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arXiv:cond-mat/9709098 · Physical review. B, Condensed matter

Correlated charge polarization in a chain of coupled quantum dots

R. Kotlyar, Charles Allen Stafford, S. Das Sarma

Published Jul 15, 1998• 15 citations
arXivHTMLPDF

Abstract

Coherent charge transfer in a linear array of tunnel-coupled quantum dots, electrostatically coupled to external gates, is investigated using the Bethe ansatz for a symmetrically biased Hubbard chain. Charge polarization in this correlated system is shown to proceed via two distinct processes: formation of bound states in the metallic phase, and charge-transfer processes corresponding to a superposition of antibound states at opposite ends of the chain in the Mott-insulating phase. The polarizability in the insulating phase of the chain exhibits a universal scaling behavior, while the polarization charge in the metallic phase of the model is shown to be quantized in units of $e/2.$

DOI
10.1103/physrevb.58.r1746

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Coherent charge transfer in a linear array of tunnel-coupled quantum dots, electrostatically coupled to external gates, is investigated using the Bethe ansatz for a symmetrically biased Hubbard chain. Charge polarization in this correlated system is shown to proceed via two distinct processes: formation of bound states in the metallic phase, and charge-transfer processes corresponding to a superposition of antibound states at opposite ends of the chain in the Mott-insulating phase. The polarizability in the insulating phase of the chain exhibits a universal scaling behavior, while the polarization charge in the metallic phase of the model is shown to be quantized in units of e/2.e/2.e/2.
The quantum phase transition in two capacitively coupled arrays of superconducting quantum dots (SQD) by considering the presence of gate voltage in each superconducting island is presented. We show explicitly that the cotunneling process associated with two coupled SQD arrays, near the maximum-charge frustration line is not sufficient to explain the correct quantum phases with physically consistent phase boundaries. We consider an extra cotunneling process along each chain to explain the correct quantum phases with physically consistent phase boundaries. There is no evidence of supersolid phase in our study. The Bethe ansatz and Abelian bosonization method is used to solve the problem.
We investigate the role of strong Coulomb interactions beyond the standard Hubbard model in two distinct physical contexts. First, we analyze the superconducting phase transition occurring near the Mott metal-insulator transition. Second, we study transport properties of artificial nano-scale structures containing quantum dots coupled to external electrodes. In both cases, we focus on the impact of the correlated (assisted) hopping (CH) interaction. For superconductors, CH acts as a driving mechanism for the phase transition and modifies the spectral properties of the system. We present the evolution of the spectral function as the system approaches the Mott-type transition under varying model parameters. In quantum-dot-based devices, CH influences the tunneling amplitude between the dot and metallic leads. We demonstrate that the characteristic changes in the conductance of a normal metal-quantum dot-normal metal structure provide a clear signature of the presence and sign of CH interaction.
Quantum-mechanical correlations of interacting fermions result in the emergence of exotic phases.Magnetic phases naturally arise in the Mott-insulator regime of the Fermi-Hubbard model, where charges are localized and the spin degree of freedom remains.In this regime, the occurrence of phenomena such as resonating valence bonds, frustrated magnetism, and spin liquids is predicted.Quantum systems with engineered Hamiltonians can be used as simulators of such spin physics to provide insights beyond the capabilities of analytical methods and classical computers.To be useful, methods for the preparation of intricate many-body spin states and access to relevant observables are required.Here, we show the quantum simulation of magnetism in the Mott-insulator regime with a linear quantum-dot array.We characterize the energy spectrum for a Heisenberg spin chain, from which we can identify when the conditions for homogeneous exchange couplings are met.Next, we study the multispin coherence with global exchange oscillations in both the singlet and triplet subspace of the Heisenberg Hamiltonian.Last, we adiabatically prepare the low-energy global singlet of the homogeneous spin chain and probe it with two-spin singlettriplet measurements on each nearest-neighbor pair and the correlations therein.The methods and control presented here open new opportunities for the simulation of quantum magnetism benefiting from the flexibility in tuning and layout of gate-defined quantum-dot arrays.
The ground-state properties of quartet quantum-dot arrays are studied using the numerical renormalization group (NRG) method with a four-site Hubbard model connected to two noninteracting leads. Specifically, we calculate the conductance and local charge in the dots from the many-body phase shifts, which can be deduced from the fixed-point eigenvalues of NRG. As a function of the on-site energy ϵd{ϵ}_{d}ϵd​ which corresponds to the gate voltage, the conductance shows alternatively wide peaks and valleys. Simultaneously, the total number of electrons Nel{N}_{\mathrm{el}}Nel​ in the four dots shows a quantized staircase behavior due to a large Coulomb interaction UUU. The conductance plateaus of the unitary limit emerging for odd Nel{N}_{\mathrm{el}}Nel​ are caused by the Kondo effect. The valleys of the conductance emerge for even Nel{N}_{\mathrm{el}}Nel​, and their width becomes substantially large at half-filling. It can be regarded as a kind of the Mott-Hubbard insulating behavior manifesting in a small system. These structures of the plateaus and valleys become weak for large values of the hybridization strength $\ensuremath{\Gamma}$ between the chain and leads. We also discuss the parallel conductance for the array connected to four leads.
Strongly interacting electron systems can provide insight into quantum many-body phenomena, such as Mott insulating behavior and spin liquidity, facilitating semiconductor optimization. The Fermi-Hubbard model is the prototypical model used to study such systems. Recent research, however, has shown that the extended Fermi-Hubbard model, which accounts for long-range interactions, is more accurate, especially for systems far from half-filling. In this study, we use the extended Fermi-Hubbard model to mathematically analyze charge transport through a lattice of quantum dots. One-dimensional chains with spinless electrons and source-drain bias are observed, focusing on the transition between the ground state and the first excited state. Level repulsion decreases the expected energy levels of anticrossings as the hopping onto the chain tends to the hopping within the chain. The distribution of charge density along the chain is characterized in terms of the hopping, nuclear, and Coulomb parameters and novel plasmonic behavior is analyzed. Minor perturbations in electron transport are identified, corresponding to the one-dimensional nature of the observed systems. This research will lead to a better understanding of electron behavior in silicon-doped semiconductors, like the formation of correlation-induced band gaps, and open the door to using the extended Fermi-Hubbard model as a more accurate alternative to study quantum many-body systems.
The ground-state persistent current and electron addition spectrum in two-dimensional quantum dot arrays and one-dimensional quantum dot rings, pierced by an external magnetic flux, are investigated using the extended Hubbard model. The collective multidot problem is shown to map exactly into the strong-field noninteracting finite-size Hofstadter butterfly problem at the spin polarization transition. The finite-size Hofstadter problem is discussed, and an analytical solution for limiting values of flux is obtained. In weak fields we predict interesting flux periodic oscillations in the spin component along the quantization axis with a periodicity given by $\ensuremath{\nu}h/e$ $(\ensuremath{\nu}<~1)$. The sensitivity of the calculated persistent current to interaction and disorder is shown to reflect the intricacies of various Mott-Hubbard quantum phase transitions in two-dimensional systems: the persistent current is suppressed in the antiferromagnetic Mott-insulating phase governed by intradot Coulomb interactions; the persistent current is maximized at the spin density wave--charge density wave transition driven by the nearest-neighbor interdot interaction; the Mott-insulating phase persistent current is enhanced by the long-range interdot interactions to its noninteracting value; the strong suppression of the noninteracting current in the presence of random disorder is seen only at large disorder strengths; at half-filling even a relatively weak intradot Coulomb interaction enhances the disordered noninteracting system persistent current; in general, the suppression of the persistent current by disorder is less significant in the presence of the long-range interdot Coulomb interaction.