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arXiv:cond-mat/9406025 · Physical Review Letters

Disorder Induced Phase Transition in a Two-Dimensional Random Quantum Antiferromagnet

Anders W. Sandvik, Marco Vekić

Published Feb 13, 1995• 36 citations
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Abstract

A two-dimensional Heisenberg model with random antiferromagnetic nearest-neighbor exchange is studied using quantum Monte Carlo techniques. As the strength of the randomness is increased, the system undergoes a transition from an antiferromagnetically ordered ground state to a gapless disordered state. The finite-size scaling of the staggered structure factor and susceptibility is consistent with a dynamic exponent $z=2$.

DOI
10.1103/physrevlett.74.1226

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A two-dimensional Heisenberg model with random antiferromagnetic nearest-neighbor exchange is studied using quantum Monte Carlo techniques. As the strength of the randomness is increased, the system undergoes a transition from an antiferromagnetically ordered ground state to a gapless disordered state. The finite-size scaling of the staggered structure factor and susceptibility is consistent with a dynamic exponent z=2z=2z=2.
Ground state properties of the randomly diluted two-dimensional Heisenberg antiferromagnet are discussed. Quantum Monte Carlo (stochastic series expansion) data for L×L lattices, with L up to 64, are extrapolated to infinite size for dilution fractions p between 0 (clean system) and p* (the percolation threshold). The sublattice magnetization is calculated using a decomposition into a classical and a quantum mechanical factor, which are evaluated separately. The quantum mechanical factor (the sublattice magnetization of the largest connected cluster of magnetic sites) remains finite at the percolation threshold, implying that the dilution driven order-disorder transition is a classical percolation transition. The spin stiffness is calculated using the winding number fluctuations.
Using quantum Monte Carlo simulations, we study effects of disorder on the S=1/2S=1/2S=1/2 Heisenberg model with exchange constant JJJ on the square lattice supplemented by multispin interactions QQQ. It was found recently [L. Liu et al., Phys. Rev. X 8, 041040 (2018)] that the ground state of this $J\ensuremath{-}Q$ model with random couplings undergoes a quantum phase transition from the N\'eel antiferromagnetic state into a randomness-induced spin-liquid-like state that is a close analog to the well known random-singlet (RS) state of the Heisenberg chain with random couplings. This 2D RS state arises from a spontaneously symmetry-broken fourfold degenerate columnar valence-bond solid that is broken up by the disorder into finite domains, with spinons localized at topological defects. The interacting spinons form a critical collective many-body state without magnetic long range order but with the mean spin-spin correlations decaying with distance rrr as ${r}^{\ensuremath{-}2}$, as in the one-dimensional RS state. The dynamic exponent $z\ensuremath{\ge}2$, varying continuously with the model parameters. In this work, we further investigate the properties of the RS state in the $J\ensuremath{-}Q$ model with random QQQ couplings. We study the temperature dependence of the specific heat and various susceptibilities for large enough systems to reach the thermodynamic limit. We also analyze the size dependence of the critical magnetic order parameter and its susceptibility in the ground state. For all these quantities, we find consistency with the conventional quantum-critical scaling laws when the condition implied by the ${r}^{\ensuremath{-}2}$ form of the spin correlations is imposed. In particular, all the different quantities can be explained by the same value of the dynamic exponent zzz at fixed model parameters. We argue that the RS state identified in the $J\ensuremath{-}Q$ model corresponds to a generic renormalization group fixed point that can be reached in many quantum magnets with random couplings and that it has already been observed experimentally.
The two-dimensional antiferromagnetic S=1/2 Heisenberg model with random bond dilution is studied using quantum Monte Carlo simulation at the percolation threshold (50% of the bonds removed). Finite-size scaling of the staggered structure factor averaged over the largest connected clusters of sites on L*L lattices shows that long-range order exists within the percolating fractal clusters in the thermodynamic limit. This implies that the order-disorder transition driven by bond-dilution occurs exactly at the percolation threshold and that the exponents are classical. This result should apply also to the site-diluted system.
We use quantum Monte Carlo simulations to study a disordered S=1/2S=1/2S=1/2 Heisenberg quantum spin model with three different nearest-neighbor interactions, ${J}_{1}\ensuremath{\le}{J}_{2}\ensuremath{\le}{J}_{3}$, on the square lattice. We consider the regime in which J1{J}_{1}J1​ represents weak bonds, and J2{J}_{2}J2​ and J3{J}_{3}J3​ correspond to two kinds of stronger bonds (dimers) which are randomly distributed on columns forming coupled two-leg ladders. When increasing the average intradimer coupling (J2+J3)/2({J}_{2}+{J}_{3})/2(J2​+J3​)/2, the system undergoes a N\'eel to quantum glass transition of the ground state and later a second transition into a quantum paramagnet. The quantum glass phase is of the gapless Mott glass type (i.e., in boson language it is incompressible at temperature T=0T=0T=0), and we find that the temperature dependence of the uniform magnetic susceptibility follows the stretched exponential form $\ensuremath{\chi}\ensuremath{\sim}exp(\ensuremath{-}b/{T}^{\ensuremath{\alpha}})$, with $0<\ensuremath{\alpha}<1$. At the N\'eel-glass transition, we observe the standard O(3) critical exponents, which implies that the Harris criterion for the relevance of the disorder is violated in this system.
A model of spin-polarized fermions hopping on a two-dimensional lattice with a near-neighbor repulsive interaction is simulated with the use of Monte Carlo methods. This system exhibits an Ising-like order-disorder phase transition as the temperature is lowered. Results for the structure factor, staggered susceptibility, and order parameter are obtained, and finite-size scaling on lattices of 4\ifmmode\times\else\texttimes\fi{}4, 6\ifmmode\times\else\texttimes\fi{}6, and 8\ifmmode\times\else\texttimes\fi{}8 is used to estimate Tc{T}_{c}Tc​ and test the nature of the phase transition.
We present Monte Carlo simulations of a two-dimensional bilayer quantum Heisenberg antiferromagnet with random dimer dilution. In contrast with exotic scaling scenarios found in other random quantum systems, the quantum phase transition in this system is characterized by a finite-disorder fixed point with power-law scaling. After accounting for corrections to scaling, with a leading irrelevant exponent of omega approximately 0.48, we find universal critical exponents z=1.310(6) and nu=1.16(3). We discuss the consequences of these findings and suggest new experiments.