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arXiv:cond-mat/9611129 · Physical Review Letters

Weakly Coupled Antiferromagnetic Quantum Spin Chains

Ziqiang Wang

Published Jan 6, 1997• 40 citations
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Abstract

Quasi-one-dimensional quantum antiferromagnets formed by a $d$-dimensional hypercubic lattice of weakly coupled spin- $\frac{1}{2}$ antiferromagnetic Heisenberg chains are studied by combining exact results in one-dimension and renormalization group analyses of the interchain correlations. It is shown that $d$-dimensional magnetic long-range order develops at zero temperature for infinitesimal antiferromagnetic or ferromagnetic interchain couplings. In the presence of weak bond alternations, the order-disorder transition occurs at a finite interchain coupling. Relevances to the lightly doped quantum antiferromagnets and multilayer quantum Hall systems are discussed.

DOI
10.1103/physrevlett.78.126

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The ground-state properties of the quasi-one-dimensional spin-1/21/21/2 antiferromagnetic Heisenberg model is investigated by using a variational method. Spins on chains along the xxx direction are antiferromagnetically coupled with exchange J>0J>0J>0, while spins between chains in the yyy direction are coupled either ferromagnetically (${J}^{\ensuremath{'}}<0$) or antiferromagnetically (${J}^{\ensuremath{'}}>0$). The staggered and the colinear antiferromagnetic magnetizations are computed and their dependence on the anisotropy parameter $\ensuremath{\lambda}=|{J}^{\ensuremath{'}}|/J$ is analyzed. It is found that an infinitesimal interchain coupling parameter is sufficient to stabilize a long-range order with either a staggered magnetization ms{m}_{s}ms​ (${J}^{\ensuremath{'}}>0$) or a colinear antiferromagnetic magnetization mcaf{m}_{caf}mcaf​ (${J}^{\ensuremath{'}}<0$), both behaving as $\ensuremath{\simeq}{\ensuremath{\lambda}}^{1/2}$ for $\ensuremath{\lambda}\ensuremath{\rightarrow}0$.
We study the quenching of the Haldane gap in quasi-one-dimensional systems of weakly coupled spin-1 antiferromagnetic Heisenberg chains. The critical interchain coupling Jc required to stabilize long range magnetic order can be accurately determined from large scale quantum Monte Carlo calculations. Several different geometries of coupled chains are studied, illustrating the dependence of Jc on the coordination of chains. For bipartite geometries, ferromagnetically coupled chains yield similar magnitudes for Jc.
We study the quenching of the Haldane gap in quasi-one-dimensional systems of weakly coupled spin-1 antiferromagnetic Heisenberg chains. The critical interchain coupling Jc required to stabilize long range magnetic order can be accurately determined from large scale quantum Monte Carlo calculations. Several different geometries of coupled chains are studied, illustrating the dependence of Jc on the coordination of chains. For bipartite geometries, ferromagnetically coupled chains yield similar magnitudes for Jc.
The ordering of weakly coupled random antiferromagnetic S=1/2S=1/2S=1/2 chains, as relevant for the recent experimentally investigated spin chain materials, is considered theoretically. The one-dimensional isotropic Heisenberg model with random exchange interactions is treated numerically on finite chains with the density-matrix renormalization-group approach as well as with the standard renormalization analysis, both within the mean-field approximation for interchain coupling ${J}_{\ensuremath{\perp}}$. Results for the ordering temperature TN{T}_{N}TN​ and for the ordered moment m0{m}_{0}m0​ are presented and are both reduced with increasing disorder, agreeing with the experimental observations. The most pronounced effect of the random singlet concept appears to be a very large span of local ordered moments, becoming wider with decreasing ${J}_{\ensuremath{\perp}}$, consistent with the $\ensuremath{\mu}$-SR experimental findings.
The linear real space renormalization group is applied to study alternating spin (1/2,1) chains. The temperature dependences of the specific heat and spin–spin correlation functions for the quantum easy-axis mixed-spin chain are found. The role of single-ion anisotropy is discussed. The phase diagram of Ising spin chains with antiferromagnetic intrachain interactions and weak ferromagnetic interchain interactions is presented. As one expects, the weak interchain coupling leads to antiferrimagnetic long-range order in several chains. The threshold value of single-ion anisotropy below which the system does not exhibit a phase transition is found.
We study weakly coupled antiferromagnetic spin chains in their ordered phase by combining an exact solution of the single-chain problem with a random-phase-approximation analysis of the interchain interaction. A single chain is described by a quantum Sine-Gordon model and dynamical staggered susceptibilities are determined by employing the form-factor approach to quantum correlation functions. We consider both antiferromagnetic order encountered in quasi-one-dimensional materials such as KCuF3{\mathrm{KCuF}}_{3}KCuF3​ and spin-Peierls order as found in CuGeO3.{\mathrm{CuGeO}}_{3}.CuGeO3​.