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arXiv:cond-mat/9909230

The two-dimensional bond-diluted quantum Heisenberg model at the classical percolation threshold

Anders W. Sandvik

Published Sep 15, 1999• 0 citations
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Abstract

The two-dimensional antiferromagnetic S=1/2 Heisenberg model with random bond dilution is studied using quantum Monte Carlo simulation at the percolation threshold (50% of the bonds removed). Finite-size scaling of the staggered structure factor averaged over the largest connected clusters of sites on L*L lattices shows that long-range order exists within the percolating fractal clusters in the thermodynamic limit. This implies that the order-disorder transition driven by bond-dilution occurs exactly at the percolation threshold and that the exponents are classical. This result should apply also to the site-diluted system.

DOI
10.48550/arxiv.cond-mat/9909230

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The two-dimensional antiferromagnetic S=1/2 Heisenberg model with random bond dilution is studied using quantum Monte Carlo simulation at the percolation threshold (50% of the bonds removed). Finite-size scaling of the staggered structure factor averaged over the largest connected clusters of sites on L*L lattices shows that long-range order exists within the percolating fractal clusters in the thermodynamic limit. This implies that the order-disorder transition driven by bond-dilution occurs exactly at the percolation threshold and that the exponents are classical. This result should apply also to the site-diluted system.
The two-dimensional antiferromagnetic S=1/2S=1/2S=1/2 Heisenberg model with random site dilution is studied using quantum Monte Carlo simulations. Ground-state properties of the largest connected cluster on $L\ifmmode\times\else\texttimes\fi{}L$ lattices, with L up to 64, are calculated at the classical percolation threshold. In addition, clusters with a fixed number Nc{N}_{c}Nc​ of spins on an infinite lattice at the percolation density are studied for Nc{N}_{c}Nc​ up to 1024. The disorder averaged sublattice magnetization per spin extrapolates to the same nonzero infinite-size value for both types of clusters. Hence, the percolating clusters, which are fractal with dimensionality d=91/48,d=91/48,d=91/48, have antiferromagnetic long-range order. This implies that the order-disorder transition driven by site dilution occurs exactly at the percolation threshold and that the exponents are classical. The same conclusion is reached for the bond-diluted system. The full sublattice magnetization versus site dilution curve is obtained in terms of a decomposition into a classical geometrical factor and a factor containing all the effects of quantum fluctuations. The spin stiffness is shown to obey the same scaling as the conductivity of a random resistor network.
Ground state properties of the randomly diluted two-dimensional Heisenberg antiferromagnet are discussed. Quantum Monte Carlo (stochastic series expansion) data for L×L lattices, with L up to 64, are extrapolated to infinite size for dilution fractions p between 0 (clean system) and p* (the percolation threshold). The sublattice magnetization is calculated using a decomposition into a classical and a quantum mechanical factor, which are evaluated separately. The quantum mechanical factor (the sublattice magnetization of the largest connected cluster of magnetic sites) remains finite at the percolation threshold, implying that the dilution driven order-disorder transition is a classical percolation transition. The spin stiffness is calculated using the winding number fluctuations.
Quantum phase transition of site-diluted and bond-diluted Heisenberg antiferromagnets on square lattices is studied. By using the novel continuous-time loop algorithm, we perform quantum Monte Carlo simulations on quite larger lattices at extremely lower temperatures than the previous numerical studies. It is found that the antiferromagnetic long-range order at T = 0 persists so long as a cluster of magnetic sites percolates, that is, the critical concentration is equal to the classical percolation threshold, in both of the site-diluted and bond-diluted cases. Furthermore, we find that some critical exponents, such as the magnetization exponent β, are non-classical and strongly depend on the spin size S. On the other hand, we show that the correlation-length exponent ν is universal and is equal to the classical value (ν=4/3).
We investigate the quantum dynamics of site diluted S=1/2 Heisenberg antiferromagnetic clusters at the 2D percolation threshold. We use Lanczos diagonalization to calculate the lowest excitation gap Delta and, to reach larger sizes, use quantum Monte Carlo simulations to study an upper bound for Delta obtained from sum rules involving the staggered structure factor and susceptibility. Scaling the gap distribution with the cluster length L, Delta approximately L(-), we obtain a dynamic exponent z approximately 2D(f), where D(f)=91/48 is the fractal dimensionality of the percolating cluster. This is in contrast with previous expectations of z=D(f). We argue that the low-energy excitations are due to weakly coupled effective moments formed due to local imbalance in sublattice occupation.
Ground-state magnetic properties of the diluted Heisenberg antiferromagnet on a square lattice are investigated by means of the quantum Monte Carlo method with the continuous-time loop algorithm. It is found that the critical concentration of magnetic sites is independent of the spin size S, and equal to the two-dimensional percolation threshold. However, the existence of quantum fluctuations makes the critical exponents deviate from those of the classical percolation transition. Furthermore, we found that the transition is not universal, i.e., the critical exponents significantly depend on S.
Randomly diluted quantum boson and spin models in two dimensions combine the physics of classical percolation with the well-known dimensionality dependence of ordering in quantum lattice models. This combination is rather subtle for models that order in two dimensions but have no true order in one dimension, as the percolation cluster near threshold is a fractal of dimension between 1 and 2: two experimentally relevant examples are the O(2)O(2)O(2) quantum rotor and the Heisenberg antiferromagnet. We study two analytic descriptions of the O(2)O(2)O(2) quantum rotor near the percolation threshold. First a spin-wave expansion is shown to predict long-ranged order, but there are statistically rare points on the cluster that violate the standard assumptions of spin-wave theory. A real-space renormalization group (RSRG) approach is then used to understand how these rare points modify ordering of the O(2)O(2)O(2) rotor. A new class of fixed points of the RSRG equations for disordered one-dimensional bosons is identified and shown to support the existence of long-range order on the percolation backbone in two dimensions. These results are relevant to experiments on bosons in optical lattices and superconducting arrays, and also (qualitatively) for the diluted Heisenberg antiferromagnet ${\mathrm{La}}_{2}{(\mathrm{Zn},\mathrm{Mg})}_{x}{\mathrm{Cu}}_{1\ensuremath{-}x}{\mathrm{O}}_{4}$.