bruce Normand

Published Apr 15, 1998• 2 citations
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Abstract

Motivated by recent experiments on low-dimensional quantum magnets in applied magnetic fields, we present a theoretical analysis of their properties based on the nonlinear sigma model. The spin stiffness and a 1/N expansion are used to map the regimes of spin-gap behavior, predominantly linear magnetization, and spin saturation. A two-parameter renormalization-group study gives the characteristic properties over the entire parameter range. The model is relevant to many systems exhibiting Haldane physics, and is applied here to the two-chain spin ladder compound CuHpCl.

DOI
10.48550/arxiv.cond-mat/9804151

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Motivated by recent experiments on low-dimensional quantum magnets in applied magnetic fields, we present a theoretical analysis of their properties based on the nonlinear sigma model. The spin stiffness and a 1/N expansion are used to map the regimes of spin-gap behavior, predominantly linear magnetization, and spin saturation. A two-parameter renormalization-group study gives the characteristic properties over the entire parameter range. The model is relevant to many systems exhibiting Haldane physics, and is applied here to the two-chain spin ladder compound CuHpCl.
Microscopic models of quantum antiferromagnets are investigated on the basis of a mapping onto effective low-energy Hamiltonians. Lattice effects are carefully taken into account and their role is discussed. We show that the presence of an external staggered magnetic field modifies in a nontrivial way the usual mapping onto the nonlinear sigma model, leading to the appearance of terms neglected in previous works. Our analysis is compared with Lanczos diagonalizations of S=1S=1S=1 Heisenberg chains in a staggered field, confirming the validity of the single-mode approximation for the evaluation of the dynamical structure factor. The results are relevant for the interpretation of experiments in quasi-one-dimensional compounds. Microscopic realizations of SU(4) spin chains are also discussed in the framework of spin-orbital lattice systems. The low-energy physics is shown to be described by sigma models with topological angle $\ensuremath{\theta}$ in one dimension. This mapping strongly suggests that the one-dimensional CP3{\mathrm{CP}}^{3}CP3 model (with $\ensuremath{\theta}=\ensuremath{\pi})$ undergoes a second-order phase transition as a function of the coupling.
We use a quantum O(N) nonlinear \ensuremath{\sigma} model to describe one-dimensional quantum Heisenberg antiferromagnets with integer spin S. A large-N analytical treatment of this effective theory leads to definite predictions for thermodynamic quantities in the low-temperature regime. We obtain the Haldane gap as a function of the temperature and note a trend similar to that found in the compound NENP. The specific heat and magnetic susceptibility are also obtained and comparison with exact numerical results for the S=1 spin chain allows us to determine the domain of validity of our approximation. By a calculation at subleading 1/N order we compute the quasiparticle lifetime. Results are given on-shell, for the width observed at the quasiparticle pole as seen in neutron-scattering experiments, and also off-shell, for the NMR relaxation rate ${\mathit{T}}_{1}^{\mathrm{\ensuremath{-}}1}$. The phenomenological interacting boson model is compared with our approach. We discuss the effects of anisotropy and compare our results with present experiments on NENP.
We study both the static and dynamic properties of gapped, one-dimensional, Heisenberg, antiferromagnetic, spin chains at finite temperature through an analysis of the O(3) nonlinear sigma model. Exploiting the integrability of this theory, we are able to compute an exact low-temperature expansion of the finite temperature correlators. We do so using a truncated ``form-factor'' expansion and so provide evidence that this technique can be successfully extended to finite temperature. As a direct test, we compute the static zero-field susceptibility and obtain an exact match to the susceptibility derived from the low-temperature expansion of the exact free energy. We also study transport properties, computing both the spin conductance and the NMR-relaxation rate, 1/T1.{1/T}_{1}.1/T1​. We find these quantities to show ballistic behavior. In particular, the computed spin conductance exhibits a nonzero Drude weight at finite temperature and zero applied field. The physics thus described differs from the spin diffusion reported by Takigawa et al. [Phys. Rev. Lett. 76, 2173 (1996)] from experiments on the Haldane gap material, AgVP2S6.{\mathrm{AgVP}}_{2}{S}_{6}.AgVP2​S6​.
The low-temperature behavior of quantum Heisenberg models can be obtained by combining a renormalization-group analysis of the quantum models with a Monte Carlo simulation of the corresponding classical model, where the ``spins'' are represented by unit vectors defined on a lattice. In this approach renormalization-group equations for the quantum models lead to an effective classical O(3) nonlinear \ensuremath{\sigma} model in appropriate regimes of the parameter space. In the present work we apply this technique, which was recently used by Chakravarty, Halperin, and Nelson to discuss the low-temperature behavior of quantum antiferromagnets, to ferromagnets and calculate the correlation length and the susceptibility of a two-dimensional quantum ferromagnet at low temperatures. The results obtained with this method are then compared with those obtained from a direct simulation of the spin S=1/2 quantum ferromagnet. Excellent agreement between the two approaches leads us to believe that the analytic expressions obtained in the renormalization-group method are accurate at low temperatures. This strengthens the validity of the procedure adopted for antiferromagnets as well, where no such simulation results are yet known. The present paper also further substantiates recent work on the properties of solid 3He^{3}\mathrm{He}3He in two dimensions.
The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-1/21/21/2 ladder, and a two-legged spin-1/21/21/2 ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an XXZ\mathrm{XXZ}XXZ spin-1/21/21/2 chain in a magnetic field; the second-order terms give corrections to the XXZ\mathrm{XXZ}XXZ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.
The behavior of Haldane-gap antiferromagnets in a strong magnetic field is not universal. While the low-energy physics of the conventional one-dimensional spin-1 Heisenberg model in its magnetized regime is described by one incommensurate soft mode, other systems with somewhat perturbed coupling constants can possess two characteristic soft modes in a certain range of the field strength. Such a two-component Luttinger liquid phase is realized above the massive Haldane-gap phase, and in general above any massive nonmagnetic phase, when the ground state exhibits short-range incommensurate fluctuations already in the absence of the field.