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arXiv:cond-mat/9611050

Memory function approach to the Hall constant in strongly correlated electron systems: Part II

Ekkehard Lange

Published Nov 7, 1996• 0 citations
arXivHTMLPDF

Abstract

The anomalous frequency and doping dependence of the Hall constant in the normal state of high-T_c superconductors are investigated within models of strongly correlated electron systems. In Mori theory, the transition of the Hall constant from infinite to zero frequency is described by a memory function. It naturally introduces a second time scale, that, within the t-J model, is identified with the spinon relaxation time of Anderson. This provides us with a phenomenological understanding of the interplay between the frequency and temperature dependence of the Hall constant for frequencies below the Mott-Hubbard gap. Within the single-band Hubbard model in the limit $U\gg t$, the memory function is calculated via its moments and shown to project out the high-energy scale U. This causes the Hall constant to decrease by a factor $(1+δ)/2$ ($δ$: doping), when the frequency is lowered from infinity to values within the Mott-Hubbard gap. Finally, it is outlined, how the Hall constant may be calculated in the low frequency regime.

DOI
10.48550/arxiv.cond-mat/9611050

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The anomalous frequency and doping dependence of the Hall constant in the normal state of high-T_c superconductors are investigated within models of strongly correlated electron systems. In Mori theory, the transition of the Hall constant from infinite to zero frequency is described by a memory function. It naturally introduces a second time scale, that, within the t-J model, is identified with the spinon relaxation time of Anderson. This provides us with a phenomenological understanding of the interplay between the frequency and temperature dependence of the Hall constant for frequencies below the Mott-Hubbard gap. Within the single-band Hubbard model in the limit U≫tU\gg tU≫t, the memory function is calculated via its moments and shown to project out the high-energy scale U. This causes the Hall constant to decrease by a factor (1+δ)/2(1+δ)/2(1+δ)/2 (δδδ: doping), when the frequency is lowered from infinity to values within the Mott-Hubbard gap. Finally, it is outlined, how the Hall constant may be calculated in the low frequency regime.
We investigate the Hall effect in two different theoretical models of strongly correlated systems: a system made of weakly coupled Luttinger liquids, in the presence of umklapp scattering, and the 2D triangular lattice, with nearest-neighbor hopping and a local Hubbard interaction. In the first model we use a memory function approach to compute the Hall coefficient as a function of temperature and frequency in the presence of umklapp scattering. We find a power-law correction to the free-fermion value (band value), with an exponent depending on the Luttinger parameter KρK_ρKρ​. At sufficiently high temperature or frequency the Hall coefficient approaches the band value. We discuss the applications to Hall experiments made in quasi 1D organic compounds. In the second model, the complete temperature and doping dependencies of the high-frequency Hall coefficient $\RH$ are evaluated analytically and numerically for small, intermediate, and strong interactions using various approximation schemes. We find that $\RH$ follows the semiclassical 1/qn∗1/qn^*1/qn∗ law near T=0, but exhibits a striking TTT-linear behavior with an interaction- and doping-dependent slope at high temperature. We compare our results with Hall measurements performed in cobaltates.
Low energy properties of the metallic state of the two-dimensional t - J model are presented for second neighbor hopping with hole-doping ( ) and electron-doping ( ), with various superexchange energy J . We use a closed set of equations for the Greens functions obtained from the extremely correlated Fermi liquid theory . These equations reproduce the known low energies features of the large U Hubbard model in infinite dimensions. The density and temperature dependent quasiparticle weight, decay rate and the peak spectral heights over the Brillouin zone are calculated. We also calculate the resistivity, Hall conductivity, Hall number and cotangent Hall angle. The spectral features display high thermal sensitivity at modest T for density , implying a suppression of the effective Fermi-liquid temperature by two orders of magnitude relative to the bare bandwidth. The cotangent Hall angle exhibits a T 2 behavior at low T , followed by an interesting kink at higher T . The Hall number exhibits strong renormalization due to correlations. Flipping the sign of changes the curvature of the resistivity versus T curves between convex and concave. Our results provide a natural route for understanding the observed difference in the temperature dependent resistivity of strongly correlated electron-doped and hole-doped matter.
The Hall coefficient exhibits anomalous behavior in lightly doped Mott insulators. For strongly interacting electrons its computation has been challenged by analytical and numerical obstacles. We calculate the leading contributions in the recently derived thermodynamic formula for the Hall coefficient. We obtain its doping and temperature dependence for the square lattice tJ-model at high temperatures. The second order corrections are evaluated to be negligible. Quantum Monte Carlo sampling extends our results to lower temperatures. We find a divergence of the Hall coefficient toward the Mott limit and a sign reversal relative to Boltzmann equation's weak scattering prediction. The Hall current near the Mott phase is carried by a low density of spin-entangled vacancies, which should constitute the Cooper pairs in any superconducting phase at lower temperatures.
We investigate the onset of a not-decaying asymptotic behavior of temporal magnetic correlations in the Hubbard model in infinite dimensions. This long-term memory feature of dynamical spin correlations can be precisely quantified by computing the difference between the zero-frequency limit of the Kubo susceptibility and the corresponding static isothermal one. Here, we present a procedure for reliably evaluating this difference starting from imaginary time-axis data, and apply it to the testbed case of the Mott-Hubbard metal-insulator transition (MIT). At low temperatures, we find long-term memory effects in the entire Mott regime, abruptly ending at the first order MIT. This directly reflects the underlying local moment physics and the associated degeneracy in the many-electron spectrum. At higher temperatures, a more gradual onset of an infinitely-long time-decay of magnetic correlations occurs in the crossover regime, not too far from the Widom line emerging from the critical point of the MIT. Our work has relevant algorithmic implications for the analytical continuation of dynamical susceptibilities in strongly correlated regimes and offers a new perspective for unveiling fundamental properties of the many-particle spectrum of the problem under scrutiny.
We investigate the onset of a not-decaying asymptotic behavior of temporal magnetic correlations in the Hubbard model in infinite dimensions. This long-term memory feature of dynamical spin correlations can be precisely quantified by computing the difference between the zero-frequency limit of the Kubo susceptibility and the corresponding static isothermal one. Here, we present a procedure for reliably evaluating this difference starting from imaginary time-axis data, and apply it to the testbed case of the Mott-Hubbard metal-insulator transition (MIT). At low temperatures, we find long-term memory effects in the entire Mott regime, abruptly ending at the first order MIT. This directly reflects the underlying local moment physics and the associated degeneracy in the many-electron spectrum. At higher temperatures, a more gradual onset of an infinitely-long time-decay of magnetic correlations occurs in the crossover regime, not too far from the Widom line emerging from the critical point of the MIT. Our work has relevant algorithmic implications for the analytical continuation of dynamical susceptibilities in strongly correlated regimes and offers a new perspective for unveiling fundamental properties of the many-particle spectrum of the problem under scrutiny.
The principal purpose of this topical review is to single out some of the universal features of high-temperature (high-Tc) and related strongly-correlated systems, which can be compared with experiment in a quantitative manner. The description starts with the concept of exchange-interaction-mediated (real-space) pairing, combined with strong correlations among narrow band electrons, for which the reference state is that of the Mott–Hubbard insulator. The physical discussion of concrete properties relies on variational approach, starting from generalized renormalized mean-field theory (RMFT) in the form of statistically-consistent Gutzwiller approximation (SGA), and its subsequent generalization, i.e., a systematic Diagrammatic Expansion of the Variational (Gutzwiller-type) Wave Function (DE-GWF). The solution leads to the two energy scales, one involving unconventional quasiparticles close to the Fermi energy, and the other reflecting the fully correlated state, involving electrons deeper below the Fermi surface. Those two regimes are separated by a kink in the dispersion relation, which is observed in photoemission. As a result, one obtains both the doping dependent properties in the correlated state, and effective renormalized quasiparticles. The reviewed ground-state characteristics for high-Tc systems encompass high-Tc superconductivity, nematicity, charge- (and pair-) density-wave effects, as well as non-BCS kinetic energy gain in the paired state. The calculated dynamic properties are: the universal Fermi velocity, the Fermi wave-vector, the effective mass enhancement, the pseudogap; and the d-wave gap magnitude. We discuss that, within the variational approach, the minimal realistic model is represented by the so-called t-J-U Hamiltonian. Inadequacy of the t-J and Hubbard models, particularly of their RMFT versions, is discussed explicitly. For heavy fermion systems, modeled by the Anderson lattice model and with the DE-GWF approach, we discuss the phase diagram, encompassing superconducting, Kondo insulating, ferro- and anti-ferromagnetic states. The superconducting state is then a two-d-wave gap system. If the orbital degeneracy of f-electrons is included, the coexistent ferromagnetic- (spin–triplet) superconducting phases appear and match those observed for UGe2 in a semiquantitative manner. Finally, in the second part, we generalize our approach to the collective spin and charge fluctuations in high-Tc systems, starting from variational approach, defining the saddle-point state, and combining it with 1/N expansion. The present scheme differs essentially from that starting from the saddle-point Hartree–Fock approximation, and incorporating the fluctuations in the random phase approximation (RPA). The spectrum of collective spin and charge excitations is determined for the Hubbard and t-J-U models, and subsequently compared quantitatively with recent experiments. The Appendices provide formal details to make this review self-contained.