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arXiv:cond-mat/0612229 · NATO science for peace and security series. B, Physics and biophysics

A Gentle Introduction to the Functional Renormalization Group: The Kondo Effect in Quantum Dots

Sabine Andergassen, Tilman Enss, Christoph Karrasch, V. Meden

Published Jan 1, 2008• 18 citations
arXivHTMLPDF
DOI
10.1007/978-1-4020-8512-3_1

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Kondo physics first surfaced into the scientific world in 1934 via an unexpected observations made by a group of experimentalists, who measured the temperature-dependent resistance of gold wires in their laboratory at the University of Leiden. When decreasing the temperature below 4 Kelvin, they observed an unexpected increase of the resistance, which resulted in a resistance minimum that was not accounted for by the theoretical understanding at that time. Only 30 years later, Jun Kondo, a Japanese physicist from Tokyo, was the first to explain this curiosity, known as the Kondo effect, under the assistance of the Kondo model. Although his findings explained the increased resistance, a more fundamental problem was raised: the Kondo problem, an unphysical divergence of the resistance at very low temperatures. To solve this problem required the development of more advanced methods beyond the scope of pure perturbative methods, namely the use of renormalization group (RG) methods. More than twenty years after Kondo’s first steps towards the solution of the resistance minimum, the Kondo effect experienced a scientific revival due to the emergence of quantum dot systems in solid state physics. A quantum dot is a very localized and spatially restricted area within a metal, where only a few electrons fit in the area. The limited spatial spread constrains the possible positions for the electrons on the dot, and forces them into strong interactions with each other–they are strongly correlated. In quantum dot systems, not only the Kondo effect in equilibrium situations between the dot and its surrounding reservoirs can be studied, but also the effects of nonequilibrium situations, where a finite bias voltage drives a current through the quantum dot. However, the nonequilibrium Kondo effect is far less explored compared to its equilibrium counterpart and it requires the development of new methods beyond established equilibrium methods. To fill this gap, we use the recently developed real-time renormalization group (RTRG) method in the weak-coupling regime and its extension to the crossover regime, from weak coupling to strong coupling. Furthermore, different combinations between the number of electrons on the dot and the number of reservoirs of electrons in the surrounding metal allow for distinct physical situations, which can be studied within the framework of the RTRG method. We subsequently characterize the properties of the the overscreened, the underscreened, and the fully screened Kondo model by analyzing their physical observables and, in parts, their time evolution. The perturbative foundation of the RTRG method gives us the opportunity to gather new analytic insights for higher spin Kondo systems, on the one hand, and provides for a qualitative comparison of obtained results to various other methods and analytic results, on the other hand.

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The Anderson Impurity Model is a generic model to describe systems in which one or more energy levels are coupled to an electronic host. On the energy levels the electrons are subject to a Coulomb interaction. Possible applications of this model are magnetic atoms in a metal or quantum dot systems. Already for one impurity it displays very interesting physics including the well known Kondo effect. For two and more impurities the properties of the system in the local moment regime are determined by an interplay of the Kondo effect and the coupling between the impurity spins. Due to the interplay of multiple energy scales, this model poses a serious task for any computational tool. For a single impurity the model can be very efficiently treated using Wilson"s numerical renormalization group (NRG). Since the numerical effort of NRG calculations rises exponentially with the number of impurities, generically it cannot be applied to systems with more than two impurities. The functional renormalization group (fRG) has been very successfully applied to quantum impurity problems in the past. In this work it will be used to calculate the single-particle dynamics for Anderson-like quantum impurity systems in equilibrium. A comparison to NRG in the case of a single impurity will serve as a benchmark before systems with two impurities and quantum dot systems with two and three dots will be studied. The interplay between the Kondo effect and magnetic and orbital ordering will be investigated in these systems. Although the truncation in the presented fRG scheme is motivated by second order perturbation theory, it will be shown that fRG works also in those cases where perturbation theory fails. Generally it will turn out that fRG is capable of treating a broad variety of Anderson impurity systems within the same framework, including asymmetric impurity levels and interaction between multiple impurities.

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Many-particle States in the Theory of the Kondo Effect

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Journal of Experimental and Theoretical Physics•Jan 1, 1972•0 citations
Kondo physics first surfaced into the scientific world in 1934 via an unexpected observations made by a group of experimentalists, who measured the temperature-dependent resistance of gold wires in their laboratory at the University of Leiden. When decreasing the temperature below 4 Kelvin, they observed an unexpected increase of the resistance, which resulted in a resistance minimum that was not accounted for by the theoretical understanding at that time. Only 30 years later, Jun Kondo, a Japanese physicist from Tokyo, was the first to explain this curiosity, known as the Kondo effect, under the assistance of the Kondo model. Although his findings explained the increased resistance, a more fundamental problem was raised: the Kondo problem, an unphysical divergence of the resistance at very low temperatures. To solve this problem required the development of more advanced methods beyond the scope of pure perturbative methods, namely the use of renormalization group (RG) methods. More than twenty years after Kondo’s first steps towards the solution of the resistance minimum, the Kondo effect experienced a scientific revival due to the emergence of quantum dot systems in solid state physics. A quantum dot is a very localized and spatially restricted area within a metal, where only a few electrons fit in the area. The limited spatial spread constrains the possible positions for the electrons on the dot, and forces them into strong interactions with each other–they are strongly correlated. In quantum dot systems, not only the Kondo effect in equilibrium situations between the dot and its surrounding reservoirs can be studied, but also the effects of nonequilibrium situations, where a finite bias voltage drives a current through the quantum dot. However, the nonequilibrium Kondo effect is far less explored compared to its equilibrium counterpart and it requires the development of new methods beyond established equilibrium methods. To fill this gap, we use the recently developed real-time renormalization group (RTRG) method in the weak-coupling regime and its extension to the crossover regime, from weak coupling to strong coupling. Furthermore, different combinations between the number of electrons on the dot and the number of reservoirs of electrons in the surrounding metal allow for distinct physical situations, which can be studied within the framework of the RTRG method. We subsequently characterize the properties of the the overscreened, the underscreened, and the fully screened Kondo model by analyzing their physical observables and, in parts, their time evolution. The perturbative foundation of the RTRG method gives us the opportunity to gather new analytic insights for higher spin Kondo systems, on the one hand, and provides for a qualitative comparison of obtained results to various other methods and analytic results, on the other hand.
The Anderson Impurity Model is a generic model to describe systems in which one or more energy levels are coupled to an electronic host. On the energy levels the electrons are subject to a Coulomb interaction. Possible applications of this model are magnetic atoms in a metal or quantum dot systems. Already for one impurity it displays very interesting physics including the well known Kondo effect. For two and more impurities the properties of the system in the local moment regime are determined by an interplay of the Kondo effect and the coupling between the impurity spins. Due to the interplay of multiple energy scales, this model poses a serious task for any computational tool. For a single impurity the model can be very efficiently treated using Wilson"s numerical renormalization group (NRG). Since the numerical effort of NRG calculations rises exponentially with the number of impurities, generically it cannot be applied to systems with more than two impurities. The functional renormalization group (fRG) has been very successfully applied to quantum impurity problems in the past. In this work it will be used to calculate the single-particle dynamics for Anderson-like quantum impurity systems in equilibrium. A comparison to NRG in the case of a single impurity will serve as a benchmark before systems with two impurities and quantum dot systems with two and three dots will be studied. The interplay between the Kondo effect and magnetic and orbital ordering will be investigated in these systems. Although the truncation in the presented fRG scheme is motivated by second order perturbation theory, it will be shown that fRG works also in those cases where perturbation theory fails. Generally it will turn out that fRG is capable of treating a broad variety of Anderson impurity systems within the same framework, including asymmetric impurity levels and interaction between multiple impurities.