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arXiv:cond-mat/0610646 · Physical Review Letters

Theory of the Quantum Critical Fluctuations in Cuprate Superconductors

Vivek Aji, Chandra Mohan Varma

Published Aug 9, 2007• 89 citations
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Abstract

The statistical mechanics of the time-reversal and inversion symmetry breaking order parameter, possibly observed in the pseudogap region of the phase diagram of the cuprates, can be represented by the Ashkin-Teller model. We add kinetic energy and dissipation to the model for a quantum generalization and show that the spectrum of the quantum-critical fluctuations is of the form postulated in 1989 to give the marginal Fermi-liquid properties. The model solved and the methods devised are likely to be of interest also to other quantum phase transitions.

DOI
10.1103/physrevlett.99.067003

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The statistical mechanics of the time-reversal and inversion symmetry breaking order parameter, possibly observed in the pseudogap region of the phase diagram of the cuprates, can be represented by the Ashkin-Teller model. We add kinetic energy and dissipation to the model for a quantum generalization and show that the spectrum of the quantum-critical fluctuations is of the form postulated in 1989 to give the marginal Fermi-liquid properties. The model solved and the methods devised are likely to be of interest also to other quantum phase transitions.
In a recent paper [V. Aji and C. M. Varma, Phys. Rev. Lett. 99, 067003 (2007)] we have shown that the dissipation driven quantum phase transition of the two-dimensional XYXYXY model represents a universality class where the correlations at criticality are local in space and power law in time. Here we provide a detailed analysis of the model. The local criticality is brought about by the decoupling of infrared singularities in space and time. The former leads to a Kosterlitz-Thouless transition whereby the excitations of the transverse component of the velocity field (vortices) unbind in space. The latter, on the other hand, leads to a transition among excitations (warps) in the longitudinal component of the velocity field, which unbind in time. The quantum Ashkin-Teller model, with which the observed loop order in the cuprates is described, maps in the critical regime to the quantum XYXYXY model. We also discuss other models which are expected to have similar properties.
Within the phase fluctuation model for the pseudogap state of cuprate superconductors we identify a novel statistical "Berry phase" interaction between the nodal quasiparticles and fluctuating vortex-antivortex excitations. The effective action describing this model assumes the form of an anisotropic Euclidean quantum electrodynamics in (2+1) dimensions (QED (3)) and naturally generates non-Fermi liquid behavior for its fermionic excitations. The doping axis in the x -T phase diagram emerges as a quantum critical line which regulates the low energy fermiology.
This thesis presents seven research papers on topics in condensed-matter theory. Five of the papers report on Monte Carlo studies of quantum phase transitions in various (d+1)-dimensional statistical mechanics models featuring Caldeira-Leggettlike dissipation. The principal motivation for these studies was to investigate a particular bond-dissipative (2+1)-dimensional XY model of circulating currents in cuprate high-temperature superconductors. It has been proposed that quantum critical fluctuations associated with a local quantum critical point described by this model can explain the marginal-Fermi-liquid behaviour of the normal state of these compounds. We present simulation results for this model for both compact and noncompact phase variables and show unambiguously that the quantum critical point in the compact case is not local. If the phases are taken to be noncompact variables, the model is also a model of resistively shunted Josephson junction arrays. The results in this case reveal a more complicated phase diagram, but we have not been able to establish critical behaviour consistent with the scenario of local quantum criticality.\n\nThe study of extended quantum dissipative models is also motivated by the general effect on condensed-matter systems of the coupling to environmental degrees of freedom. Their influence on quantum critical phenomena is characterized by the dynamical critical exponent z, a measure of spatiotemporal anisotropy, the value of which can be estimated by naive scaling arguments. We confirm by numerical means that such scaling estimates give correct results to a good approximations (with a few reservations), irrespective of system dimensionality, order parameter symmetry, or whether the variables are compact or noncompact. Corrections to the naive scaling estimates have to be invoked for strongly super-Ohmic dissipation for d = 1 due to relatively large values of the anomalous scaling dimension η.\n\nThe two last research papers are concerned with the superconducting pairing state of the recently discovered class of iron-based high-temperature superconductors. Here, we calculate possible signatures of the proposed s±-wave pairing state in conductance-spectroscopy and Josephson-effect experiments.
Abstract We present a T = 0 K renormalization group (RG) phase diagram for the hole-doped 2D Hubbard model on the square lattice. The RG method employed is nonperturbative in treating quantum fluctuations of the single-particle occupation number via the unitarily decoupling of one electronic state at every RG step. As a result, the RG phase diagram possesses the quantum fluctuation energy scale (ω) as one of its axes. Using effective Hamiltonians and wavefunctions for the low-energy many-body eigenstates for the doped Mott liquid obtained from the stable fixed point of the RG flows, we demonstrate the collapse of the pseudogap for charge excitations (Mottness) at a quantum critical point (QCP) possessing a nodal non-Fermi liquid with superconducting fluctuations, and spin-pseudogapping near the antinodes. The QCP is characterised using both thermodynamic and quantum information-theoretic measures. d-wave superconducting order is shown to arise from this quantum critical state of matter. The pseudogap phase possesses a variety of fluctuations that lead to several symmetry-broken phases at low-energies. Benchmarking of the ground state energy per particle and the double-occupancy fraction obtained from a finite-size scaling analysis against existing numerical results yields excellent agreement. We present detailed insight into the T = 0 origin of several experimentally observed findings in the cuprates, including Homes law and Planckian dissipation. We also establish that the heirarchy of temperature scales for the pseudogap (T PG), onset temperature for pairing (T ons), formation of the Mott liquid (T ML) and superconductivity (T C) obtained from our analysis is quantitatively consistent with that observed experimentally for some members of the cuprates. Our results offer insight on the ubiquitous origin of superconductivity in doped Mott insulating states, and pave the way towards a systematic search for higher superconducting transition temperatures in such systems.
The phase diagram of the superconducting cuprates is a manifestation of quantum phase transition (QPT). There is still controversy if the quantum fluctuations generating the pseudogap region is a precursor to the superconducting region or they are competing phases. By modelling the basic possible Hamiltonian for this class of materials as a nonlinear dynamic system, using doping as the tuning parameter, it is possible to obtain a visualized phase diagram which captures fairly the phase diagram of the superconducting cuprates. The numerical results depict that as we doped from slight to optimal, there are three quantum critical points (QCPs): the first at the QPT from the Mott insulator and antiferromagnetic (AFM) phase to the pseudogap at slight doping, the second at the QPT from the pseudogap to the superconducting phase at minimum doping and the third is a hidden QPT due to collapse of the pseudogap around optimal doping. Therefore, the results obtained here in the context of nonlinear dynamic visualization shed new light on the study of the phase diagram of the high TC superconducting cuprates.
The two-dimensional quantum XY model, with a Caldeira-Leggett form of dissipation, is applicable to the quantum-critical properties of diverse experimental systems, ranging from superconductor to insulator transitions, ferromagnetic and antiferromagnetic transitions in metals, to the loop-current order transition in cuprates. We solve the reexpression of this model in terms of orthogonal topological excitations, vortices, and a variety of instantons, by renormalization group methods. The calculations explain the extraordinary properties of the model discovered in Monte Carlo calculations: the product form of the quantum-critical fluctuations in space and time, a spatial correlation length proportional to the logarithm of the temporal correlation length near the transition from a disordered to a fully ordered state, and the occurrence of a phase with spatial order without temporal order. They are intimately related to the flow of the metric of time in relation to the metric of space, i.e., of the dynamical critical exponent zzz. These properties appear to be essential in understanding the strange metallic phase found in a variety of quantum-critical transitions as well as the accompanying high-temperature superconductivity.