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arXiv:cond-mat/0703308 · Physical Review A

Condensates of strongly interacting atoms and dynamically generated dimers

Eric Braaten, Dongqing Zhang

Published Jun 22, 2007• 1 citation
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Abstract

In a system of atoms with large positive scattering length, weakly bound diatomic molecules (dimers) are generated dynamically by the strong interactions between the atoms. If the atoms are modeled by a quantum field theory with an atom field only, condensates of dimers cannot be described by the mean-field approximation because there is no field associated with the dimers. We develop a method for describing dimer condensates in such a model based on the one-particle-irreducible (1PI) effective action. We construct an equivalent 1PI effective action that depends not only on the classical atom field but also on a classical dimer field. The method is illustrated by applying it to the many-body behavior of bosonic atoms with large scattering length at zero temperature using an approximation in which the two-atom amplitude is treated exactly, but irreducible $N$-atom amplitudes for $N\ensuremath{\geqslant}3$ are neglected. The two 1PI effective actions give identical results for the atom superfluid phase, but the one with a classical dimer field is much more convenient for describing the dimer superfluid phase. The results are also compared with previous work on the Bose gas near a Feshbach resonance.

DOI
10.1103/physreva.75.063624

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•Jan 1, 2011•1 citation
In a system of atoms with large positive scattering length, weakly bound diatomic molecules (dimers) are generated dynamically by the strong interactions between the atoms. If the atoms are modeled by a quantum field theory with an atom field only, condensates of dimers cannot be described by the mean-field approximation because there is no field associated with the dimers. We develop a method for describing dimer condensates in such a model based on the one-particle-irreducible (1PI) effective action. We construct an equivalent 1PI effective action that depends not only on the classical atom field but also on a classical dimer field. The method is illustrated by applying it to the many-body behavior of bosonic atoms with large scattering length at zero temperature using an approximation in which the two-atom amplitude is treated exactly, but irreducible NNN-atom amplitudes for N\ensuremath⩾3N\ensuremath{\geqslant}3N\ensuremath⩾3 are neglected. The two 1PI effective actions give identical results for the atom superfluid phase, but the one with a classical dimer field is much more convenient for describing the dimer superfluid phase. The results are also compared with previous work on the Bose gas near a Feshbach resonance.
We consider weakly bound diatomic molecules (dimers) formed in a two-component atomic Fermi gas with a large positive scattering length for the interspecies interaction. We develop a theoretical approach for calculating atom-dimer and dimer-dimer elastic scattering and for analyzing the inelastic collisional relaxation of the molecules into deep bound states. This approach is based on the single-channel zero-range approximation, and we find that it is applicable in the vicinity of a wide two-body Feshbach resonance. Our results draw prospects for various interesting manipulations of weakly bound dimers of fermionic atoms.
A Feshbach resonance in the s-wave scattering length occurs if the energy of the two atoms in the incoming open channel is close to the energy of a bound state in a coupled closed channel. Starting from the microscopic Hamiltonian that describes this situation, we derive the effective atom–molecule theory for a Bose gas near a Feshbach resonance. In order to take into account all two-body processes, we have to dress the bare couplings of the atom–molecule model with ladder diagrams. This results in a quantum field theory that exactly reproduces the scattering amplitude of the atoms and the bound-state energy of the molecules. Since these properties are incorporated at the quantum level, the theory can be applied both above and below the critical temperature of the gas. Moreover, making use of the true interatomic potentials ensures that no divergences are encountered at any stage of the calculation. We also present the mean-field theory for the Bose–Einstein condensed phase of the gas.
A dynamical many-body theory is presented which systematically extends beyond mean-field and perturbative quantum-field theoretical procedures. It allows us to study the dynamics of strongly interacting quantum-degenerate atomic gases. The nonperturbative approximation scheme is based on a systematic expansion of the two-particle irreducible effective action in powers of the inverse number of field components. This yields dynamic equations which contain direct scattering, memory, and ``off-shell'' effects that are not captured by the Gross-Pitaevskii equation. This is relevant to account for the dynamics of, e.g., strongly interacting quantum gases atoms near a scattering resonance, or of one-dimensional Bose gases in the Tonks-Girardeau regime. We apply the theory to a homogeneous ultracold Bose gas in one spatial dimension. Considering the time evolution of an initial state far from equilibrium we show that it quickly evolves to a nonequilibrium quasistationary state and discuss the possibility to attribute an effective temperature to it. The approach to thermal equilibrium is found to be extremely slow.
In the strong-coupling Bose-Einstein condensation (BEC) region where a Feshbach resonance gives rise to tightly bound dimer molecules, we show that a spin-polarized Fermi superfluid reduces to a simple Bose-Fermi mixture of Bose-condensed dimers and the leftover unpaired fermions. Using a many-body functional integral formalism, the Gaussian fluctuations give rise to an induced dimer-dimer interaction mediated by the unpaired fermions, with the dimer-fermion vertex being given by the (mean-field) Born approximation. Treating the pairing fluctuations to quartic order, we show how the action for a spin-polarized Fermi superfluid reduces to one for a Bose-Fermi mixture. This Bose-Fermi action includes an expression for the effective dimer-unpaired fermion interaction in a spin-polarized Fermi superfluid beyond the Born approximation, in the BEC limit. In the low-density limit, we show how this dimer-fermion interaction gives the sss-wave scattering length aBF=1.18aF{a}_{\mathit{BF}}=1.18{a}_{F}aBF​=1.18aF​ (aF{a}_{F}aF​ is the sss-wave fermion scattering length), a result first derived by Skorniakov and Ter-Martirosian in 1957 for three interacting fermions.
We argue that the energy of a strongly interacting gas in the unitary limit is parametrized by a universal constant β. For fermions, this parameter is known, but not for bosons. Finding β for bosons is the goal of this thesis. We present the basics of scattering theory, including the s-wave scattering length, which is the characteristic length scale for the interactions at low energies and which goes to infinity at unitarity. Shape and Feshbach resonances are explained. The conventional theory for Bose gases, Bogoliubov theory, is presented, which takes into account quantum fluctuations. It is used to derive identities for the groundstate energy, the condensate fraction and the contact. These are given as expansions in the scattering length, which therefore only hold true for weak interactions. To improve on this, we present an effective action from an atom-molecule theory, which also allows bound states. By a mean-field approach we derive universal identities for the associated energy scales, and in the unitary limit an analytical expression is found for the chemical potential, from which the value β = −0.54 is found. However, this mean-field result is qualitatively not reliable, since quantum depletion is neglected. A new approach is introduced, starting with a Jastrow Ansatz, from which the energy is expressed in the Jastrow function f and radial distribution function g. A cluster expansion is made for g, where a diagrammatic analogy is found. The Hyper-Netted Chain approximation is introduced to calculate g systematically by summing infinitely many diagrams. In HNC/0, we minimize the energy by a variational method, which is based on a well-constructed Ansatz for g. Numerical results using the HNC/0 approximation are given not only for the ground-state energy, but also for the condensate density and the contact. For large scattering lengths the calculations became increasingly less accurate, but the results from Bogoliubov theory are correctly included for small a. An extrapolation for the ground-state energy is made to find β ' −0.20, which is expected to be an upper bound. Moreover, quantum depletion is found to be higher when calculated in HNC/0 for large scattering lengths. Also, it is found that the contact at this value for unitarity remains finite and acquires the value of C ' 10.3n4/3, which is remarkably close to the value for fermions, C ' 11n4/3. Cover image courtesy of [18].