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arXiv:cond-mat/9602100 · Physical review. B, Condensed matter

Overscreened single-channel Kondo problem

Anirvan M. Sengupta, Yong Baek Kim

Published Dec 1, 1996• 19 citations
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Abstract

We consider the single-channel Kondo problem with the Kondo coupling between a spin $S$ impurity and conduction electrons with spin $j$. These problems arise as multicritical points in the parameter spaces of two-and higher-level tunneling systems and some impurity models of heavy fermion compounds. In contrast to the previous Bethe-ansatz conjectures, it turns out that the dynamics of the spin sector is the same as that of a spin-$S$ impurity coupled to $k(j)$ channels of spin-\textonehalf{} electrons with $k(j)=2\frac{j(j+1)(2j+1)}{3}$. As a result, for $2S<k(j)$, the system shows non-Fermi-liquid behavior with the same exponents for the thermodynamic quantities as those of the $k(j)$-channel Kondo problem. However, both the finite-size spectrum and the operator content are different due to the presence of the other sectors and can be obtained by conformal field theory techniques.

DOI
10.1103/physrevb.54.14918

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We consider the single-channel Kondo problem with the Kondo coupling between a spin SSS impurity and conduction electrons with spin jjj. These problems arise as multicritical points in the parameter spaces of two-and higher-level tunneling systems and some impurity models of heavy fermion compounds. In contrast to the previous Bethe-ansatz conjectures, it turns out that the dynamics of the spin sector is the same as that of a spin-SSS impurity coupled to k(j)k(j)k(j) channels of spin-\textonehalf{} electrons with k(j)=2j(j+1)(2j+1)3k(j)=2\frac{j(j+1)(2j+1)}{3}k(j)=23j(j+1)(2j+1)​. As a result, for 2S<k(j)2S<k(j)2S<k(j), the system shows non-Fermi-liquid behavior with the same exponents for the thermodynamic quantities as those of the k(j)k(j)k(j)-channel Kondo problem. However, both the finite-size spectrum and the operator content are different due to the presence of the other sectors and can be obtained by conformal field theory techniques.
The Kondo problem, which describes the interaction of a spin sss magnetic impurity with a free Fermi gas, is a classic example of strongly coupled physics. Historically, the problem has been solved by Wilson's numerical renormalization group and later by Bethe ansatz. In this paper, we present an alternate analytic solution of the Kondo problem that combines an expansion in 1/s1/s1/s with the renormalization group. We study both the case of an impurity interacting with a single channel K=1K=1K=1 of fermions in the s→∞s \rightarrow \inftys→∞ limit and the case with KKK channels in the double-scaling limit K→∞K \rightarrow \inftyK→∞, s→∞s \to \inftys→∞, K/sK/sK/s fixed. Our approach allows us to describe analytically intermediate scales of the Kondo problem at large sss and compute thermodynamic observables such as the impurity entropy and susceptibility. We find these observables to agree with the Bethe ansatz results. We also compute the impurity spectral function, finite temperature resistivity and the Kondo screening cloud profile, properties that are not easily accessible from Bethe ansatz. Notably, in the regime K>2sK > 2sK>2s we access the "non-Fermi-liquid" overscreened fixed point of the multichannel Kondo problem.
The traditional multichannel Kondo effect takes place when several gapless metallic electronic channels interact with a localized spin-SSS impurity, with the number of channels nnn exceeding the size of the impurity spin, n>2Sn>2Sn>2S, leading to the emergence of non-Fermi liquid impurity behavior at low temperatures. Here, we show that the effect can be realized even when the electronic degrees of freedom are strongly correlated and gapped. The system under consideration consists of a single spin-12\frac{1}{2}21​ impurity coupled isotropically to nnn spin singlet superconducting channels realized by one-dimensional leads with quasi-long-range superconducting order. The competition between the Kondo and superconducting fluctuations induces multiple distinct ground states and boundary phases depending on the relative strengths of the bulk and boundary interactions. Using the Bethe Ansatz technique, we identify four regimes: an overscreened Kondo phase, a zero-mode phase, a Yu-Shiba-Rusinov (YSR) phase, and a local-moment phase with an unscreened impurity, each with its own experimental characteristic. We describe the renormalization-group flow, the excitation spectrum, and the full impurity thermodynamics in each phase. Remarkably, even in the presence of a bulk mass gap, the boundary critical behavior in the Kondo phase is governed by the same exponents as in the gapless theory with the low-energy impurity sector flowing to the SU(2)nSU(2)_nSU(2)n​ Wess-Zumino-Witten (WZW) fixed point, and the impurity entropy monotonically decreasing as a function of temperature. In both the overscreened Kondo and zero-mode phases, the residual impurity entropy is Simp(T→0)=ln⁡[2cos⁡(π/(n+2))]S_{\mathrm{imp}}(T \to 0) = \ln[2\cos(π/(n+2))]Simp​(T→0)=ln[2cos(π/(n+2))]. In the YSR and unscreened phases on the other hand the impurity entropy exhibits non-monotonic temperature dependence and is effectively free at low temperatures with Simp(T→0)=ln⁡2S_{\mathrm{imp}}(T \to 0) = \ln 2Simp​(T→0)=ln2.
We propose a possible realization of the overscreened Kondo impurity problem by a magnetic s=1/2s=1/2s=1/2 impurity embedded in a two-dimensional S=1S=1S=1 U(1)U(1)U(1) spin liquid with a Fermi surface. This problem contains an interesting interplay between non-Fermi-liquid behavior induced by a U(1)U(1)U(1) gauge field coupled to fermions and a non-Fermi-liquid fixed point in the overscreened Kondo problem. Using a large-NNN expansion together with an expansion in the dynamical exponent of the gauge field, we find that the coupling to the gauge field leads to weak but observable changes in the physical properties of the system at the overscreened Kondo fixed point. We discuss the extrapolation of this result to a physical case and argue that the realization of overscreened Kondo physics could lead to observations of effects due to gauge fields.
The non-Fermi-liquid fixed point of the overscreened Kondo problem is studied in the limit of a large number of conduction electron channels, k\ensuremath{\gg}1, using perturbation theory in 1/k. By expanding the beta function and self-energy to sub-leading-order in 1/k, we examine the scaling, thermodynamics, and dynamic response functions in detail. Our results compliment and extend previous work based on conformal field theory. We present the dynamical spin susceptibility for the first time and show that the impurity spin is marginally quenched, with an inelastic linewidth of order T.
The multichannel Kondo model with SU(N)\mathrm{SU}(N)SU(N) spin symmetry and SU(K)\mathrm{SU}(K)SU(K) channel symmetry is considered. The impurity spin is chosen to transform as an antisymmetric representation of SU(N),\mathrm{SU}(N),SU(N), corresponding to a fixed number of Abrikosov fermions ${\ensuremath{\sum}}_{\ensuremath{\alpha}}{f}_{\ensuremath{\alpha}}^{\ifmmode\dagger\else\textdagger\fi{}}{f}_{\ensuremath{\alpha}}=Q.$ For more than one channel (K>1),(K>1),(K>1), and all values of NNN and Q,Q,Q, the model displays non-Fermi behavior associated with the overscreening of the impurity spin. Universal low-temperature thermodynamic and transport properties of this non-Fermi-liquid state are computed using conformal field theory methods. A large-NNN limit of the model is then considered, in which $K/N\ensuremath{\equiv}\ensuremath{\gamma}$ and $Q/N\ensuremath{\equiv}{q}_{0}$ are held fixed. Spectral densities satisfy coupled integral equations in this limit, corresponding to a (time-dependent) saddle point. A low-frequency, low-temperature analysis of these equations reveals universal scaling properties in the variable $\ensuremath{\omega}/T,$ in agreement with conformal invariance. The universal scaling form is obtained analytically and used to compute the low-temperature universal properties of the model in the large-NNN limit, such as the T=0T=0T=0 residual entropy and residual resistivity, and the critical exponents associated with the specific heat and susceptibility. The connections with the ``noncrossing approximation'' and the previous work of Cox and Ruckenstein are discussed.
We investigate quantum transport through the Kondo impurity assuming both a large number of orbital channels $\mathcal{K}\ensuremath{\gg}1$ for the itinerant electrons and a semiclassical spin $\mathcal{S}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}1$ for the impurity. The non-Fermi-liquid regime of the Kondo problem is achieved in the overscreened sector K>2S\mathcal{K}>2\mathcal{S}K>2S. We show that there exist two distinct semiclassical regimes for the quantum transport through impurity: (i) $\mathcal{K}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}\mathcal{S}\phantom{\rule{4pt}{0ex}}\ensuremath{\gg}\phantom{\rule{4pt}{0ex}}1$, differential conductance vanishes, and (ii) S/K=C\mathcal{S}/\mathcal{K}=\mathcal{C}S/K=C with 0<C<1/20<\mathcal{C}<1/20<C<1/2, differential conductance reaches some nonvanishing fraction of its unitary value. Using the conformal field theory approach we analyze the behavior of the quantum transport observables and residual entropy in both semiclassical regimes. We show that the semiclassical limit (ii) preserves the key features of resonance scattering and the most essential fingerprints of the non-Fermi-liquid behavior. We discuss possible realization of two semiclassical regimes in semiconductor quantum transport experiments.